Arid
DOI10.3390/atmos10110680
Dust Heterogeneous Reactions during Long-Range Transport of a Severe Dust Storm in May 2017 over East Asia
Wang, Zhe1,2; Uno, Itsushi1; Yumimoto, Keiya1; Pan, Xiaole2; Chen, Xueshun2; Li, Jie2; Wang, Zifa2; Shimizu, Atsushi3; Sugimoto, Nobuo3
通讯作者Wang, Zhe
来源期刊ATMOSPHERE
EISSN2073-4433
出版年2019
卷号10期号:11
英文摘要Dust aerosol has important climate and environmental effects, which could be changed by internally mixing with anthropogenic aerosol as a result of heterogeneous reactions; however, the importance of these reactions is not fully understood yet. In this study, synergetic observations and an air quality model were used to analyze the transport of a severe dust storm and its impacts on nitrate and sulfate levels over East Asia between 3 and 11 May 2017. The model successfully reproduced the occurrence and transport of the dust storm compared to dust RGB imageries of the Himawari-8 satellite and dust extinction coefficients observed by LIDAR. The model also reasonably simulated the variations of observed nitrate and sulfate concentrations, and the results indicated that the dust heterogeneous reactions were dominant pathways for nitrate formation, but they had limited contribution for sulfate in both fine and coarse mode in Fukuoka, Japan. Dust nitrate formed rapidly after leaving China, and the highest period-averaged concentration of dust nitrate (>5 mu g m(-3)) was shown over the Yellow Sea. Based on model results; we found that the mass ratio of dust nitrate to dust aerosol could reach 10% over the Pacific Ocean. Our results confirmed the importance of heterogeneous reactions on compositions of dust particles.
英文关键词mineral dust heterogeneous reaction acid uptake Himawari-8 LIDAR NAQPMS
类型Article
语种英语
国家Japan ; Peoples R China
开放获取类型gold
收录类别SCI-E
WOS记录号WOS:000502272000042
WOS关键词AIR-QUALITY ; MINERAL DUST ; ANTHROPOGENIC POLLUTANTS ; DESERT DUST ; MODEL ; AEROSOL ; EMISSION ; OZONE ; DEPOSITION ; PARTICLES
WOS类目Environmental Sciences ; Meteorology & Atmospheric Sciences
WOS研究方向Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
EI主题词2019-11-01
来源机构中国科学院大气物理研究所
资源类型期刊论文
条目标识符http://119.78.100.177/qdio/handle/2XILL650/310539
作者单位1.Kyushu Univ, Res Inst Appl Mech, Fukuoka, Fukuoka 8168580, Japan;
2.Chinese Acad Sci, Inst Atmospher Phys, State Key Lab Atmospher Boundary Layer Phys & Atm, Beijing 100029, Peoples R China;
3.Natl Inst Environm Studies, Tsukuba, Ibaraki 3058506, Japan
推荐引用方式
GB/T 7714
Wang, Zhe,Uno, Itsushi,Yumimoto, Keiya,et al. Dust Heterogeneous Reactions during Long-Range Transport of a Severe Dust Storm in May 2017 over East Asia[J]. 中国科学院大气物理研究所,2019,10(11).
APA Wang, Zhe.,Uno, Itsushi.,Yumimoto, Keiya.,Pan, Xiaole.,Chen, Xueshun.,...&Sugimoto, Nobuo.(2019).Dust Heterogeneous Reactions during Long-Range Transport of a Severe Dust Storm in May 2017 over East Asia.ATMOSPHERE,10(11).
MLA Wang, Zhe,et al."Dust Heterogeneous Reactions during Long-Range Transport of a Severe Dust Storm in May 2017 over East Asia".ATMOSPHERE 10.11(2019).
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