干旱区生态环境知识资源中心(Arid): High Resolution Chemistry Transport Modeling with the On-Line CHIMERE-WRF Model over the French Alps-Analysis of a Feedback of Surface Particulate Matter Concentrations on Mountain Meteorology

Arid

DOI	10.3390/atmos11060565
	High Resolution Chemistry Transport Modeling with the On-Line CHIMERE-WRF Model over the French Alps-Analysis of a Feedback of Surface Particulate Matter Concentrations on Mountain Meteorology
	Bessagnet, Bertrand 1,6; Menut, Laurent 1; Lapere, Remy 1; Couvidat, Florian 2; Jaffrezo, Jean-Luc 3; Mailler, Sylvain 1; Favez, Olivier 2; Pennel, Romain 1; Siour, Guillaume 4,5
通讯作者	Bessagnet, Bertrand
来源期刊	ATMOSPHERE
EISSN	2073-4433
出版年	2020
卷号	11 期号:6
英文摘要	Air pollution is of major concern throughout the world and the use of modeling tools to analyze and forecast the pollutant concentrations in complex orographic areas remains challenging. This work proposes an exhaustive framework to analyze the ability of models to simulate the air quality over the French Alps up to 1.2 km resolution over Grenoble and the Arve Valley. The on-line coupled suite of models CHIMERE-WRF is used in its recent version to analyze a 1 month episode in November-December 2013. As expected, an improved resolution increases the concentrations close to the emission areas and reduced the negative bias for Particulate Matter that is the usual weakness of air quality models. However, the nitrate concentrations seem overestimated with at the same time an overestimation of surface temperature in the morning by WRF. Different WRF settings found in the literature are tested to improve the results, particularly the ability of the meteorological model to simulate the strong thermal inversions in the morning. Wood burning is one of the main contributor of air pollution during the period ranging from 80 to 90% of the Organic Matter. The activation of the on-line coupling has a moderate impact on the background concentrations but surprisingly a change of Particulate Matter (PM) concentrations in the valley will affect more the meteorology nearby high altitude areas than in the valley. This phenomenon is the result of a chain of processes involving the radiative effects and the water vapor column gradients in complex orographic areas. At last, the model confirms that the surrounding glaciers are largely impacted by long range transport of desert dust. However, in wintertime some outbreaks of anthropogenic pollution from the valley when the synoptic situation changes can be advected up to the nearby high altitude areas, then deposited.
英文关键词	Alps CHIMERE WRF on-line coupling air pollution organic matter dispersion deposition radiative effects
类型	Article
语种	英语
国家	France
开放获取类型	gold, Green Submitted
收录类别	SCI-E
WOS记录号	WOS:000551736200001
WOS关键词	RADIATION-CLOUD INTERACTIONS ; AIR-POLLUTION ; ORGANIC AEROSOL ; BOUNDARY-LAYER ; BLACK CARBON ; LIFE-CYCLE ; PARAMETERIZATION ; MICROPHYSICS ; SIMULATIONS ; SENSITIVITY
WOS类目	Environmental Sciences ; Meteorology & Atmospheric Sciences
WOS研究方向	Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
来源机构	French National Research Institute for Sustainable Development
资源类型	期刊论文
条目标识符	http://119.78.100.177/qdio/handle/2XILL650/319429
作者单位	1.PSL Univ, Sorbonne Univ, Inst Polytech Paris, CNRS,LMD IPSL,Ecole Polytech,ENS, F-91128 Palaiseau, France; 2.Inst Natl Environm Ind & Risques, Parc Technol ALATA, F-60550 Verneuil En Halatte, France; 3.Univ Grenoble Alpes, IGE, CNRS, IRD, F-38000 Grenoble, France; 4.Univ Paris Est Creteil, Lab Interuniv Syst Atmospher, UMR CNRS 7583, F-94000 Creteil, France; 5.Univ Paris, Inst Pierre Simon Laplace, F-94000 Creteil, France; 6.Citepa Tech Reference Ctr Air Pollut & Climat, 42 Rue Paradis, F-75010 Paris, France
推荐引用方式 GB/T 7714	Bessagnet, Bertrand,Menut, Laurent,Lapere, Remy,et al. High Resolution Chemistry Transport Modeling with the On-Line CHIMERE-WRF Model over the French Alps-Analysis of a Feedback of Surface Particulate Matter Concentrations on Mountain Meteorology[J]. French National Research Institute for Sustainable Development,2020,11(6).
APA	Bessagnet, Bertrand.,Menut, Laurent.,Lapere, Remy.,Couvidat, Florian.,Jaffrezo, Jean-Luc.,...&Siour, Guillaume.(2020).High Resolution Chemistry Transport Modeling with the On-Line CHIMERE-WRF Model over the French Alps-Analysis of a Feedback of Surface Particulate Matter Concentrations on Mountain Meteorology.ATMOSPHERE,11(6).
MLA	Bessagnet, Bertrand,et al."High Resolution Chemistry Transport Modeling with the On-Line CHIMERE-WRF Model over the French Alps-Analysis of a Feedback of Surface Particulate Matter Concentrations on Mountain Meteorology".ATMOSPHERE 11.6(2020).