Knowledge Resource Center for Ecological Environment in Arid Area
DOI | 10.3390/atmos10110680 |
Dust Heterogeneous Reactions during Long-Range Transport of a Severe Dust Storm in May 2017 over East Asia | |
Wang, Zhe1,2; Uno, Itsushi1; Yumimoto, Keiya1; Pan, Xiaole2; Chen, Xueshun2; Li, Jie2; Wang, Zifa2; Shimizu, Atsushi3; Sugimoto, Nobuo3 | |
通讯作者 | Wang, Zhe |
来源期刊 | ATMOSPHERE
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EISSN | 2073-4433 |
出版年 | 2019 |
卷号 | 10期号:11 |
英文摘要 | Dust aerosol has important climate and environmental effects, which could be changed by internally mixing with anthropogenic aerosol as a result of heterogeneous reactions; however, the importance of these reactions is not fully understood yet. In this study, synergetic observations and an air quality model were used to analyze the transport of a severe dust storm and its impacts on nitrate and sulfate levels over East Asia between 3 and 11 May 2017. The model successfully reproduced the occurrence and transport of the dust storm compared to dust RGB imageries of the Himawari-8 satellite and dust extinction coefficients observed by LIDAR. The model also reasonably simulated the variations of observed nitrate and sulfate concentrations, and the results indicated that the dust heterogeneous reactions were dominant pathways for nitrate formation, but they had limited contribution for sulfate in both fine and coarse mode in Fukuoka, Japan. Dust nitrate formed rapidly after leaving China, and the highest period-averaged concentration of dust nitrate (>5 mu g m(-3)) was shown over the Yellow Sea. Based on model results; we found that the mass ratio of dust nitrate to dust aerosol could reach 10% over the Pacific Ocean. Our results confirmed the importance of heterogeneous reactions on compositions of dust particles. |
英文关键词 | mineral dust heterogeneous reaction acid uptake Himawari-8 LIDAR NAQPMS |
类型 | Article |
语种 | 英语 |
国家 | Japan ; Peoples R China |
开放获取类型 | gold |
收录类别 | SCI-E |
WOS记录号 | WOS:000502272000042 |
WOS关键词 | AIR-QUALITY ; MINERAL DUST ; ANTHROPOGENIC POLLUTANTS ; DESERT DUST ; MODEL ; AEROSOL ; EMISSION ; OZONE ; DEPOSITION ; PARTICLES |
WOS类目 | Environmental Sciences ; Meteorology & Atmospheric Sciences |
WOS研究方向 | Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences |
EI主题词 | 2019-11-01 |
来源机构 | 中国科学院大气物理研究所 |
资源类型 | 期刊论文 |
条目标识符 | http://119.78.100.177/qdio/handle/2XILL650/310539 |
作者单位 | 1.Kyushu Univ, Res Inst Appl Mech, Fukuoka, Fukuoka 8168580, Japan; 2.Chinese Acad Sci, Inst Atmospher Phys, State Key Lab Atmospher Boundary Layer Phys & Atm, Beijing 100029, Peoples R China; 3.Natl Inst Environm Studies, Tsukuba, Ibaraki 3058506, Japan |
推荐引用方式 GB/T 7714 | Wang, Zhe,Uno, Itsushi,Yumimoto, Keiya,et al. Dust Heterogeneous Reactions during Long-Range Transport of a Severe Dust Storm in May 2017 over East Asia[J]. 中国科学院大气物理研究所,2019,10(11). |
APA | Wang, Zhe.,Uno, Itsushi.,Yumimoto, Keiya.,Pan, Xiaole.,Chen, Xueshun.,...&Sugimoto, Nobuo.(2019).Dust Heterogeneous Reactions during Long-Range Transport of a Severe Dust Storm in May 2017 over East Asia.ATMOSPHERE,10(11). |
MLA | Wang, Zhe,et al."Dust Heterogeneous Reactions during Long-Range Transport of a Severe Dust Storm in May 2017 over East Asia".ATMOSPHERE 10.11(2019). |
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