Arid
DOI10.1016/j.atmosenv.2018.03.006
Chemical, optical and radiative characteristics of aerosols during haze episodes of winter in the North China Plain
Ding, Jing1; Zhang, Yufen1; Han, Suqin2; Xiao, Zhimei3; Wang, Jiao1; Feng, Yinchang1
通讯作者Zhang, Yufen ; Han, Suqin
来源期刊ATMOSPHERIC ENVIRONMENT
ISSN1352-2310
EISSN1873-2844
出版年2018
卷号181页码:164-176
英文摘要

Aerosol and water vapor radiative forcings, shortwave atmospheric heating rates and longwave atmospheric cooling rates were determined based on in situ physical and chemical measurements of aerosol, associated with the Mie theory and a radiative transfer model, LOWTRAN7, during the two haze episodes in the winter of 2013 in Tianjin, China. The aerosol types considered in LOWTRAN7 included rural, urban, marine, desert and custom aerosols. The default ratio of the absorption coefficient to the extinction coefficient for urban aerosol in LOWTRAN7 was approximately double of those found in this work, implying the weaker absorption ability of aerosols in the North China Plain (NCP). Moreover, the aerosol is assumed to be evenly distributed below 1 km of planetary boundary layer (PBL) on hazy days in LOWTRAN7. If the default urban aerosol optical properties and extinction profile in LOWTRAN7 is employed directly, a larger energy imbalance between the atmosphere and surface is generated and the warming effect of the aerosol is magnified. Hence, modified urban aerosol optical properties were established to replace the corresponding parameters’ database in LOWTRAN7. The aerosol extinction profiles were obtained based on a 255-m meteorological tower and observed results from the studies about Tianjin. In the NCP, the aerosol had little impact on atmospheric counter radiation. The water vapor is the crucial factor that affects atmospheric counter radiation. Both modified high shortwave heating rates and longwave cooling rates occur near the surface due to the abundance of aerosol and water vapor. The modified net atmospheric heating rate near the surface is 1.2 K d(-1) on hazy days and 0.3 K d(-1) on non-hazy days. Compared with the default urban aerosol optical properties and its vertical distribution in LOWTRAN7, the feedback effect of the modified urban aerosol on the boundary layer may not necessarily result in a stable lower atmosphere, but depends on the aerosol light absorption ability and its vertical distribution.


英文关键词Aerosol Chemical components Optical properties Radiative forcing Heating rate
类型Article
语种英语
国家Peoples R China
收录类别SCI-E
WOS记录号WOS:000430621500017
WOS关键词PLANETARY BOUNDARY-LAYER ; SINGLE-SCATTERING ALBEDO ; BLACK CARBON ; RELATIVE-HUMIDITY ; LIGHT-ABSORPTION ; AIR-POLLUTION ; SIZE DISTRIBUTIONS ; MIXING STATE ; URBAN ; EXTINCTION
WOS类目Environmental Sciences ; Meteorology & Atmospheric Sciences
WOS研究方向Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
资源类型期刊论文
条目标识符http://119.78.100.177/qdio/handle/2XILL650/207926
作者单位1.Nankai Univ, Coll Environm Sci & Engn, State Environm Protect Key Lab Urban Ambient Air, Tianjin 300071, Peoples R China;
2.Tianjin Inst Meteorol Sci, Tianjin, Peoples R China;
3.Tianjin Environm Monitoring Ctr, Tianjin, Peoples R China
推荐引用方式
GB/T 7714
Ding, Jing,Zhang, Yufen,Han, Suqin,et al. Chemical, optical and radiative characteristics of aerosols during haze episodes of winter in the North China Plain[J],2018,181:164-176.
APA Ding, Jing,Zhang, Yufen,Han, Suqin,Xiao, Zhimei,Wang, Jiao,&Feng, Yinchang.(2018).Chemical, optical and radiative characteristics of aerosols during haze episodes of winter in the North China Plain.ATMOSPHERIC ENVIRONMENT,181,164-176.
MLA Ding, Jing,et al."Chemical, optical and radiative characteristics of aerosols during haze episodes of winter in the North China Plain".ATMOSPHERIC ENVIRONMENT 181(2018):164-176.
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