Knowledge Resource Center for Ecological Environment in Arid Area
DOI | 10.3390/atmos11040390 |
Atmospheric Trace Metal Deposition near the Great Barrier Reef, Australia | |
Strzelec, Michal1; Proemse, Bernadette C.1,2; Gault-Ringold, Melanie3; Boyd, Philip W.1,3; Perron, Morgane M. G.1; Schofield, Robyn4,5; Ryan, Robert G.4,5; Ristovski, Zoran D.6; Alroe, Joel6; Humphries, Ruhi S.7; Keywood, Melita D.7; Ward, Jason7; Bowie, Andrew R.1,3 | |
通讯作者 | Strzelec, Michal |
来源期刊 | ATMOSPHERE
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EISSN | 2073-4433 |
出版年 | 2020 |
卷号 | 11期号:4 |
英文摘要 | Aerosols deposited into the Great Barrier Reef (GBR) contain iron (Fe) and other trace metals, which may act as micronutrients or as toxins to this sensitive marine ecosystem. In this paper, we quantified the atmospheric deposition of Fe and investigated aerosol sources in Mission Beach (Queensland) next to the GBR. Leaching experiments were applied to distinguish pools of Fe with regard to its solubility. The labile Fe concentration in aerosols was 2.3-10.6 ng m(-3), which is equivalent to 4.9-11.4% of total Fe and was linked to combustion and biomass burning processes, while total Fe was dominated by crustal sources. A one-day precipitation event provided more soluble iron than the average dry deposition flux, 0.165 and 0.143 mu mol m(-2) day(-1), respectively. Scanning Electron Microscopy indicated that alumina-silicates were the main carriers of total Fe and samples affected by combustion emissions were accompanied by regular round-shaped carbonaceous particulates. Collected aerosols contained significant amounts of Cd, Co, Cu, Mo, Mn, Pb, V, and Zn, which were mostly (47.5-96.7%) in the labile form. In this study, we provide the first field data on the atmospheric delivery of Fe and other trace metals to the GBR and propose that this is an important delivery mechanism to this region. |
英文关键词 | aerosols Fe solubility leaching experiments global Fe cycle source apportionment anthropogenic emissions |
类型 | Article |
语种 | 英语 |
国家 | Australia |
开放获取类型 | Green Published, gold, Green Accepted |
收录类别 | SCI-E |
WOS记录号 | WOS:000539492200077 |
WOS关键词 | FRACTIONAL IRON SOLUBILITY ; AEOLIAN DUST DEPOSITION ; NITROGEN-FIXATION ; MINERAL DUST ; PHYTOPLANKTON DYNAMICS ; ELEMENT CONCENTRATIONS ; BIOGEOCHEMICAL CYCLES ; FERTILIZATION SUCCESS ; DESERT DUST ; AEROSOLS |
WOS类目 | Environmental Sciences ; Meteorology & Atmospheric Sciences |
WOS研究方向 | Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences |
来源机构 | Commonwealth Scientific and Industrial Research Organisation |
资源类型 | 期刊论文 |
条目标识符 | http://119.78.100.177/qdio/handle/2XILL650/319422 |
作者单位 | 1.Univ Tasmania, Inst Marine & Antarctic Studies, Hobart, Tas 7005, Australia; 2.Univ Tasmania, Australian Ctr Res Separat Sci, Hobart, Tas 7005, Australia; 3.Univ Tasmania, Antarctic Climate & Ecosyst CRC, Hobart, Tas 7005, Australia; 4.Univ Melbourne, Sch Earth Sci, Melbourne, Vic 3010, Australia; 5.Univ New South Wales, ARC Ctr Excellence Climate Syst Sci, Sydney, NSW 2052, Australia; 6.Queensland Univ Technol QUT, Int Lab Air Qual & Hlth, Brisbane, Qld 4000, Australia; 7.CSIRO, Climate Sci Ctr, Oceans & Atmosphere, 107-121 Stn St, Aspendale, Vic 3195, Australia |
推荐引用方式 GB/T 7714 | Strzelec, Michal,Proemse, Bernadette C.,Gault-Ringold, Melanie,et al. Atmospheric Trace Metal Deposition near the Great Barrier Reef, Australia[J]. Commonwealth Scientific and Industrial Research Organisation,2020,11(4). |
APA | Strzelec, Michal.,Proemse, Bernadette C..,Gault-Ringold, Melanie.,Boyd, Philip W..,Perron, Morgane M. G..,...&Bowie, Andrew R..(2020).Atmospheric Trace Metal Deposition near the Great Barrier Reef, Australia.ATMOSPHERE,11(4). |
MLA | Strzelec, Michal,et al."Atmospheric Trace Metal Deposition near the Great Barrier Reef, Australia".ATMOSPHERE 11.4(2020). |
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