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DOI | 10.1007/s10874-018-9379-y |
Seasonal and annual trends of carbonaceous species of PM10 over a megacity Delhi, India during 2010-2017 | |
Sharma, S. K.; Mandal, T. K.; Sharma, A.; Saraswati; Jain, Srishti | |
通讯作者 | Sharma, S. K. |
来源期刊 | JOURNAL OF ATMOSPHERIC CHEMISTRY
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ISSN | 0167-7764 |
EISSN | 1573-0662 |
出版年 | 2018 |
卷号 | 75期号:3页码:305-318 |
英文摘要 | PM10 samples were collected to characterize the seasonal and annual trends of carbonaceous content inPM(10) at an urban site of megacity Delhi, India from January 2010 to December 2017. Organic carbon (OC) and elemental carbon (EC) concentrations were quantified by thermal-optical transmission (TOT) method of PM10 samples collected at Delhi. The average concentrations of PM10, OC, EC and TCA (total carbonaceous aerosol) were 222 +/- 87 (range: 48.2-583.8gm(-3)), 25.6 +/- 14.0 (range: 4.2-82.5gm(-3)), 8.7 +/- 5.8 (range: 0.8-35.6gm(-3)) and 54.7 +/- 30.6gm(-3) (range: 8.4-175.2gm(-3)), respectively during entire sampling period. The average secondary organic carbon (SOC) concentration ranged from 2.5-9.1 gm(-3) in PM10, accounting from 14 to 28% of total OC mass concentration of PM10. Significant seasonal variations were recorded in concentrations of PM10, OC, EC and TCA with maxima during winter and minima during monsoon seasons. In the present study, the positive linear trend between OC and EC were recorded during winter (R-2=0.53), summer (R-2=0.59) and monsoon (R-2=0.78) seasons. This behaviour suggests the contribution of similar sources and common atmospheric processes in both the fractions. OC/EC weightratio suggested that vehicular emissions, fossil fuel combustion and biomass burning could be the major sources of carbonaceous aerosols of PM10 at the megacity Delhi, India. Trajectory analysis indicates that the air mass approches to the sampling site is mainly from Indo Gangetic plain (IGP) region (Uttar Pradesh, Haryana and Punjab etc.), Thar desert, Afghanistan, Pakistan and surrounding areas. |
英文关键词 | PM10 Organic carbon Elemental carbon Carbonaceous aerosols |
类型 | Article |
语种 | 英语 |
国家 | India |
收录类别 | SCI-E |
WOS记录号 | WOS:000451048000004 |
WOS关键词 | SOURCE APPORTIONMENT ; ORGANIC-CARBON ; URBAN-ENVIRONMENT ; ELEMENTAL CARBON ; AEROSOL ; PM2.5 ; EC ; OC ; VARIABILITY ; OUTFLOW |
WOS类目 | Environmental Sciences ; Meteorology & Atmospheric Sciences |
WOS研究方向 | Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences |
资源类型 | 期刊论文 |
条目标识符 | http://119.78.100.177/qdio/handle/2XILL650/210683 |
作者单位 | CSIR, Natl Phys Lab, Environm Sci & Biomed Metrol Div, Dr K S Krishnan Rd, New Delhi 110012, India |
推荐引用方式 GB/T 7714 | Sharma, S. K.,Mandal, T. K.,Sharma, A.,et al. Seasonal and annual trends of carbonaceous species of PM10 over a megacity Delhi, India during 2010-2017[J],2018,75(3):305-318. |
APA | Sharma, S. K.,Mandal, T. K.,Sharma, A.,Saraswati,&Jain, Srishti.(2018).Seasonal and annual trends of carbonaceous species of PM10 over a megacity Delhi, India during 2010-2017.JOURNAL OF ATMOSPHERIC CHEMISTRY,75(3),305-318. |
MLA | Sharma, S. K.,et al."Seasonal and annual trends of carbonaceous species of PM10 over a megacity Delhi, India during 2010-2017".JOURNAL OF ATMOSPHERIC CHEMISTRY 75.3(2018):305-318. |
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