Knowledge Resource Center for Ecological Environment in Arid Area
DOI | 10.1016/j.scitotenv.2021.150481 |
Geographical drivers of geochemical and mineralogical evolution of Motianling peatland (Northeast China) exposed to different sources of rare earth elements and Pb, Nd, and Sr isotopes | |
Fialkiewicz-Koziel, Barbara; Bao, Kunshan; Smieja-Krol, Beata | |
通讯作者 | Fialkiewicz-Koziel, B (corresponding author), Adam Mickiewicz Univ, Inst Geoinformat & Geoecol, Krygowskiego 10, Poznan, Poland. |
来源期刊 | SCIENCE OF THE TOTAL ENVIRONMENT |
ISSN | 0048-9697 |
EISSN | 1879-1026 |
出版年 | 2022 |
卷号 | 807 |
英文摘要 | Geochemical shifts triggered by surface runoff and atmospheric fallout in a Chinese peatland were investigated by using Pb, Sr, and Nd, REE and by SEM mineralogical analysis. Motianling peatland (Northeast China) is located at 1670 ma.s.l., near the China-Mongolia border. Based on division of profile into two phases of different trophy, the total Sigma REE value determined for the minerotrophic part of the profile (from 62 to 46 cm) varied from 67 to 31 mg.kg(-1) and mineralogical analysis revealed the occurrence of weathered volcanic rocks, supported by a high epsilon Nd value (-3.26). After the transition from minerotrophic to more ombrotrophic conditions, the peatland became independent of the local bedrock weathering, which was manifested by a much lower concentration of REE (7-20 mg.kg(-1)) and lower eNd values (-7.37; -8.11). Moreover, PAAS-normalized pattern of REE distribution in the bottom part revealed the highest Eu/Eu* value (1.24), as well as a slight enrichment in Eu. The anthropogenic effect was visible from 1964, during which period the spheroidal aluminosilicate particles (SAP), produced by coal-fired power-plant activity, appeared for the first time, followed by an abrupt decrease in Pb-206/Pb-207 isotopic signature to 1.167. The dimensions of SAP (similar to 1.5 mu m), as well as the time of first appearance, indicated long-range transport. The REE ratios obtained in this study are characteristic of the eolian deposition signature, which is like the Gobi and northern Chinese deserts. The anthropogenic activity was manifested by a slight enrichment in Gd during reduced delivery of natural dust. Both, North Chinese and Asian part of the Russian industry supply anthropogenic dust. Topography, wind direction, and patterns of precipitation, as well as the initial phases of Asian industrial development, are the most important drivers promoting the deposition of chemical elements. (C) 2021 The Authors. Published by Elsevier B.V. |
英文关键词 | Peat bog Stable isotopes Rare earth elements Anthropocene Source provenance |
类型 | Article |
语种 | 英语 |
开放获取类型 | hybrid |
收录类别 | SCI-E |
WOS记录号 | WOS:000707662000004 |
WOS关键词 | ATMOSPHERIC METAL-DEPOSITION ; GREAT HINGGAN MOUNTAIN ; LONG-RANGE TRANSPORT ; ASIAN DUST STORM ; C-14 YR BP ; JURA MOUNTAINS ; INORGANIC GEOCHEMISTRY ; ANTHROPOGENIC LEAD ; TRACE-ELEMENTS ; AIR-POLLUTANTS |
WOS类目 | Environmental Sciences |
WOS研究方向 | Environmental Sciences & Ecology |
资源类型 | 期刊论文 |
条目标识符 | http://119.78.100.177/qdio/handle/2XILL650/364637 |
作者单位 | [Fialkiewicz-Koziel, Barbara] Adam Mickiewicz Univ, Inst Geoinformat & Geoecol, Krygowskiego 10, Poznan, Poland; [Bao, Kunshan] South China Normal Univ, Sch Geog, Guangzhou 510631, Peoples R China; [Smieja-Krol, Beata] Univ Silesia, Inst Earth Sci, Fac Nat Sci, Bedzinska 60, PL-41200 Sosnowiec, Poland |
推荐引用方式 GB/T 7714 | Fialkiewicz-Koziel, Barbara,Bao, Kunshan,Smieja-Krol, Beata. Geographical drivers of geochemical and mineralogical evolution of Motianling peatland (Northeast China) exposed to different sources of rare earth elements and Pb, Nd, and Sr isotopes[J],2022,807. |
APA | Fialkiewicz-Koziel, Barbara,Bao, Kunshan,&Smieja-Krol, Beata.(2022).Geographical drivers of geochemical and mineralogical evolution of Motianling peatland (Northeast China) exposed to different sources of rare earth elements and Pb, Nd, and Sr isotopes.SCIENCE OF THE TOTAL ENVIRONMENT,807. |
MLA | Fialkiewicz-Koziel, Barbara,et al."Geographical drivers of geochemical and mineralogical evolution of Motianling peatland (Northeast China) exposed to different sources of rare earth elements and Pb, Nd, and Sr isotopes".SCIENCE OF THE TOTAL ENVIRONMENT 807(2022). |
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