干旱区生态环境知识资源中心(Arid): An assessment of natural and anthropogenic trace elements in the atmospheric deposition during 1776-2004 AD using the Miaoergou ice core, eastern Tien Shan, China

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DOI	10.1016/j.atmosenv.2019.117112
	An assessment of natural and anthropogenic trace elements in the atmospheric deposition during 1776-2004 AD using the Miaoergou ice core, eastern Tien Shan, China
	Zou, Xiang 1; Hou, Shugui 1,2; Wu, Shuangye 1,3; Zhang, Wangbin 1; Liu, Ke 1; Yu, Jinhai 1; Liu, Yaping 4; Pang, Hongxi 1
通讯作者	Hou, Shugui
来源期刊	ATMOSPHERIC ENVIRONMENT
ISSN	1352-2310
EISSN	1873-2844
出版年	2020
卷号	221
英文摘要	An annually resolved trace element (TE) record is established for V, Mn, Co, Ni, Cu, As, Rb, Sr, Mo, Sn, Sb, Ba, Tl, Bi, Th, U, Cr, and Pb from the Miaoergou ice core, eastern Tien Shan, China, covering the period 1776-2004 A.D.. Using this record, we examined the continuous changes of atmospheric TE compositions and identified their natural and anthropogenic sources based on the analysis of their enrichment factors (EF) and excess (Ex) concentrations. First, the record shows high concentrations of crustal elements during the periods of 1787-1813 A. D., 1825-1887 A.D., 1941-1978 A.D., likely originated from the surrounding deserts, especially the Taklimakan Desert. Second, similar to other natural archive records from the Northern Hemisphere, the data show sporadic Ex concentrations of Pb, Sn, Cu, Tl before the 1950s, likely related to the coal combustion and non-ferrous production/smelting in the European countries since the Industrial Revolution. Finally, the record reveals significant anthropogenic contribution to concentrations of Pb, Sn, Cu, Sb, As, Bi, and Tl in the second half of the 20th century. The Ex concentration of these elements started to increase sharply in the 19505, reached the maximum levels in the 1970s-1980s, subsequently declined in the early 1990s, and finally rose again in the late 1990s. The temporal TE trends could reflect the industrial and agricultural development in the possible source regions (e.g., the former Soviet Union). Therefore, our high-resolution record of atmospheric TEs provides a valuable historical perspective on air pollution emissions in these regions surrounding Miaoergou since the Industrial Revolution.
英文关键词	Trace elements Ice core Air pollution Eastern Tien Shan
类型	Article
语种	英语
国家	Peoples R China ; USA
开放获取类型	Bronze
收录类别	SCI-E
WOS记录号	WOS:000503097100003
WOS关键词	MT. QOMOLANGMA EVEREST ; CENTRAL-ASIA ; TIBETAN PLATEAU ; HG POLLUTION ; HEAVY-METALS ; RECORD ; SNOW ; DUST ; LEAD ; EMISSIONS
WOS类目	Environmental Sciences ; Meteorology & Atmospheric Sciences
WOS研究方向	Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
EI主题词	2020-01-15
来源机构	南京大学
资源类型	期刊论文
条目标识符	http://119.78.100.177/qdio/handle/2XILL650/312490
作者单位	1.Nanjing Univ, Sch Geog & Oceanog Sci, Nanjing, Jiangsu, Peoples R China; 2.CAS Ctr Excellence Tibetan Plateau Earth Sci, Beijing, Peoples R China; 3.Univ Dayton, Dept Geol, Dayton, OH 45469 USA; 4.Chinese Acad Sci, Northwest Inst Ecoenvironm & Resources, State Key Lab Cryospher Sci, Lanzhou, Gansu, Peoples R China
推荐引用方式 GB/T 7714	Zou, Xiang,Hou, Shugui,Wu, Shuangye,et al. An assessment of natural and anthropogenic trace elements in the atmospheric deposition during 1776-2004 AD using the Miaoergou ice core, eastern Tien Shan, China[J]. 南京大学,2020,221.
APA	Zou, Xiang.,Hou, Shugui.,Wu, Shuangye.,Zhang, Wangbin.,Liu, Ke.,...&Pang, Hongxi.(2020).An assessment of natural and anthropogenic trace elements in the atmospheric deposition during 1776-2004 AD using the Miaoergou ice core, eastern Tien Shan, China.ATMOSPHERIC ENVIRONMENT,221.
MLA	Zou, Xiang,et al."An assessment of natural and anthropogenic trace elements in the atmospheric deposition during 1776-2004 AD using the Miaoergou ice core, eastern Tien Shan, China".ATMOSPHERIC ENVIRONMENT 221(2020).