Arid
DOI10.1016/j.chemosphere.2018.09.021
Distinctive distributions and migrations of 239+240PU and Am-241 in Chinese forest, grassland and desert soils
Ni, Youyi1,3; Wang, Zhongtang2; Guo, Qiuju1; Zheng, Jian3; Li, Sixuan1; Lin, Jinxian2; Tan, Zhaoyi2; Huang, Wenna4
通讯作者Wang, Zhongtang ; Zheng, Jian
来源期刊CHEMOSPHERE
ISSN0045-6535
EISSN1879-1298
出版年2018
卷号212页码:1002-1009
英文摘要

The vertical distributions and downward migrations of the global fallout derived Pu239+240 and Am-241 in diverse types of Chinese soils (forest, grassland and desert) were studied. The mean Pu239+240 and Am-241 activity concentrations in the investigated soil cores were 0.28-0.69 mBq/g and 0.13-037 mBq/g, respectively, while the accumulative inventories were 61.53-138.99 Bq/m(2) for Pu239+240 and 28.29-61.05 Bq/m(2) for Am-241. The convection-dispersion equation (CDE) was used to calculate the migration parameters of 239+240PU and higher apparent dispersion coefficients (D) were observed for the acidic forest soils compared with the alkaline grassland and desert soils; meanwhile a compartment model was employed to compare the migration of 239+240PU and Am-241 in successive soil layers which showed that the migration behaviors of 239+240PU and Am-241 were rather similar; both velocities were less than 0.3 cm/y in diverse types of soils and these findings were compatible with those of short-term laboratory simulation experiments in China. (C) 2018 Elsevier Ltd. All rights reserved.


英文关键词Plutonium Americium Global fallout CDE Compartment model
类型Article
语种英语
国家Peoples R China ; Japan
收录类别SCI-E
WOS记录号WOS:000447478100108
WOS关键词PU ISOTOPES ; VERTICAL MIGRATION ; FALLOUT PU-239+240 ; PLUTONIUM ISOTOPES ; GLOBAL FALLOUT ; CS-137 ; RADIONUCLIDES ; ASSOCIATION ; PU-238 ; SR-90
WOS类目Environmental Sciences
WOS研究方向Environmental Sciences & Ecology
来源机构北京大学
资源类型期刊论文
条目标识符http://119.78.100.177/qdio/handle/2XILL650/208400
作者单位1.Peking Univ, Sch Phys, State Key Lab Nucl Phys & Technol, Beijing 100871, Peoples R China;
2.China Acad Engn Phys, Inst Nucl Phys & Chem, Mianyang 621900, Peoples R China;
3.Natl Inst Quantum & Radiol Sci & Technol, Natl Inst Radiol Sci, Inage Ku, 4-9-1 Anagawa, Chiba 2638555, Japan;
4.Minist Environm Protect, Radiat Monitoring Tech Ctr, Hangzhou 310012, Zhejiang, Peoples R China
推荐引用方式
GB/T 7714
Ni, Youyi,Wang, Zhongtang,Guo, Qiuju,et al. Distinctive distributions and migrations of 239+240PU and Am-241 in Chinese forest, grassland and desert soils[J]. 北京大学,2018,212:1002-1009.
APA Ni, Youyi.,Wang, Zhongtang.,Guo, Qiuju.,Zheng, Jian.,Li, Sixuan.,...&Huang, Wenna.(2018).Distinctive distributions and migrations of 239+240PU and Am-241 in Chinese forest, grassland and desert soils.CHEMOSPHERE,212,1002-1009.
MLA Ni, Youyi,et al."Distinctive distributions and migrations of 239+240PU and Am-241 in Chinese forest, grassland and desert soils".CHEMOSPHERE 212(2018):1002-1009.
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