Arid
DOI10.1021/acsapm.3c01561
All-Weather Atmospheric Water Harvesting Enabled by Hygroscopic Hydrogel Paint
Wang, Ling; Li, Yawen; Yu, Yang; Guo, Luxuan; Li, Chencan; Zhang, Zhuo
通讯作者Zhang, Z
来源期刊ACS APPLIED POLYMER MATERIALS
ISSN2637-6105
出版年2023
卷号5期号:11页码:9063-9075
英文摘要Hygroscopic hydrogels have been receiving widespread attention as effective atmospheric water harvesters due to their freshwater production capabilities for alleviating water scarcity stress in arid regions. Nevertheless, not only can the hydrophilic networks notably hinder water release but also harsh preparation conditions (UV light and oxygen-free environment) are required to achieve free-radical polymerization. Herein, facile and processable moisture-harvesting hydrogel paints (MHPs) have been developed to address these challenges. Benefiting from the high tunability and processability, the MHPs can be optionally cured into moisture-harvesting hydrogels (MHGs) with different sizes by various operations according to actual circumstances, manifesting their potential for multiscenario applications. Via the synergistic effect of thermal-responsive networks and hygroscopic components, the MHGs can harvest atmospheric water with a broad range of relative humidities (RH, 10-90%), high water uptake (highest similar to 50% of hydrogel's own weight at similar to 90% RH, 25 degrees C within 24 h), fast moisture-absorbing rate (up to similar to 0.23 g g(-1) h(-1) at similar to 90% RH, 25 degrees C), low energy, rapid water release rate (similar to 0.2 g g(-1) h(-1) at similar to 90% RH, 4 degrees C), and outstanding cycling stability. Also demonstrated is a proof-of-concept outdoor water-collecting system, which possesses similar to 2.5 mL g(-1) (L kg(-1)) water yield per day to satisfy an adult's daily water demand. Our low-cost and easy-to-scale-up MHGs can provide a viable solution to design next-generation atmospheric water harvesters for achieving efficient, sustainable, and multiscenario applications.
英文关键词atmospheric water harvester hydrogel paint thermal-responsive network hygroscopic component multiscenario application
类型Article
语种英语
收录类别SCI-E
WOS记录号WOS:001103626900001
WOS类目Materials Science, Multidisciplinary ; Polymer Science
WOS研究方向Materials Science ; Polymer Science
资源类型期刊论文
条目标识符http://119.78.100.177/qdio/handle/2XILL650/394936
推荐引用方式
GB/T 7714
Wang, Ling,Li, Yawen,Yu, Yang,et al. All-Weather Atmospheric Water Harvesting Enabled by Hygroscopic Hydrogel Paint[J],2023,5(11):9063-9075.
APA Wang, Ling,Li, Yawen,Yu, Yang,Guo, Luxuan,Li, Chencan,&Zhang, Zhuo.(2023).All-Weather Atmospheric Water Harvesting Enabled by Hygroscopic Hydrogel Paint.ACS APPLIED POLYMER MATERIALS,5(11),9063-9075.
MLA Wang, Ling,et al."All-Weather Atmospheric Water Harvesting Enabled by Hygroscopic Hydrogel Paint".ACS APPLIED POLYMER MATERIALS 5.11(2023):9063-9075.
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