干旱区生态环境知识资源中心(Arid): Profiles of cloud condensation nuclei, dust mass concentration, and ice-nucleating-particle-relevant aerosol properties in the Saharan Air Layer over Barbados from polarization lidar and airborne in situ measurements

Arid

DOI	10.5194/acp-19-13773-2019
	Profiles of cloud condensation nuclei, dust mass concentration, and ice-nucleating-particle-relevant aerosol properties in the Saharan Air Layer over Barbados from polarization lidar and airborne in situ measurements
	Haarig, Moritz 1; Walser, Adrian 2; Ansmann, Albert 1; Dollner, Maximilian 2; Althausen, Dietrich 1; Sauer, Daniel 3; Farrell, David 4; Weinzierl, Bernadett 2
通讯作者	Haarig, Moritz
来源期刊	ATMOSPHERIC CHEMISTRY AND PHYSICS
ISSN	1680-7316
EISSN	1680-7324
出版年	2019
卷号	19 期号:22 页码:13773-13788
英文摘要	The present study aims to evaluate lidar retrievals of cloud-relevant aerosol properties by using polarization lidar and coincident airborne in situ measurements in the Saharan Air Layer (SAL) over the Barbados region. Vertical profiles of the number concentration of cloud condensation nuclei (CCN), large particles (diameter d > 500 nm), surface area, mass, and ice-nucleating particle (INP) concentration are derived from the lidar measurements and compared with CCN concentrations and the INP-relevant aerosol properties measured in situ with aircraft. The measurements were performed in the framework of the Saharan Aerosol Long-range Transport and Aerosol-Cloud-Interaction Experiment (SALTRACE) in summer 2013. The CCN number concentrations derived from lidar observations were up to a factor of 2 higher than the ones measured in situ aboard the research aircraft Falcon. Possible reasons for the difference are discussed. The number concentration of particles with a dry radius of more than 250 nm and the surface-area concentration obtained from the lidar observations and used as input for the INP parameterizations agreed well (< 30 %-50% deviation) with the aircraft measurements. In a pronounced lofted dust layer during summer (10 July 2013), the lidar retrieval yielded 100-300 CCN per cubic centimeter at 0.2% water supersaturation and 10-200 INPs per liter at 25 degrees C. Excellent agreement was also obtained in the comparison of mass concentration profiles. During the SALTRACE winter campaign (March 2014), the dust layer from Africa was mixed with smoke particles which dominated the CCN number concentration. This example highlights the unique lidar potential to separate smoke and dust contributions to the CCN reservoir and thus to identify the sensitive role of smoke in trade wind cumuli developments over the tropical Atlantic during the winter season.
类型	Article
语种	英语
国家	Germany ; Austria ; Barbados
开放获取类型	gold, Green Accepted
收录类别	SCI-E
WOS记录号	WOS:000497781300001
WOS关键词	DROPLET ACTIVATION KINETICS ; DEPOLARIZATION-RATIO ; OPTICAL-PROPERTIES ; RAMAN LIDAR ; DESERT-DUST ; COARSE DUST ; CCN ; EXTINCTION ; SPECTROMETER ; INSTRUMENT
WOS类目	Environmental Sciences ; Meteorology & Atmospheric Sciences
WOS研究方向	Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
EI主题词	2019-11-18
资源类型	期刊论文
条目标识符	http://119.78.100.177/qdio/handle/2XILL650/310917
作者单位	1.Leibniz Inst Tropospher Res, Leipzig, Germany; 2.Univ Vienna, Fac Phys, Vienna, Austria; 3.Deutsch Zentrum Luft & Raumfahrt, Inst Phys Atmosphare, Oberpfaffenhofen, Germany; 4.Caribbean Inst Meteorol & Hydrol, Bridgetown, Barbados
推荐引用方式 GB/T 7714	Haarig, Moritz,Walser, Adrian,Ansmann, Albert,et al. Profiles of cloud condensation nuclei, dust mass concentration, and ice-nucleating-particle-relevant aerosol properties in the Saharan Air Layer over Barbados from polarization lidar and airborne in situ measurements[J],2019,19(22):13773-13788.
APA	Haarig, Moritz.,Walser, Adrian.,Ansmann, Albert.,Dollner, Maximilian.,Althausen, Dietrich.,...&Weinzierl, Bernadett.(2019).Profiles of cloud condensation nuclei, dust mass concentration, and ice-nucleating-particle-relevant aerosol properties in the Saharan Air Layer over Barbados from polarization lidar and airborne in situ measurements.ATMOSPHERIC CHEMISTRY AND PHYSICS,19(22),13773-13788.
MLA	Haarig, Moritz,et al."Profiles of cloud condensation nuclei, dust mass concentration, and ice-nucleating-particle-relevant aerosol properties in the Saharan Air Layer over Barbados from polarization lidar and airborne in situ measurements".ATMOSPHERIC CHEMISTRY AND PHYSICS 19.22(2019):13773-13788.