Arid
DOI10.4209/aaqr.2015.04.0256
Water-Soluble Organic Nitrogen in High Mountain Snow Samples from Central Japan
Mochizuki, Tomoki1; Kawamura, Kimitaka1; Aoki, Kazuma2
通讯作者Kawamura, Kimitaka
会议名称2nd Atmospheric Chemistry and Physics at Mountain Sites Symposium
会议日期AUG 11-15, 2014
会议地点Steamboat Springs, CO
英文摘要

We measured water-soluble organic nitrogen (WSON) in snow pit samples, which were collected at the Murodo-Daira snowfield near the summit of Mt. Tateyama, central Japan in 2008, 2009, and 2011. The concentrations of WSON ranged from 12.8 to 96.7 ng g(-1), which were significantly lower than those reported in continental wet deposition samples from the Asian continent. WSON may be largely diluted in the snow samples during snowing processes over the high mountains. We found that WSON significantly correlated with nss-Ca2+ and water-soluble organic carbon (WSOC). Concentrations of WSON are likely controlled by the intensity of Asian dust events. Contributions of WSON to water soluble total nitrogen (WSTN) in snow pit sequence was found to be 15 +/- 10%, which is lower than those (63-91%) of reference dust materials collected in China. Mass concentration ratio of WSOC/WSON was on average 23.7, which is significantly higher than the C/N weight ratio (5.6) calculated from the Redfield ratio. This result suggests that WSOC is largely produced by secondary photochemical oxidation of anthropogenic volatile organic compounds during the transport from East Asia to the high mountain areas in Japan. On the other hand, WSON may be contributed from Asian dusts from arid areas in China whereas water-soluble inorganic nitrogen may be derived from pollution sources.


英文关键词Water-soluble organic nitrogen High mountain snow Central Japan Long-range atmospheric transport East Asia
来源出版物AEROSOL AND AIR QUALITY RESEARCH
ISSN1680-8584
EISSN2071-1409
出版年2016
卷号16
期号3
页码632-639
出版者TAIWAN ASSOC AEROSOL RES-TAAR
类型Article;Proceedings Paper
语种英语
国家Japan
收录类别SCI-E ; CPCI-S
WOS记录号WOS:000371498900014
WOS关键词AEROSOLS ; DEPOSITION ; CARBON ; FOG ; COMPONENTS ; PARTICLES ; ORIGIN ; MATTER ; VALLEY ; FOREST
WOS类目Environmental Sciences
WOS研究方向Environmental Sciences & Ecology
资源类型会议论文
条目标识符http://119.78.100.177/qdio/handle/2XILL650/304880
作者单位1.Hokkaido Univ, Inst Low Temp Sci, Kita Ku, N19 W8, Sapporo, Hokkaido 0600819, Japan;
2.Toyama Univ, Dept Earth Sci, Fac Sci, 3190 Gofuku, Toyama 9308555, Japan
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Mochizuki, Tomoki,Kawamura, Kimitaka,Aoki, Kazuma. Water-Soluble Organic Nitrogen in High Mountain Snow Samples from Central Japan[C]:TAIWAN ASSOC AEROSOL RES-TAAR,2016:632-639.
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