Arid
DOI10.1038/s41561-022-00901-w
Dominant role of mineral dust in cirrus cloud formation revealed by global-scale measurements
Froyd, Karl D.; Yu, Pengfei; Schill, Gregory P.; Brock, Charles A.; Kupc, Agnieszka; Williamson, Christina J.; Jensen, Eric J.; Ray, Eric; Rosenlof, Karen H.; Bian, Huisheng; Darmenov, Anton S.; Colarco, Peter R.; Diskin, Glenn S.; Bui, ThaoPaul; Murphy, Daniel M.
通讯作者Froyd, KD (corresponding author),NOAA, Chem Sci Lab, Boulder, CO 80305 USA. ; Froyd, KD (corresponding author),Univ Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA.
来源期刊NATURE GEOSCIENCE
ISSN1752-0894
EISSN1752-0908
出版年2022-02
英文摘要Airborne mineral dust particles can act as natural seeds for cirrus clouds in the upper troposphere. However, the atmospheric abundance of dust is unconstrained in cirrus-forming regions, hampering our ability to predict these radiatively important clouds. Here we present global-scale measurements of dust aerosol abundance in the upper troposphere and incorporate these into a detailed cirrus-formation model. We show that dust aerosol initiates cirrus clouds throughout the extra-tropics in all seasons and dominates cirrus formation in the Northern Hemisphere (75-93% of clouds seasonally). Using a global transport model with improved dust treatment, we also explore which of Earth's deserts are the largest contributors of dust aerosol to cirrus-forming regions. We find that the meteorological environment downstream of each emission region modulates dust atmospheric lifetime and transport efficiency to the upper troposphere so that source contributions are disproportionate to emissions. Our findings establish the critical role of dust in Earth's climate system through the formation of cirrus clouds. Cirrus cloud formation in the Northern Hemisphere is primarily triggered by mineral dust, according to global-scale dust observations and a cirrus-formation model.
类型Article ; Early Access
语种英语
收录类别SCI-E
WOS记录号WOS:000761836900003
WOS关键词IN-SITU MEASUREMENTS ; SIZE DISTRIBUTIONS ; ICE NUCLEATION ; FORMATION MECHANISMS ; PARTICLE ANALYSIS ; TIBETAN PLATEAU ; DESERT DUST ; AEROSOL ; SENSITIVITY ; PHASE
WOS类目Geosciences, Multidisciplinary
WOS研究方向Geology
资源类型期刊论文
条目标识符http://119.78.100.177/qdio/handle/2XILL650/377231
作者单位[Froyd, Karl D.; Yu, Pengfei; Schill, Gregory P.; Brock, Charles A.; Kupc, Agnieszka; Williamson, Christina J.; Jensen, Eric J.; Ray, Eric; Rosenlof, Karen H.; Murphy, Daniel M.] NOAA, Chem Sci Lab, Boulder, CO 80305 USA; [Froyd, Karl D.; Yu, Pengfei; Schill, Gregory P.; Williamson, Christina J.; Jensen, Eric J.; Ray, Eric] Univ Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA; [Yu, Pengfei] Jinan Univ, Inst Environm & Climate Res, Guangzhou, Peoples R China; [Kupc, Agnieszka] Univ Vienna, Fac Phys Aerosol Phys & Environm Phys, Vienna, Austria; [Bian, Huisheng; Darmenov, Anton S.; Colarco, Peter R.] NASA, Goddard Space Flight Ctr, Greenbelt, MD USA; [Bian, Huisheng] Univ Maryland Baltimore Cty, Baltimore, MD USA; [Diskin, Glenn S.] NASA, Langley Res Ctr, Hampton, VA 23665 USA; [Bui, ThaoPaul] NASA, Ames Res Ctr, Moffett Field, CA 94035 USA
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GB/T 7714
Froyd, Karl D.,Yu, Pengfei,Schill, Gregory P.,et al. Dominant role of mineral dust in cirrus cloud formation revealed by global-scale measurements[J],2022.
APA Froyd, Karl D..,Yu, Pengfei.,Schill, Gregory P..,Brock, Charles A..,Kupc, Agnieszka.,...&Murphy, Daniel M..(2022).Dominant role of mineral dust in cirrus cloud formation revealed by global-scale measurements.NATURE GEOSCIENCE.
MLA Froyd, Karl D.,et al."Dominant role of mineral dust in cirrus cloud formation revealed by global-scale measurements".NATURE GEOSCIENCE (2022).
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