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DOI10.1016/j.nanoen.2020.105311
Metal-based nanomaterials for efficient CO2 electroreduction: Recent advances in mechanism, material design and selectivity
Hoang, Van Chinh; Gomes, Vincent G.; Kornienko, Nikolay
通讯作者Gomes, VG
来源期刊NANO ENERGY
ISSN2211-2855
EISSN2211-3282
出版年2020
卷号78
英文摘要Increasing global demands for energy supply have accelerated fossil fuel consumption, triggering a gradual increase in atmospheric CO2, leading to adverse environmental effects of global warming, desertification and ocean acidification. Thus, reducing carbon emissions to mitigate climate change is an urgent imperative. Among several feasible strategies, electrochemical reduction of CO2 into value-added feedstocks is a promising one since such processes can be integrated with renewable electricity and powered by intermittent energy sources: wind, solar and hydro among others. The efficiency of CO2 reduction reaction (CO2RR) and its resulting economic feasibility strongly depends on the intrinsic properties of catalyst used. Several approaches have been proposed to attain high electrocatalytic performance of heterogenous electrocatalysts by controlling their size, morphology, surface defects, grain boundaries and crystal facets and by coupling with other synergistic components to synthesize nanocomposites, e.g., metallic alloys or metal/carbon-based nanomaterials. This review presents the latest achievements with metal-based nanomaterials for efficient electrochemical CO2 reduction reaction, their mechanism of action, and promising applications in selective conversions valuable chemicals/fuels, including carbon monoxide, formic acid, hydrocarbons and alcohols.
英文关键词Electrochemical catalysis CO2 reduction Catalytic selectivity Metallic nanomaterials Metallic composites Electrocatalysts
类型Article
语种英语
收录类别SCI-E
WOS记录号WOS:000595293200003
WOS类目Chemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary ; Physics, Applied
WOS研究方向Chemistry ; Science & Technology - Other Topics ; Materials Science ; Physics
资源类型期刊论文
条目标识符http://119.78.100.177/qdio/handle/2XILL650/327822
作者单位[Hoang, Van Chinh; Gomes, Vincent G.] Univ Sydney, Sch Chem & Biomol Engn, Sydney, NSW 2006, Australia; [Kornienko, Nikolay] Univ Montreal, Dept Chem, Roger Gaudry Bldg, Montreal, PQ H3C 3J7, Canada
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Hoang, Van Chinh,Gomes, Vincent G.,Kornienko, Nikolay. Metal-based nanomaterials for efficient CO2 electroreduction: Recent advances in mechanism, material design and selectivity[J],2020,78.
APA Hoang, Van Chinh,Gomes, Vincent G.,&Kornienko, Nikolay.(2020).Metal-based nanomaterials for efficient CO2 electroreduction: Recent advances in mechanism, material design and selectivity.NANO ENERGY,78.
MLA Hoang, Van Chinh,et al."Metal-based nanomaterials for efficient CO2 electroreduction: Recent advances in mechanism, material design and selectivity".NANO ENERGY 78(2020).
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