Arid
DOI10.3390/atmos11040390
Atmospheric Trace Metal Deposition near the Great Barrier Reef, Australia
Strzelec, Michal1; Proemse, Bernadette C.1,2; Gault-Ringold, Melanie3; Boyd, Philip W.1,3; Perron, Morgane M. G.1; Schofield, Robyn4,5; Ryan, Robert G.4,5; Ristovski, Zoran D.6; Alroe, Joel6; Humphries, Ruhi S.7; Keywood, Melita D.7; Ward, Jason7; Bowie, Andrew R.1,3
通讯作者Strzelec, Michal
来源期刊ATMOSPHERE
EISSN2073-4433
出版年2020
卷号11期号:4
英文摘要Aerosols deposited into the Great Barrier Reef (GBR) contain iron (Fe) and other trace metals, which may act as micronutrients or as toxins to this sensitive marine ecosystem. In this paper, we quantified the atmospheric deposition of Fe and investigated aerosol sources in Mission Beach (Queensland) next to the GBR. Leaching experiments were applied to distinguish pools of Fe with regard to its solubility. The labile Fe concentration in aerosols was 2.3-10.6 ng m(-3), which is equivalent to 4.9-11.4% of total Fe and was linked to combustion and biomass burning processes, while total Fe was dominated by crustal sources. A one-day precipitation event provided more soluble iron than the average dry deposition flux, 0.165 and 0.143 mu mol m(-2) day(-1), respectively. Scanning Electron Microscopy indicated that alumina-silicates were the main carriers of total Fe and samples affected by combustion emissions were accompanied by regular round-shaped carbonaceous particulates. Collected aerosols contained significant amounts of Cd, Co, Cu, Mo, Mn, Pb, V, and Zn, which were mostly (47.5-96.7%) in the labile form. In this study, we provide the first field data on the atmospheric delivery of Fe and other trace metals to the GBR and propose that this is an important delivery mechanism to this region.
英文关键词aerosols Fe solubility leaching experiments global Fe cycle source apportionment anthropogenic emissions
类型Article
语种英语
国家Australia
开放获取类型Green Published, gold, Green Accepted
收录类别SCI-E
WOS记录号WOS:000539492200077
WOS关键词FRACTIONAL IRON SOLUBILITY ; AEOLIAN DUST DEPOSITION ; NITROGEN-FIXATION ; MINERAL DUST ; PHYTOPLANKTON DYNAMICS ; ELEMENT CONCENTRATIONS ; BIOGEOCHEMICAL CYCLES ; FERTILIZATION SUCCESS ; DESERT DUST ; AEROSOLS
WOS类目Environmental Sciences ; Meteorology & Atmospheric Sciences
WOS研究方向Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
来源机构Commonwealth Scientific and Industrial Research Organisation
资源类型期刊论文
条目标识符http://119.78.100.177/qdio/handle/2XILL650/319422
作者单位1.Univ Tasmania, Inst Marine & Antarctic Studies, Hobart, Tas 7005, Australia;
2.Univ Tasmania, Australian Ctr Res Separat Sci, Hobart, Tas 7005, Australia;
3.Univ Tasmania, Antarctic Climate & Ecosyst CRC, Hobart, Tas 7005, Australia;
4.Univ Melbourne, Sch Earth Sci, Melbourne, Vic 3010, Australia;
5.Univ New South Wales, ARC Ctr Excellence Climate Syst Sci, Sydney, NSW 2052, Australia;
6.Queensland Univ Technol QUT, Int Lab Air Qual & Hlth, Brisbane, Qld 4000, Australia;
7.CSIRO, Climate Sci Ctr, Oceans & Atmosphere, 107-121 Stn St, Aspendale, Vic 3195, Australia
推荐引用方式
GB/T 7714
Strzelec, Michal,Proemse, Bernadette C.,Gault-Ringold, Melanie,et al. Atmospheric Trace Metal Deposition near the Great Barrier Reef, Australia[J]. Commonwealth Scientific and Industrial Research Organisation,2020,11(4).
APA Strzelec, Michal.,Proemse, Bernadette C..,Gault-Ringold, Melanie.,Boyd, Philip W..,Perron, Morgane M. G..,...&Bowie, Andrew R..(2020).Atmospheric Trace Metal Deposition near the Great Barrier Reef, Australia.ATMOSPHERE,11(4).
MLA Strzelec, Michal,et al."Atmospheric Trace Metal Deposition near the Great Barrier Reef, Australia".ATMOSPHERE 11.4(2020).
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