干旱区生态环境知识资源中心(Arid): Assessment of Aerosol Mechanisms and Aerosol Meteorology Feedback over an Urban Airshed in India Using a Chemical Transport Model

Arid

DOI	10.3390/atmos12111417
	Assessment of Aerosol Mechanisms and Aerosol Meteorology Feedback over an Urban Airshed in India Using a Chemical Transport Model
	Gupta, Medhavi; Mohan, Manju
通讯作者	Mohan, M (corresponding author), Indian Inst Technol Delhi, Ctr Atmospher Sci, New Delhi 110016, India.
来源期刊	ATMOSPHERE
EISSN	2073-4433
出版年	2021
卷号	12 期号:11
英文摘要	The direct aerosol-radiative effects in the WRF-Chem model account for scattering/absorption of solar radiation due to aerosols, while aerosol-cloud interactions result in modifying wet scavenging of the ambient concentrations as an indirect aerosol effect. In this study, impact of aerosol on meteorological parameters, PM10 and ozone concentrations are analysed which revealed (i) that a net decrease in shortwave and longwave radiation by direct feedback results in decrease in temperature up to 0.05 K, (ii) that a net increase due to longwave and shortwave radiation when both direct and indirect effects are taken together results in an increase in temperature up to 0.25 K (where the mean of temperature is 33.5 & DEG;C and standard deviation 2.13 & DEG;C), (iii) a marginal increase in boundary layer height of 50 m with increase in temperature with feedbacks, (iv) overall net increase in radiation by direct and indirect effect together result in an increase in PM10 concentration up to 12 mu g m(-3) (with PM10 mean as 84.5 mu g m(-3) and standard deviation 28 mu g m(-3)) and an increase in ozone concentration up to 3 mu g m(-3) (with ozone mean as 29.65 mu g m(-3) and standard deviation 5.2 mu g m(-3)) mainly due to net increase in temperature. Furthermore, impact of sensitivity of different aerosol mechanisms on PM10 concentrations was scrutinized for two different mechanisms that revealed underestimation by both of the mechanisms with MOSAIC scheme, showing less fractional bias than MADE/SORGAM. For the dust storm period, MOSAIC scheme simulated higher mass concentrations than MADE/SORGAM scheme and performed well for dust-storm days while closely capturing the peaks of high dust concentrations. This study is one of the first few to demonstrate the impact of both direct and indirect aerosol feedback on local meteorology and air quality using a meteorology-chemistry modelling framework; the WRF-Chem model in a tropical urban airshed in India located in semi-arid climatic zone. It is inferred that semi-arid climatic conditions behave in a vastly different manner than other climatic zones for direct and indirect radiative feedback effects.
英文关键词	aerosol-meteorology feedback PM10 ozone the WRF-Chem aerosol mechanisms megacity Delhi
类型	Article
语种	英语
开放获取类型	gold
收录类别	SCI-E
WOS记录号	WOS:000724859300001
WOS关键词	WRF-CHEM ; AIR-QUALITY ; FORECASTING-MODEL ; OZONE SIMULATION ; WEATHER RESEARCH ; WRF/CHEM MODEL ; RADIATION ; SENSITIVITY ; CHEMISTRY ; IMPACT
WOS类目	Environmental Sciences ; Meteorology & Atmospheric Sciences
WOS研究方向	Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
资源类型	期刊论文
条目标识符	http://119.78.100.177/qdio/handle/2XILL650/373745
作者单位	[Gupta, Medhavi; Mohan, Manju] Indian Inst Technol Delhi, Ctr Atmospher Sci, New Delhi 110016, India
推荐引用方式 GB/T 7714	Gupta, Medhavi,Mohan, Manju. Assessment of Aerosol Mechanisms and Aerosol Meteorology Feedback over an Urban Airshed in India Using a Chemical Transport Model[J],2021,12(11).
APA	Gupta, Medhavi,&Mohan, Manju.(2021).Assessment of Aerosol Mechanisms and Aerosol Meteorology Feedback over an Urban Airshed in India Using a Chemical Transport Model.ATMOSPHERE,12(11).
MLA	Gupta, Medhavi,et al."Assessment of Aerosol Mechanisms and Aerosol Meteorology Feedback over an Urban Airshed in India Using a Chemical Transport Model".ATMOSPHERE 12.11(2021).