干旱区生态环境知识资源中心(Arid): Final Report for SERDP Project RC-1649: Advanced Chemical Measurements of Smoke from DoD-prescribed Burns

Arid

DOI	10.2172/1113606
报告编号	PNNL--23025
来源ID	OSTI_ID: 1113606
	Final Report for SERDP Project RC-1649: Advanced Chemical Measurements of Smoke from DoD-prescribed Burns
	Johnson, Timothy J. [Pacific Northwest National Lab. (PNNL), Richland, WA (United States)]; Weise, David [Pacific Northwest National Lab. (PNNL), Richland, WA (United States)]; Lincoln, E. N. [Pacific Northwest National Lab. (PNNL), Richland, WA (United States)]; Sams, Robert L. [Pacific Northwest National Lab. (PNNL), Richland, WA (United States)]; Cameron, Melanie [Pacific Northwest National Lab. (PNNL), Richland, WA (United States)]; Veres, Patrick [Pacific Northwest National Lab. (PNNL), Richland, WA (United States)]; Yokelson, Robert J. [Pacific Northwest National Lab. (PNNL), Richland, WA (United States)]; Urbanski, Shawn [Pacific Northwest National Lab. (PNNL), Richland, WA (United States)]; Profeta, Luisa T. [Pacific Northwest National Lab. (PNNL), Richland, WA (United States)]; Williams, S. [Pacific Northwest National Lab. (PNNL), Richland, WA (United States)]; Gilman, Jessica [Pacific Northwest National Lab. (PNNL), Richland, WA (United States)]; Kuster, W. C. [Pacific Northwest National Lab. (PNNL), Richland, WA (United States)]; Akagi, Sheryl [Pacific Northwest National Lab. (PNNL), Richland, WA (United States)]; Stockwell, Chelsea E. [Pacific Northwest National Lab. (PNNL), Richland, WA (United States)]; Mendoza, Albert [Pacific Northwest National Lab. (PNNL), Richland, WA (United States)]; Wold, Cyle E. [Pacific Northwest National Lab. (PNNL), Richland, WA (United States)]; Warneke, Carsten [Pacific Northwest National Lab. (PNNL), Richland, WA (United States)]; de Gouw, Joost A. [Pacific Northwest National Lab. (PNNL), Richland, WA (United States)]; Burling, Ian R. [Pacific Northwest National Lab. (PNNL), Richland, WA (United States)]; Reardon, James [Pacific Northwest National Lab. (PNNL), Richland, WA (United States)]; Schneider, Matthew D. [Pacific Northwest National Lab. (PNNL), Richland, WA (United States)]; Griffith, David W.T. [Pacific Northwest National Lab. (PNNL), Richland, WA (United States)]; Roberts, James M. [Pacific Northwest National Lab. (PNNL), Richland, WA (United States)]
英文摘要	Objectives: Project RC-1649, 鈥淎dvanced Chemical Measurement of Smoke from DoD-prescribed Burns鈥?was undertaken to use advanced instrumental techniques to study in detail the particulate and vapor-phase chemical composition of the smoke that results from prescribed fires used as a land management tool on DoD bases, particularly bases in the southeastern U.S. The statement of need (SON) called for 鈥?1) improving characterization of fuel consumption鈥?and 鈥?2) improving characterization of air emissions under both flaming and smoldering conditions with respect to volatile organic compounds, heavy metals, and reactive gases.鈥?The measurements and fuels were from several bases throughout the southeast (Camp Lejeune, Ft. Benning, and Ft. Jackson) and were carried out in collaboration and conjunction with projects 1647 (models) and 1648 (particulates, SW bases). Technical Approach: We used an approach that featured developing techniques for measuring biomass burning emission species in both the laboratory and field and developing infrared (IR) spectroscopy in particular. Using IR spectroscopy and other methods, we developed emission factors (EF, g of effluent per kg of fuel burned) for dozens of chemical species for several common southeastern fuel types. The major measurement campaigns were laboratory studies at the Missoula Fire Sciences Laboratory (FSL) as well as field campaigns at Camp Lejeune, NC, Ft. Jackson, SC, and in conjunction with 1648 at Vandenberg AFB, and Ft. Huachuca. Comparisons and fusions of laboratory and field data were also carried out, using laboratory fuels from the same bases. Results: The project enabled new technologies and furthered basic science, mostly in the area of infrared spectroscopy, a broadband method well suited to biomass burn studies. Advances in hardware, software and supporting reference data realized a nearly 20x improvement in sensitivity and now provide quantitative IR spectra for potential detection of ~60 new species and actual field quantification of several new species such as nitrous acid, glycolaldehyde, 伪-/尾-pinene and D-limonene. The new reference data also permit calculation of the global warming potential (GWP) of the greenhouse gases by enabling 1) detection of their ambient concentrations, and 2) quantifying their ability to absorb IR radiation.
出版年	2013
报告类型	Technical Report
语种	英语
国家	美国
来源学科分类	47 OTHER INSTRUMENTATION
URL	http://www.osti.gov/scitech/servlets/purl/1113606
资源类型	科技报告
条目标识符	http://119.78.100.177/qdio/handle/2XILL650/270878
推荐引用方式 GB/T 7714	Johnson, Timothy J. [Pacific Northwest National Lab. ,Weise, David [Pacific Northwest National Lab. ,Lincoln, E. N. [Pacific Northwest National Lab. ,et al. Final Report for SERDP Project RC-1649: Advanced Chemical Measurements of Smoke from DoD-prescribed Burns,2013.