Arid
DOI10.1007/s10874-018-9379-y
Seasonal and annual trends of carbonaceous species of PM10 over a megacity Delhi, India during 2010-2017
Sharma, S. K.; Mandal, T. K.; Sharma, A.; Saraswati; Jain, Srishti
通讯作者Sharma, S. K.
来源期刊JOURNAL OF ATMOSPHERIC CHEMISTRY
ISSN0167-7764
EISSN1573-0662
出版年2018
卷号75期号:3页码:305-318
英文摘要

PM10 samples were collected to characterize the seasonal and annual trends of carbonaceous content inPM(10) at an urban site of megacity Delhi, India from January 2010 to December 2017. Organic carbon (OC) and elemental carbon (EC) concentrations were quantified by thermal-optical transmission (TOT) method of PM10 samples collected at Delhi. The average concentrations of PM10, OC, EC and TCA (total carbonaceous aerosol) were 222 +/- 87 (range: 48.2-583.8gm(-3)), 25.6 +/- 14.0 (range: 4.2-82.5gm(-3)), 8.7 +/- 5.8 (range: 0.8-35.6gm(-3)) and 54.7 +/- 30.6gm(-3) (range: 8.4-175.2gm(-3)), respectively during entire sampling period. The average secondary organic carbon (SOC) concentration ranged from 2.5-9.1 gm(-3) in PM10, accounting from 14 to 28% of total OC mass concentration of PM10. Significant seasonal variations were recorded in concentrations of PM10, OC, EC and TCA with maxima during winter and minima during monsoon seasons. In the present study, the positive linear trend between OC and EC were recorded during winter (R-2=0.53), summer (R-2=0.59) and monsoon (R-2=0.78) seasons. This behaviour suggests the contribution of similar sources and common atmospheric processes in both the fractions. OC/EC weightratio suggested that vehicular emissions, fossil fuel combustion and biomass burning could be the major sources of carbonaceous aerosols of PM10 at the megacity Delhi, India. Trajectory analysis indicates that the air mass approches to the sampling site is mainly from Indo Gangetic plain (IGP) region (Uttar Pradesh, Haryana and Punjab etc.), Thar desert, Afghanistan, Pakistan and surrounding areas.


英文关键词PM10 Organic carbon Elemental carbon Carbonaceous aerosols
类型Article
语种英语
国家India
收录类别SCI-E
WOS记录号WOS:000451048000004
WOS关键词SOURCE APPORTIONMENT ; ORGANIC-CARBON ; URBAN-ENVIRONMENT ; ELEMENTAL CARBON ; AEROSOL ; PM2.5 ; EC ; OC ; VARIABILITY ; OUTFLOW
WOS类目Environmental Sciences ; Meteorology & Atmospheric Sciences
WOS研究方向Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
资源类型期刊论文
条目标识符http://119.78.100.177/qdio/handle/2XILL650/210683
作者单位CSIR, Natl Phys Lab, Environm Sci & Biomed Metrol Div, Dr K S Krishnan Rd, New Delhi 110012, India
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GB/T 7714
Sharma, S. K.,Mandal, T. K.,Sharma, A.,et al. Seasonal and annual trends of carbonaceous species of PM10 over a megacity Delhi, India during 2010-2017[J],2018,75(3):305-318.
APA Sharma, S. K.,Mandal, T. K.,Sharma, A.,Saraswati,&Jain, Srishti.(2018).Seasonal and annual trends of carbonaceous species of PM10 over a megacity Delhi, India during 2010-2017.JOURNAL OF ATMOSPHERIC CHEMISTRY,75(3),305-318.
MLA Sharma, S. K.,et al."Seasonal and annual trends of carbonaceous species of PM10 over a megacity Delhi, India during 2010-2017".JOURNAL OF ATMOSPHERIC CHEMISTRY 75.3(2018):305-318.
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