Knowledge Resource Center for Ecological Environment in Arid Area
DOI | 10.1016/j.envpol.2022.118875 |
Multisize particulate matter and volatile organic compounds in arid and semiarid areas of Northwest China | |
Zhou, Xi; Li, Zhongqin; Zhang, Tingjun; Wang, Feiteng; Tao, Yan; Zhang, Xin | |
通讯作者 | Li, ZQ (corresponding author),Chinese Acad Sci, State Key Lab Cryospher Sci, Northwest Inst Ecoenvironm & Resources, Lanzhou 730000, Peoples R China. ; Li, ZQ (corresponding author),Chinese Acad Sci, Tianshan Glaciol Stn, Lanzhou 730000, Peoples R China. |
来源期刊 | ENVIRONMENTAL POLLUTION |
ISSN | 0269-7491 |
EISSN | 1873-6424 |
出版年 | 2022 |
卷号 | 300 |
英文摘要 | To investigate the chemical components, sources, and interactions of particulate matter (PM) and volatile organic compounds (VOCs), a field campaign was implemented during the spring of 2018 in nine cities in northwestern (NW) China. PM was mainly contributed by organic matter and water-soluble inorganic ions (41% for PM10 and approximately 60% for PM2.5 and PM1). Two typical haze patterns were observed: anthropogenic pollution type (AP-type), wherein contributions of sulfate, nitrate, and ammonium (SNA) increased, and dust pollution type (DP-type), wherein contributions of Ca2+ increased and SNA decreased. Source appointment suggested that regional sources contributed close to half to PM2.5 pollution (40% for AP-type and 50% for DPtype). Thus, sources from regional transport are also important for haze and dust pollution. The ranking of VOC concentrations was methanol > acetaldehyde > formic acid + ethanol > acetone. Compared with other cities, there are higher oxygenated VOCs (OVOCs) and lower aromatics in NW China. The relationships between VOCs and PM were discussed. The dominating secondary organic aerosols (SOA) formation potential precursors were C10-aromatics, xylene, and styrene under low-nitrogen oxide (NOx) conditions, and benzene, C10-aromatics, and toluene dominated under high-NOx conditions. The quadratic polynomial was the most suitable fitting model for their correlation, and the results suggested that VOC oxidations explained 6.1-10.8% and 9.9-20.7% of SOA formation under high-NOx and low-NOx conditions, respectively. |
英文关键词 | Particulate matter Volatile organic compounds PTR-MS Black carbon NW China |
类型 | Article |
语种 | 英语 |
收录类别 | SCI-E |
WOS记录号 | WOS:000758454600002 |
WOS关键词 | YANGTZE-RIVER DELTA ; ABSORPTION ANGSTROM EXPONENT ; REACTION MASS-SPECTROMETRY ; SOURCE APPORTIONMENT ; CHEMICAL-CHARACTERIZATION ; AEROSOL FORMATION ; BLACK CARBON ; ATMOSPHERIC CHEMISTRY ; SOURCE IDENTIFICATION ; BACKGROUND SITE |
WOS类目 | Environmental Sciences |
WOS研究方向 | Environmental Sciences & Ecology |
资源类型 | 期刊论文 |
条目标识符 | http://119.78.100.177/qdio/handle/2XILL650/376183 |
作者单位 | [Zhou, Xi; Zhang, Tingjun; Tao, Yan] Lanzhou Univ, Coll Earth & Environm Sci, Minist Educ, Key Lab Western Chinas Environm Syst, Lanzhou 730000, Peoples R China; [Li, Zhongqin; Wang, Feiteng; Zhang, Xin] Chinese Acad Sci, State Key Lab Cryospher Sci, Northwest Inst Ecoenvironm & Resources, Lanzhou 730000, Peoples R China; [Li, Zhongqin; Wang, Feiteng; Zhang, Xin] Chinese Acad Sci, Tianshan Glaciol Stn, Lanzhou 730000, Peoples R China; [Li, Zhongqin] Shihezi Univ, Coll Sci, Shihezi 832000, Xinjiang, Peoples R China; [Li, Zhongqin] Northwest Normal Univ, Coll Geog & Environm Sci, Lanzhou 730000, Peoples R China |
推荐引用方式 GB/T 7714 | Zhou, Xi,Li, Zhongqin,Zhang, Tingjun,et al. Multisize particulate matter and volatile organic compounds in arid and semiarid areas of Northwest China[J],2022,300. |
APA | Zhou, Xi,Li, Zhongqin,Zhang, Tingjun,Wang, Feiteng,Tao, Yan,&Zhang, Xin.(2022).Multisize particulate matter and volatile organic compounds in arid and semiarid areas of Northwest China.ENVIRONMENTAL POLLUTION,300. |
MLA | Zhou, Xi,et al."Multisize particulate matter and volatile organic compounds in arid and semiarid areas of Northwest China".ENVIRONMENTAL POLLUTION 300(2022). |
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