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In this review, the shifts in organic matter (OM) accumulation and C:N ratios in lake sediments to reconstruct paleoclimate and paleo-environmental changes since the early Holocene period are presented. The C:N proxy data of total OM reflect wet climatic conditions during early Holocene (10 to 8.2 kyrs BP) due to enhanced southwest monsoon. This was followed by intermittent arid conditions during the mid and late Holocene period (8.2 to 2.8 kyr BP). Enhanced values of C:N ratio during middle to late Holocene (7.8-2.3 kyrs B.P) indicate periods with lower lake levels and minimum precipitation, while decreased C:N ratio point to stronger SW monsoon and expansion of the lakes. Further, C:N and delta C-13 results from the lake sediments reveal a detailed and continuous paleo-environmental changes in the relative sources of OM (allochthonous vs autochthonous). Proxy records using such natural archives have also been utilized to reconstruct past extreme events and environmental changes around the lake systems, such as causes for lake desiccation, hydrographic changes, alternations between C-3 and C-4 vegetation and historical disturbances in the catchment area since the early-late Holocene period coupled with the Indian summer monsoon.