Knowledge Resource Center for Ecological Environment in Arid Area
DOI | 10.1016/j.envpol.2020.113918 |
A quantitative assessment of atmospheric emissions and spatial distribution of trace elements from natural sources in China | |
Wu, Yiming1,2; Lin, Shumin1,2; Tian, Hezhong1,2; Zhang, Kai3,4; Wang, Yifei1; Sun, Bowen1; Liu, Xiangyang1,2; Liu, Kaiyun5; Xue, Yifeng1,2,6; Hao, Jiming5; Liu, Huanjia1,2; Liu, Shuhan1,2; Shao, Panyang1,2,7; Luo, Lining1,2; Bai, Xiaoxuan1,2; Liu, Wei1,2; Wu, Bobo1,2; Zhao, Shuang1,2 | |
通讯作者 | Tian, Hezhong |
来源期刊 | ENVIRONMENTAL POLLUTION
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ISSN | 0269-7491 |
EISSN | 1873-6424 |
出版年 | 2020 |
卷号 | 259 |
英文摘要 | Natural sources, such as soil and wind erosion dust (SWD), biomass open burning (BOB), sea salt spray (SSAS) and biogenic source (BIO), are major contributors to atmospheric emissions of trace elements (TEs) globally. In this study, we used a comprehensive approach to account for area-, production- and biofuel consumption-based emission factor calculation methods, and thus developed an integrated high-resolution emission inventory for 15 types of TEs (As, B, Cd, Co, Cr, Cu, Hg, Mn, Mo, Ni, Pb, Sb, Se, V and Zn) originated from natural sources in China for the year 2015. The results show that national emissions of TEs in 2015 range from 7.45 tons (Hg) to 1, 400 tons (Zn) except for the extremely high emissions of Mn (10, 677 tons). SWD and BIO are identified as the top two source contributors, accounting for approximately 67.7% and 26.1% of the total emissions, respectively. Absolute emissions of TEs from natural sources are high in the Xinjiang, Inner Mongolia and Tibet autonomous regions with large areas of bare soil and desert. However, emission intensity of TEs per unit area in the Southern provinces of China is higher than those in Northern China and Southwestern China, with the Yunnan and Sichuan provinces displaying the highest emission intensity. Our results suggest that controlling SWD can play a significant role in reducing fugitive particulate matter and the associated emissions of TEs from natural sources in China; and desertification control is particularly critical in the Northwest provinces where the majority of deserts are located. (C) 2020 Elsevier Ltd. All rights reserved. |
英文关键词 | Trace element Natural source Emission inventory Soil and wind-erosion dust Biogenic source Spatial distribution |
类型 | Article |
语种 | 英语 |
国家 | Peoples R China ; USA |
收录类别 | SCI-E |
WOS记录号 | WOS:000528534600004 |
WOS关键词 | ANTHROPOGENIC MERCURY EMISSIONS ; MUNICIPAL SOLID-WASTE ; TOXIC HEAVY-METALS ; TEMPORAL TRENDS ; SPATIOTEMPORAL VARIATION ; CHEMICAL-COMPOSITION ; ISOPRENE EMISSION ; AIR-POLLUTANTS ; WIND EROSION ; SEA-SALT |
WOS类目 | Environmental Sciences |
WOS研究方向 | Environmental Sciences & Ecology |
来源机构 | 北京师范大学 ; 清华大学 |
资源类型 | 期刊论文 |
条目标识符 | http://119.78.100.177/qdio/handle/2XILL650/318963 |
作者单位 | 1.Beijing Normal Univ, Sch Environm, State Key Joint Lab Environm Simulat & Pollut Con, Beijing 100875, Peoples R China; 2.Beijing Normal Univ, Ctr Atmospher Environm Studies, Beijing 100875, Peoples R China; 3.Univ Texas Hlth Sci Ctr Houston, Dept Epidemiol Human Genet & Environm Sci, Sch Publ Hlth, Houston, TX 77030 USA; 4.Univ Texas Hlth Sci Ctr Houston, Southwest Ctr Occupat & Environm Hlth, Sch Publ Hlth, Houston, TX 77030 USA; 5.Tsinghua Univ, Sch Environm, State Environm Protect Key Lab Sources & Control, Beijing 10084, Peoples R China; 6.Beijing Municipal Res Inst Environm Protect, Natl Engn Res Ctr Urban Environm Pollut Control, Beijing 100037, Peoples R China; 7.CRAES, Beijing 100012, Peoples R China |
推荐引用方式 GB/T 7714 | Wu, Yiming,Lin, Shumin,Tian, Hezhong,et al. A quantitative assessment of atmospheric emissions and spatial distribution of trace elements from natural sources in China[J]. 北京师范大学, 清华大学,2020,259. |
APA | Wu, Yiming.,Lin, Shumin.,Tian, Hezhong.,Zhang, Kai.,Wang, Yifei.,...&Zhao, Shuang.(2020).A quantitative assessment of atmospheric emissions and spatial distribution of trace elements from natural sources in China.ENVIRONMENTAL POLLUTION,259. |
MLA | Wu, Yiming,et al."A quantitative assessment of atmospheric emissions and spatial distribution of trace elements from natural sources in China".ENVIRONMENTAL POLLUTION 259(2020). |
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