Arid
DOI10.1039/c8nr09353a
Hybrid organic nanocrystal/carbon nanotube film electrodes for air- and photo-stable perovskite photovoltaics
Siram, Raja Bhaskar Kanth1,2; Khenkin, Mark V.3; Niazov-Elkan, Angelica1; Anoop, K. M.3; Weissman, Haim1; Katz, Eugene A.3,4; Visoly-Fisher, Iris3,4; Rybtchinski, Boris1
通讯作者Katz, Eugene A. ; Visoly-Fisher, Iris ; Rybtchinski, Boris
来源期刊NANOSCALE
ISSN2040-3364
EISSN2040-3372
出版年2019
卷号11期号:8页码:3733-3740
英文摘要We report on utilizing free-standing hybrid perylenediimide/carbon nanotube (PDI/CNT) films fabricated in air as back contacts for fully inorganic perovskite solar cells (glass/FTO/dense TiO2/mesoporous TiO2/ CsPbBr3/back electrode). The back contact electrode connection is performed by film transfer rather than by vacuum deposition or by wet processing, allowing the formation of highly homogeneous contacts under ambient conditions. The use of this novel electrode in solar cells based on CsPbBr3 resulted in efficiency of 5.8% without a hole transporting layer; it is significantly improved in comparison to the reference cells with standard gold electrodes. Overall device fabrication can be performed on air, using inexpensive processing methods. The hybrid film electrodes dramatically improve the cell photo-stability under ambient conditions and under real-life operating conditions outdoors. The champion unencapsulated device demonstrated less than 30% efficiency loss over 6 weeks of outdoor aging in Negev desert conditions. The CNT/PDI electrodes offer the combination of fabrication simplicity, unique contacting approach, high efficiency and good operational stability for perovskite photovoltaics.
类型Article
语种英语
国家Israel ; India
收录类别SCI-E
WOS记录号WOS:000459504400030
WOS关键词LONG-TERM STABILITY ; SOLAR-CELLS ; INDUCED DEGRADATION ; CARBON NANOTUBES ; EFFICIENT ; DIFFUSION ; LENGTHS ; IMPACT ; LAYER ; GOLD
WOS类目Chemistry, Multidisciplinary ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary ; Physics, Applied
WOS研究方向Chemistry ; Science & Technology - Other Topics ; Materials Science ; Physics
来源机构Ben-Gurion University of the Negev
资源类型期刊论文
条目标识符http://119.78.100.177/qdio/handle/2XILL650/217708
作者单位1.Weizmann Inst Sci, Dept Organ Chem, IL-76100 Rehovot, Israel;
2.Gitam Univ, Sch Sci, Dept Chem, Hyderabad 502329, Telangana, India;
3.Ben Gurion Univ Negev, J Blaustein Inst Desert Res, Swiss Inst Dryland Environm & Energy Res, Dept Solar Energy & Environm Phys, IL-8499000 Midreshet Ben Gurion, Israel;
4.Ben Gurion Univ Negev, Ilse Katz Inst Nanoscale Sci & Technol, IL-8410501 Beer Sheva, Israel
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GB/T 7714
Siram, Raja Bhaskar Kanth,Khenkin, Mark V.,Niazov-Elkan, Angelica,et al. Hybrid organic nanocrystal/carbon nanotube film electrodes for air- and photo-stable perovskite photovoltaics[J]. Ben-Gurion University of the Negev,2019,11(8):3733-3740.
APA Siram, Raja Bhaskar Kanth.,Khenkin, Mark V..,Niazov-Elkan, Angelica.,Anoop, K. M..,Weissman, Haim.,...&Rybtchinski, Boris.(2019).Hybrid organic nanocrystal/carbon nanotube film electrodes for air- and photo-stable perovskite photovoltaics.NANOSCALE,11(8),3733-3740.
MLA Siram, Raja Bhaskar Kanth,et al."Hybrid organic nanocrystal/carbon nanotube film electrodes for air- and photo-stable perovskite photovoltaics".NANOSCALE 11.8(2019):3733-3740.
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