Arid
DOI10.1021/acs.est.9b02386
Climate and Vegetation As Primary Drivers for Global Mercury Storage in Surface Soil
Wang, Xun1; Yuan, Wei1,2; Lin, Che-Jen3,4; Zhang, Leiming5; Zhang, Hui1; Feng, Xinbin1,6
通讯作者Feng, Xinbin
来源期刊ENVIRONMENTAL SCIENCE & TECHNOLOGY
ISSN0013-936X
EISSN1520-5851
出版年2019
卷号53期号:18页码:10665-10675
英文摘要Soil is the largest Hg reservoir globally. Data of Hg concentration in surface soil are fundamental to understanding environmental Hg cycling. However, present knowledge on the quantity and global distribution of Hg in soil remains deficient. Using stable Hg isotopic analyses and geospatial data, the concentration and global spatial distribution of Hg in surface soil of 0-20 cm depth have been developed. It is estimated that 1088 +/- 379 Gg of Hg is stored in surface soil globally. Thirty-two percent of the surface Hg storage resides in tropical/subtropical forest regions, 23% in temperate/boreal forest regions, 28% in grassland and steppe and shrubland, 7% in tundra, and 10% in desert and xeric shrubland. Evidence from Hg isotopic signatures points to atmospheric Hg-0 dry deposition through vegetation uptake as the primary source of Hg in surface soil. Given the influence of changing climate on vegetative development, global climate change can act as an important forcing factor for shaping spatial distribution of Hg in surface soil. This active forcing cycle significantly dilutes the impacts caused by Hg release from anthropogenic sources, and needs to be considered in assessing the effectiveness of reducing Hg use and emissions as specified in Minamata Convention on Mercury.
类型Article
语种英语
国家Peoples R China ; USA ; Canada
收录类别SCI-E
WOS记录号WOS:000487163000016
WOS关键词GASEOUS ELEMENTAL MERCURY ; ATMOSPHERIC MERCURY ; ISOTOPIC COMPOSITION ; SPATIAL-DISTRIBUTION ; METHYL MERCURY ; UNITED-STATES ; FOREST FLOOR ; MINING AREA ; DEPOSITION ; FLUXES
WOS类目Engineering, Environmental ; Environmental Sciences
WOS研究方向Engineering ; Environmental Sciences & Ecology
资源类型期刊论文
条目标识符http://119.78.100.177/qdio/handle/2XILL650/215530
作者单位1.Chinese Acad Sci, Inst Geochem, State Key Lab Environm Geochem, Guiyang 550081, Guizhou, Peoples R China;
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China;
3.Lamar Univ, Ctr Adv Water & Air Qual, Beaumont, TX 77705 USA;
4.Lamar Univ, Dept Civil & Environm Engn, Beaumont, TX 77705 USA;
5.Environm & Climate Change Canada, Air Qual Res Div, Sci & Technol Branch, Toronto, ON M3H 5T4, Canada;
6.Chinese Acad Sci, Ctr Excellence Quaternary Sci & Global Change, Xian 710061, Shaanxi, Peoples R China
推荐引用方式
GB/T 7714
Wang, Xun,Yuan, Wei,Lin, Che-Jen,et al. Climate and Vegetation As Primary Drivers for Global Mercury Storage in Surface Soil[J],2019,53(18):10665-10675.
APA Wang, Xun,Yuan, Wei,Lin, Che-Jen,Zhang, Leiming,Zhang, Hui,&Feng, Xinbin.(2019).Climate and Vegetation As Primary Drivers for Global Mercury Storage in Surface Soil.ENVIRONMENTAL SCIENCE & TECHNOLOGY,53(18),10665-10675.
MLA Wang, Xun,et al."Climate and Vegetation As Primary Drivers for Global Mercury Storage in Surface Soil".ENVIRONMENTAL SCIENCE & TECHNOLOGY 53.18(2019):10665-10675.
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