Arid
DOI10.1016/j.nimb.2018.08.047
Carbon-14 content in tree and soil samples at the Idaho National Laboratory nuclear site
Ward, Jessica L.; Snow, Mathew S.; Olson, John E.; Ball, Duane; Adamic, Mary L.
通讯作者Ward, Jessica L.
来源期刊NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS
ISSN0168-583X
EISSN1872-9584
出版年2018
卷号437页码:103-109
英文摘要

Idaho National Laboratory (INL) is a nuclear research facility located in southeastern Idaho, USA; over the course of its operational history, INL has operated 52 reactors and 1 reactor fuel reprocessing facility. To determine the extent to which previous nuclear operations at INL have impacted local environmental carbon-14 (C-14) concentrations, tree and soil samples from the INL desert and surrounding areas were collected, combusted, and analyzed by Accelerator Mass Spectrometry (AMS). Transport models of the plumes from the Advanced Test Reactor Facility (ATR) and the Idaho Chemical Processing Plant (ICPP) suggest the historic annual integrated plume distributions from each of these source terms was most likely in the northeast-southwest direction, with very little ground contact from stack emissions in the immediate vicinity of the facilities and maximum estimated ground contact arising similar to 400-1000 m to the northeast/southwest from each facility. C-14 data from annual growth ring data from trees located immediately adjacent to the ATR, INL’s Central Facilities Area (CFA), and Mud Lake, Idaho (ML) are in statistical agreement with regional nuclear weapons testing fallout backgrounds. Surface soil samples taken near a low level radioactive disposal facility and downwind from the ICPP show percent modern carbon (pMC) values ranging from 28 +/- 2 to 92 +/- 4, suggesting a mixture of aged and modern background carbon containing materials. Taken together, these data suggest that C-14 in the INL region is predominantly derived from a mixture of aged and modern background sources (e.g. nuclear weapons testing fallout), with insignificant contributions from INL source terms.


英文关键词Accelerator mass spectrometry AMS Carbon-14 Idaho National Laboratory
类型Article
语种英语
国家USA
收录类别SCI-E
WOS记录号WOS:000452933000017
WOS类目Instruments & Instrumentation ; Nuclear Science & Technology ; Physics, Atomic, Molecular & Chemical ; Physics, Nuclear
WOS研究方向Instruments & Instrumentation ; Nuclear Science & Technology ; Physics
资源类型期刊论文
条目标识符http://119.78.100.177/qdio/handle/2XILL650/211857
作者单位Idaho Natl Lab, POB 1625, Idaho Falls, ID 83415 USA
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GB/T 7714
Ward, Jessica L.,Snow, Mathew S.,Olson, John E.,et al. Carbon-14 content in tree and soil samples at the Idaho National Laboratory nuclear site[J],2018,437:103-109.
APA Ward, Jessica L.,Snow, Mathew S.,Olson, John E.,Ball, Duane,&Adamic, Mary L..(2018).Carbon-14 content in tree and soil samples at the Idaho National Laboratory nuclear site.NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS,437,103-109.
MLA Ward, Jessica L.,et al."Carbon-14 content in tree and soil samples at the Idaho National Laboratory nuclear site".NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS 437(2018):103-109.
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