Arid
DOI10.1007/s11356-020-08070-2
Metals and PFAS in stormwater and surface runoff in a semi-arid Canadian city subject to large variations in temperature among seasons
Codling, Garry1,2; Yuan, Hongda1; Jones, Paul D.1; Giesy, John P.1,3,4,5,6; Hecker, Markus1
通讯作者Codling, Garry
来源期刊ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH
ISSN0944-1344
EISSN1614-7499
出版年2020
卷号27期号:15页码:18232-18241
英文摘要Because compounds accumulate through dry periods and enter aquatic systems in just a few seasonal events such as snowmelt and summer storms, surface waters in semi-arid, cold regions, such as the Canadian Prairies, are particularly vulnerable to loading of contaminant from runoff events from surfaces. This study assessed concentrations of metals and selected trace organics entering a river via surface runoff from an urban region and how these semi-arid regions with large seasonal variations in temperature might differ from more temperate regions. Selected potentially harmful elements (PHEs) including, Mn with Cr, Cu, Zn, Ba and U all exceeded guideline discharge values set by the Canadian Council of the Ministers of the Environment (CCME) by as much as 16-fold. Variation among discharges during spring, summer and winter was observed. For example, across the whole city, an estimated 6 kg of zinc was discharged in a spring storm, 36 kg in a summer storm and 17 tonnes in snowmelt. The mass of Zn discharged is similar to the annual loading estimated for Stockholm, Sweden, but in Saskatoon, Saskatchewan, Canada, the bulk of runoff was during snowmelt. The mean sum of poly- and per-fluoroalkyl substances (PFAS) in stormwater was 9.0 ng L-1, which is consistent with concentrations observed in other Canadian cities (6.5-16 ng L-1). These concentrations of PFAS are likely due to dispersed sources and orders of magnitude less than thresholds for toxicity to fish and aquatic invertebrates.
英文关键词Inorganic Organic Contaminants Stormwater Snowmelt Seasonality PFAS North America Prairies
类型Article
语种英语
国家Canada ; Czech Republic ; USA
收录类别SCI-E
WOS记录号WOS:000519860800002
WOS关键词EARLY-LIFE STAGES ; WHITE STURGEON ; ACUTE TOXICITY ; HEAVY-METALS ; HEALTH-RISK ; COPPER IONS ; WATER ; ADSORPTION ; ZINC ; POLLUTION
WOS类目Environmental Sciences
WOS研究方向Environmental Sciences & Ecology
资源类型期刊论文
条目标识符http://119.78.100.177/qdio/handle/2XILL650/314468
作者单位1.Univ Saskatchewan, Toxicol Ctr, Saskatoon, SK S7N 5B3, Canada;
2.Masaryk Univ, Res Ctr Contaminants Environm, Pavil 29, Brno, Czech Republic;
3.Univ Saskatchewan, Dept Vet Biomed Sci, 44 Campus Dr, Saskatoon, SK S7N 5B3, Canada;
4.Michigan State Univ, Dept Zool, E Lansing, MI 48824 USA;
5.Michigan State Univ, Ctr Integrat Toxicol, E Lansing, MI 48824 USA;
6.Baylor Univ, Dept Environm Sci, Waco, TX 76798 USA
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Codling, Garry,Yuan, Hongda,Jones, Paul D.,et al. Metals and PFAS in stormwater and surface runoff in a semi-arid Canadian city subject to large variations in temperature among seasons[J],2020,27(15):18232-18241.
APA Codling, Garry,Yuan, Hongda,Jones, Paul D.,Giesy, John P.,&Hecker, Markus.(2020).Metals and PFAS in stormwater and surface runoff in a semi-arid Canadian city subject to large variations in temperature among seasons.ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH,27(15),18232-18241.
MLA Codling, Garry,et al."Metals and PFAS in stormwater and surface runoff in a semi-arid Canadian city subject to large variations in temperature among seasons".ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH 27.15(2020):18232-18241.
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