Arid
DOI10.1016/j.talanta.2018.03.059
Quantitative study of the mineralogical composition of mineral dust aerosols by X-ray diffraction
Nowak, Sophie1; Lafon, Sandra2; Caquineau, Sandrine3; Journet, Emilie2; Laurent, Benoit2
通讯作者Nowak, Sophie
来源期刊TALANTA
ISSN0039-9140
EISSN1873-3573
出版年2018
卷号186页码:133-139
英文摘要

Mineral dust aerosols, produced by wind erosion in arid regions and semi-arid surfaces, are important components of the atmosphere that affect the Earth radiative budget, atmospheric chemistry and biogeochemical cycles. Dust aerosol particles are composed of a complex mixture of various minerals, mainly clays, calcite, quartz, feldspars and iron oxides. The nature and the relative abundance of the minerals are key parameters to evaluate mineral dust environmental impacts. Strong limitations remain to quantify the mineralogical composition of dust particles, mainly due to the low mass of in-situ collected dust particle samples. In this study, an analytical method and X-Ray Diffraction (XRD) measurements are presented to quantify the mineralogical composition of low mass aerosol particle samples. The method is applied on reference minerals (illite, kaolinite and palygorskite) commonly present in desert dust aerosols, as well as on lab-generated dust aerosols from desert soils. XRD measurements of theses samples in rotation in a glass capillary are combined with the Rietveld refinement method. The results obtained are repeatable and confronted to theoretical values given in the literature for the reference minerals. This method allows us to quantify the mineralogical composition of low mass dust mineral samples with an unprecedented accuracy.


英文关键词Mineralogical composition Mineral dust particles Powder X-Ray Diffraction Rietveld analysis
类型Article
语种英语
国家France
收录类别SCI-E
WOS记录号WOS:000435048800019
WOS关键词SOURCE REGIONS ; SAHARAN DUST ; IRON-OXIDES ; SOLUBILITY ; DEPOSITION ; PATTERNS ; ATLANTIC ; OCEAN ; LINE
WOS类目Chemistry, Analytical
WOS研究方向Chemistry
来源机构French National Research Institute for Sustainable Development ; E17
资源类型期刊论文
条目标识符http://119.78.100.177/qdio/handle/2XILL650/213416
作者单位1.Univ Paris Diderot, UFR Chim, Plateforme Rayons X, Paris, France;
2.Univ Paris Est Creteil, Univ Paris Diderot, IPSL, LISA,UMR 7583, Creteil, France;
3.Sorbonne Univ, UPMC, CNRS, MNHN,IRD,LOCEAN, Bondy, France
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GB/T 7714
Nowak, Sophie,Lafon, Sandra,Caquineau, Sandrine,et al. Quantitative study of the mineralogical composition of mineral dust aerosols by X-ray diffraction[J]. French National Research Institute for Sustainable Development, E17,2018,186:133-139.
APA Nowak, Sophie,Lafon, Sandra,Caquineau, Sandrine,Journet, Emilie,&Laurent, Benoit.(2018).Quantitative study of the mineralogical composition of mineral dust aerosols by X-ray diffraction.TALANTA,186,133-139.
MLA Nowak, Sophie,et al."Quantitative study of the mineralogical composition of mineral dust aerosols by X-ray diffraction".TALANTA 186(2018):133-139.
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