干旱区生态环境知识资源中心(Arid): Thermoelectrically Regulating Heat Flux in Metal-Organic Framework Monoliths for High-Yield Atmospheric Water Harvesting in Arid Regions

Arid

DOI	10.1021/acs.iecr.4c02097
	Thermoelectrically Regulating Heat Flux in Metal-Organic Framework Monoliths for High-Yield Atmospheric Water Harvesting in Arid Regions
	Tao, Yingle; Zhu, Baokun; Zhu, Dunru; Li, Haiqing
通讯作者	Li, HQ
来源期刊	INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH
ISSN	0888-5885
EISSN	1520-5045
出版年	2024
卷号	63 期号:31 页码:13600-13610
英文摘要	The efficacy of atmospheric water harvesting (AWH) using metal-organic frameworks (MOFs) has been greatly hindered by insufficient heat regulation within MOFs. Herein, a sandwich-structured thermoelectric cooler (TEC)-integrated MIL-101(Cr) monolith (MOF/TEC/MOF, MTM) is developed. By leveraging the Peltier effect of TEC, the MTM allows for reversible heat transfer between its two MOF sides, simultaneously creating a cold MOF side for atmospheric water capture and a hot MOF side for water release. This not only maintains the water adsorption process at low temperatures, facilitating water adsorption at low RH, but also achieves effective recycling of water adsorption heat for water release. Benefiting from these advantages, a continuous MTM-based AWH device achieves water productivity of 3.7 LH2O kg-1 day-1 at 30% RH and 25 degrees C. Thermoelectrically regulating heat flux in MOFs demonstrates a groundbreaking strategy for achieving high-yield AWH in arid regions.
类型	Article
语种	英语
收录类别	SCI-E
WOS记录号	WOS:001276232300001
WOS关键词	ADSORPTION
WOS类目	Engineering, Chemical
WOS研究方向	Engineering
资源类型	期刊论文
条目标识符	http://119.78.100.177/qdio/handle/2XILL650/404167
推荐引用方式 GB/T 7714	Tao, Yingle,Zhu, Baokun,Zhu, Dunru,et al. Thermoelectrically Regulating Heat Flux in Metal-Organic Framework Monoliths for High-Yield Atmospheric Water Harvesting in Arid Regions[J],2024,63(31):13600-13610.
APA	Tao, Yingle,Zhu, Baokun,Zhu, Dunru,&Li, Haiqing.(2024).Thermoelectrically Regulating Heat Flux in Metal-Organic Framework Monoliths for High-Yield Atmospheric Water Harvesting in Arid Regions.INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH,63(31),13600-13610.
MLA	Tao, Yingle,et al."Thermoelectrically Regulating Heat Flux in Metal-Organic Framework Monoliths for High-Yield Atmospheric Water Harvesting in Arid Regions".INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH 63.31(2024):13600-13610.