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DOI10.3390/ijms232315193
One-Step Pyrolysis of Nitrogen-Containing Chemicals and Biochar Derived from Walnut Shells to Absorb Polycyclic Aromatic Hydrocarbons (PAHs)
Wang, Wendong; Li, Donghua; Xiang, Ping; Zheng, Yunwu; Zheng, Zhifeng; Lin, Xu; He, Xiahong; Liu, Can
通讯作者He, XH ; Liu, C
来源期刊INTERNATIONAL JOURNAL OF MOLECULAR SCIENCES
EISSN1422-0067
出版年2022
卷号23期号:23
英文摘要The pyrolysis of biomass is an efficient means of utilizing biomass resources. Biomass can be converted into various high-performance chemicals and functional materials through pyrolysis. However, current pyrolysis technologies suffer from low conversion rates and single products, so the preparation of nitrogen compounds with high economic value remains a challenge. The walnut shell was soaked in three nitrogen-containing compound solutions before carbonization to produce high-value-added nitrogen-containing chemicals (with a nitrogen content of 59.09%) and biochar for the adsorption of polycyclic aromatic hydrocarbons (PAHs). According to biochar analysis, biochar has a porous structure with a specific surface area of 1161.30 m(2)/g and a high level of rocky desertification. The surface forms a dense pyrrole structure, and the structure produces pi-pi interactions with naphthalene molecules, exhibiting excellent naphthalene adsorption with a maximum capacity of 214.98 mg/g. This study provides an efficient, rapid, and environmentally friendly method for producing nitrogen-containing chemicals with high-added value and biochar.
英文关键词walnut shell pyrolysis nitrogenous chemicals PAHs biochar
类型Article
语种英语
开放获取类型Green Published, gold
收录类别SCI-E
WOS记录号WOS:000897257200001
WOS关键词N-CONTAINING COMPOUNDS ; AQUEOUS-SOLUTION ; ACTIVATED CARBONS ; NAPHTHALENE ; ADSORPTION ; REMOVAL ; ACID ; PHENANTHRENE ; CONVERSION ; EVOLUTION
WOS类目Biochemistry & Molecular Biology ; Chemistry, Multidisciplinary
WOS研究方向Biochemistry & Molecular Biology ; Chemistry
资源类型期刊论文
条目标识符http://119.78.100.177/qdio/handle/2XILL650/393203
推荐引用方式
GB/T 7714
Wang, Wendong,Li, Donghua,Xiang, Ping,et al. One-Step Pyrolysis of Nitrogen-Containing Chemicals and Biochar Derived from Walnut Shells to Absorb Polycyclic Aromatic Hydrocarbons (PAHs)[J],2022,23(23).
APA Wang, Wendong.,Li, Donghua.,Xiang, Ping.,Zheng, Yunwu.,Zheng, Zhifeng.,...&Liu, Can.(2022).One-Step Pyrolysis of Nitrogen-Containing Chemicals and Biochar Derived from Walnut Shells to Absorb Polycyclic Aromatic Hydrocarbons (PAHs).INTERNATIONAL JOURNAL OF MOLECULAR SCIENCES,23(23).
MLA Wang, Wendong,et al."One-Step Pyrolysis of Nitrogen-Containing Chemicals and Biochar Derived from Walnut Shells to Absorb Polycyclic Aromatic Hydrocarbons (PAHs)".INTERNATIONAL JOURNAL OF MOLECULAR SCIENCES 23.23(2022).
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