Arid
DOI10.5194/amt-14-7657-2021
Compositional data analysis (CoDA) as a tool to evaluate a new low-cost settling-based PM10 sampling head in a desert dust source region
Xu-Yang, Yangjunjie; Losno, Remi; Monna, Fabrice; Rajot, Jean-Louis; Labiadh, Mohamed; Bergametti, Gilles; Marticorena, Beatrice
通讯作者Losno, R (corresponding author), Univ Paris, CNRS, Inst Phys Globe Paris, Paris, France.
来源期刊ATMOSPHERIC MEASUREMENT TECHNIQUES
ISSN1867-1381
EISSN1867-8548
出版年2021
卷号14期号:12页码:7657-7680
英文摘要This paper presents a new sampling head design and the method used to evaluate it. The elemental composition of aerosols collected by two different sampling devices in a semi-arid region of Tunisia is compared by means of compositional perturbation vectors and biplots. This set of underused mathematical tools belongs to a family of statistics created specifically to deal with compositional data. The two sampling devices operate at a flow rate in the range of 1 m(3) h(-1), with a cut-off diameter of 10 mu m. The first device is a low-cost laboratory-made system, where the largest particles are removed by gravitational settling in a vertical tube. This new system will be compared to the second device, a brand-new standard commercial PM10 sampling head, where size segregation is achieved by particle impaction on a metal surface. A total of 44 elements (including rare earth elements, REEs, together with Al, As, Ba, Be, Ca, Cd, Co, Cr, Cu, Fe, K, Li, Mg, Mn, Mo, Na, Ni, P, Pb, Rb, S, Sc, Se, Sr, Ti, Tl, U, V, Zn, and Zr) were analysed in 16 paired samples, collected during a 2-week field campaign in Tunisian dry lands, close to source areas, with high levels of large particles. The contrasting meteorological conditions encountered during the field campaign allowed a broad range of aerosol compositions to be collected, with very different aerosol mass concentrations. The compositional data analysis (CoDA) tools show that no compositional differences were observed between samples collected simultaneously by the two devices. The mass concentration of the particles collected was estimated through chemical analysis. Results for the two sampling devices were very similar to those obtained from an online aerosol weighing system, FLOM (tapered element oscillating microbalance), installed next to them. These results suggest that the commercial PM10 impactor head can therefore be replaced by the decanter, without any measurable bias, for the determination of chemical composition and for further assessment of PM10 concentrations in source regions.
类型Article
语种英语
开放获取类型gold, Green Submitted
收录类别SCI-E
WOS记录号WOS:000728539300001
WOS关键词AEROSOL ; NORTH ; PERTURBATION ; SIMULATION ; EFFICIENCY ; PARTICLES ; DISPLAY ; MODEL ; CYCLE
WOS类目Meteorology & Atmospheric Sciences
WOS研究方向Meteorology & Atmospheric Sciences
资源类型期刊论文
条目标识符http://119.78.100.177/qdio/handle/2XILL650/374121
作者单位[Xu-Yang, Yangjunjie; Losno, Remi] Univ Paris, CNRS, Inst Phys Globe Paris, Paris, France; [Monna, Fabrice] Univ Bourgogne Franche Comte, UMR CNRS 6298, ARTEHIS, Dijon, France; [Rajot, Jean-Louis; Bergametti, Gilles; Marticorena, Beatrice] Univ Paris, LISA Lab Interuniv Syst Atmospher, F-75013 Paris, France; [Rajot, Jean-Louis; Bergametti, Gilles; Marticorena, Beatrice] Univ Paris Est Creteil, CNRS, F-75013 Paris, France; [Rajot, Jean-Louis] Univ Paris, iEES Paris Inst Ecol & Sci Environm, UMR IRD 242, Univ Paris Est Creteil,Sorbonne Univ,CNRS,INRA, Bondy, France; [Labiadh, Mohamed] Inst Reg Arides, Medenine, Tunisia
推荐引用方式
GB/T 7714
Xu-Yang, Yangjunjie,Losno, Remi,Monna, Fabrice,et al. Compositional data analysis (CoDA) as a tool to evaluate a new low-cost settling-based PM10 sampling head in a desert dust source region[J],2021,14(12):7657-7680.
APA Xu-Yang, Yangjunjie.,Losno, Remi.,Monna, Fabrice.,Rajot, Jean-Louis.,Labiadh, Mohamed.,...&Marticorena, Beatrice.(2021).Compositional data analysis (CoDA) as a tool to evaluate a new low-cost settling-based PM10 sampling head in a desert dust source region.ATMOSPHERIC MEASUREMENT TECHNIQUES,14(12),7657-7680.
MLA Xu-Yang, Yangjunjie,et al."Compositional data analysis (CoDA) as a tool to evaluate a new low-cost settling-based PM10 sampling head in a desert dust source region".ATMOSPHERIC MEASUREMENT TECHNIQUES 14.12(2021):7657-7680.
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