Knowledge Resource Center for Ecological Environment in Arid Area
DOI | 10.1016/j.atmosenv.2018.03.006 |
Chemical, optical and radiative characteristics of aerosols during haze episodes of winter in the North China Plain | |
Ding, Jing1; Zhang, Yufen1; Han, Suqin2; Xiao, Zhimei3; Wang, Jiao1; Feng, Yinchang1 | |
通讯作者 | Zhang, Yufen ; Han, Suqin |
来源期刊 | ATMOSPHERIC ENVIRONMENT
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ISSN | 1352-2310 |
EISSN | 1873-2844 |
出版年 | 2018 |
卷号 | 181页码:164-176 |
英文摘要 | Aerosol and water vapor radiative forcings, shortwave atmospheric heating rates and longwave atmospheric cooling rates were determined based on in situ physical and chemical measurements of aerosol, associated with the Mie theory and a radiative transfer model, LOWTRAN7, during the two haze episodes in the winter of 2013 in Tianjin, China. The aerosol types considered in LOWTRAN7 included rural, urban, marine, desert and custom aerosols. The default ratio of the absorption coefficient to the extinction coefficient for urban aerosol in LOWTRAN7 was approximately double of those found in this work, implying the weaker absorption ability of aerosols in the North China Plain (NCP). Moreover, the aerosol is assumed to be evenly distributed below 1 km of planetary boundary layer (PBL) on hazy days in LOWTRAN7. If the default urban aerosol optical properties and extinction profile in LOWTRAN7 is employed directly, a larger energy imbalance between the atmosphere and surface is generated and the warming effect of the aerosol is magnified. Hence, modified urban aerosol optical properties were established to replace the corresponding parameters’ database in LOWTRAN7. The aerosol extinction profiles were obtained based on a 255-m meteorological tower and observed results from the studies about Tianjin. In the NCP, the aerosol had little impact on atmospheric counter radiation. The water vapor is the crucial factor that affects atmospheric counter radiation. Both modified high shortwave heating rates and longwave cooling rates occur near the surface due to the abundance of aerosol and water vapor. The modified net atmospheric heating rate near the surface is 1.2 K d(-1) on hazy days and 0.3 K d(-1) on non-hazy days. Compared with the default urban aerosol optical properties and its vertical distribution in LOWTRAN7, the feedback effect of the modified urban aerosol on the boundary layer may not necessarily result in a stable lower atmosphere, but depends on the aerosol light absorption ability and its vertical distribution. |
英文关键词 | Aerosol Chemical components Optical properties Radiative forcing Heating rate |
类型 | Article |
语种 | 英语 |
国家 | Peoples R China |
收录类别 | SCI-E |
WOS记录号 | WOS:000430621500017 |
WOS关键词 | PLANETARY BOUNDARY-LAYER ; SINGLE-SCATTERING ALBEDO ; BLACK CARBON ; RELATIVE-HUMIDITY ; LIGHT-ABSORPTION ; AIR-POLLUTION ; SIZE DISTRIBUTIONS ; MIXING STATE ; URBAN ; EXTINCTION |
WOS类目 | Environmental Sciences ; Meteorology & Atmospheric Sciences |
WOS研究方向 | Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences |
资源类型 | 期刊论文 |
条目标识符 | http://119.78.100.177/qdio/handle/2XILL650/207926 |
作者单位 | 1.Nankai Univ, Coll Environm Sci & Engn, State Environm Protect Key Lab Urban Ambient Air, Tianjin 300071, Peoples R China; 2.Tianjin Inst Meteorol Sci, Tianjin, Peoples R China; 3.Tianjin Environm Monitoring Ctr, Tianjin, Peoples R China |
推荐引用方式 GB/T 7714 | Ding, Jing,Zhang, Yufen,Han, Suqin,et al. Chemical, optical and radiative characteristics of aerosols during haze episodes of winter in the North China Plain[J],2018,181:164-176. |
APA | Ding, Jing,Zhang, Yufen,Han, Suqin,Xiao, Zhimei,Wang, Jiao,&Feng, Yinchang.(2018).Chemical, optical and radiative characteristics of aerosols during haze episodes of winter in the North China Plain.ATMOSPHERIC ENVIRONMENT,181,164-176. |
MLA | Ding, Jing,et al."Chemical, optical and radiative characteristics of aerosols during haze episodes of winter in the North China Plain".ATMOSPHERIC ENVIRONMENT 181(2018):164-176. |
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