Arid
DOI10.5194/acp-18-7237-2018
Competition for water vapour results in suppression of ice formation in mixed-phase clouds
Simpson, Emma L.; Connolly, Paul J.; McFiggans, Gordon
通讯作者McFiggans, Gordon
来源期刊ATMOSPHERIC CHEMISTRY AND PHYSICS
ISSN1680-7316
EISSN1680-7324
出版年2018
卷号18期号:10页码:7237-7250
英文摘要

The formation of ice in clouds can initiate precipitation and influence a cloud’s reflectivity and lifetime, affecting climate to a highly uncertain degree. Nucleation of ice at elevated temperatures requires an ice nucleating particle (INP), which results in so-called heterogeneous freezing. Previously reported measurements for the ability of a particle to nucleate ice have been made in the absence of other aerosol which will act as cloud condensation nuclei (CCN) and are ubiquitous in the atmosphere. Here we show that CCN can "outcompete" INPs for available water vapour thus suppressing ice formation, which has the potential to significantly affect the Earth’s radiation budget. The magnitude of this suppression is shown to be dependent on the mass of condensed water required for freezing. Here we show that ice formation in a state-of-the-art cloud parcel model is strongly dependent on the criteria for heterogeneous freezing selected from those previously hypothesised. We have developed an alternative criteria which agrees well with observations from cloud chamber experiments. This study demonstrates the dominant role that competition for water vapour can play in ice formation, highlighting both a need for clarity in the requirements for heterogeneous freezing and for measurements under atmospherically appropriate conditions.


类型Article
语种英语
国家England
收录类别SCI-E
WOS记录号WOS:000433159600002
WOS关键词ADSORPTION ACTIVATION ; INSOLUBLE PARTICLES ; STRATIFORM CLOUDS ; DROPLET FORMATION ; DUST SAMPLES ; DESERT DUST ; PART 1 ; NUCLEATION ; PARAMETERIZATION ; IMMERSION
WOS类目Environmental Sciences ; Meteorology & Atmospheric Sciences
WOS研究方向Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
资源类型期刊论文
条目标识符http://119.78.100.177/qdio/handle/2XILL650/207889
作者单位Univ Manchester, Ctr Atmospher Sci, Sch Earth & Environm Sci, Manchester M13 9PL, Lancs, England
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GB/T 7714
Simpson, Emma L.,Connolly, Paul J.,McFiggans, Gordon. Competition for water vapour results in suppression of ice formation in mixed-phase clouds[J],2018,18(10):7237-7250.
APA Simpson, Emma L.,Connolly, Paul J.,&McFiggans, Gordon.(2018).Competition for water vapour results in suppression of ice formation in mixed-phase clouds.ATMOSPHERIC CHEMISTRY AND PHYSICS,18(10),7237-7250.
MLA Simpson, Emma L.,et al."Competition for water vapour results in suppression of ice formation in mixed-phase clouds".ATMOSPHERIC CHEMISTRY AND PHYSICS 18.10(2018):7237-7250.
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