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DOI10.5194/acp-21-15847-2021
Speciated atmospheric mercury at the Waliguan Global Atmosphere Watch station in the northeastern Tibetan Plateau: implication of dust-related sources for particulate bound mercury
Zhang, Hui; Fu, Xuewu; Yu, Ben; Li, Baoxin; Liu, Peng; Zhang, Guoqing; Zhang, Leiming; Feng, Xinbin
通讯作者Fu, XW ; Feng, XB (corresponding author), Chinese Acad Sci, Inst Geochem, State Key Lab Environm Geochem, 99 Lincheng West Rd, Guiyang 550081, Peoples R China. ; Fu, XW ; Feng, XB (corresponding author), Chinese Acad Sci, CAS Ctr Excellence Quaternary Sci & Global Change, Inst Earth Environm, Xian 710061, Peoples R China. ; Feng, XB (corresponding author), Univ Chinese Acad Sci, Beijing 100049, Peoples R China.
来源期刊ATMOSPHERIC CHEMISTRY AND PHYSICS
ISSN1680-7316
EISSN1680-7324
出版年2021
卷号21期号:20页码:15847-15859
英文摘要To understand the ambient levels and sources of atmospheric mercury (Hg) in the Tibetan Plateau, a full-year continuous measurement of speciated atmospheric mercury was conducted at the Waliguan (WLG) Baseline Observatory (3816ma.s.l.) from May 2012 to April 2013. Mean concentrations (+/- 1 SD) of gaseous elemental mercury (GEM), gaseous oxidized mercury (GOM) and particulate bound mercury (PBM) during the whole study period were 1.90 +/- 0.80 ngm 3, 12.0 +/- 10.6 and 65.4 +/- 63.2 pg m(-3), respectively. Seasonal variations of GEM were very small, while those of PBM were quite large with mean values being 4 times higher in the cold (102.3 +/- 66.7 pg m(-3)) than warm (22.8 +/- 14.6 pg m(-3)) season. Anthropogenic emissions to the east of the Tibetan Plateau contributed significantly to GEM pollution at WLG, while dust particles originating from desert and Gobi regions in Xinjiang province and the Tibetan Plateau to the west of WLG were responsible for PBM pollution at WLG. This finding is also supported by the significant positive correlation between daily PBM concentration and daily cumulative absorbing aerosol index (AAI) in air masses transported during the preceding 2 d.
类型Article
语种英语
开放获取类型gold, Green Submitted
收录类别SCI-E
WOS记录号WOS:000711010900001
WOS关键词REACTIVE GASEOUS MERCURY ; MINERAL DUST ; GAW STATION ; EMISSIONS ; TRANSPORT ; CHINA ; SITE ; AIR ; DESERTS ; CLIMATE
WOS类目Environmental Sciences ; Meteorology & Atmospheric Sciences
WOS研究方向Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
来源机构中国科学院地球环境研究所
资源类型期刊论文
条目标识符http://119.78.100.177/qdio/handle/2XILL650/368097
作者单位[Zhang, Hui; Fu, Xuewu; Feng, Xinbin] Chinese Acad Sci, Inst Geochem, State Key Lab Environm Geochem, 99 Lincheng West Rd, Guiyang 550081, Peoples R China; [Fu, Xuewu; Feng, Xinbin] Chinese Acad Sci, CAS Ctr Excellence Quaternary Sci & Global Change, Inst Earth Environm, Xian 710061, Peoples R China; [Yu, Ben] Chinese Acad Sci, Res Ctr Ecoenvironm Sci, State Key Lab Environm Chem & Ecotoxicol, Beijing 100085, Peoples R China; [Li, Baoxin; Liu, Peng; Zhang, Guoqing] Qinghai Meteorol Bur, China Global Atmosphere Watch Baseline Observ, Xining 810001, Peoples R China; [Zhang, Leiming] Environm & Climate Change Canada, Sci & Technol Branch, Air Qual Res Div, Toronto, ON M3H 5T4, Canada; [Feng, Xinbin] Univ Chinese Acad Sci, Beijing 100049, Peoples R China
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GB/T 7714
Zhang, Hui,Fu, Xuewu,Yu, Ben,et al. Speciated atmospheric mercury at the Waliguan Global Atmosphere Watch station in the northeastern Tibetan Plateau: implication of dust-related sources for particulate bound mercury[J]. 中国科学院地球环境研究所,2021,21(20):15847-15859.
APA Zhang, Hui.,Fu, Xuewu.,Yu, Ben.,Li, Baoxin.,Liu, Peng.,...&Feng, Xinbin.(2021).Speciated atmospheric mercury at the Waliguan Global Atmosphere Watch station in the northeastern Tibetan Plateau: implication of dust-related sources for particulate bound mercury.ATMOSPHERIC CHEMISTRY AND PHYSICS,21(20),15847-15859.
MLA Zhang, Hui,et al."Speciated atmospheric mercury at the Waliguan Global Atmosphere Watch station in the northeastern Tibetan Plateau: implication of dust-related sources for particulate bound mercury".ATMOSPHERIC CHEMISTRY AND PHYSICS 21.20(2021):15847-15859.
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