Knowledge Resource Center for Ecological Environment in Arid Area
DOI | 10.5194/acp-18-7237-2018 |
Competition for water vapour results in suppression of ice formation in mixed-phase clouds | |
Simpson, Emma L.; Connolly, Paul J.; McFiggans, Gordon | |
通讯作者 | McFiggans, Gordon |
来源期刊 | ATMOSPHERIC CHEMISTRY AND PHYSICS
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ISSN | 1680-7316 |
EISSN | 1680-7324 |
出版年 | 2018 |
卷号 | 18期号:10页码:7237-7250 |
英文摘要 | The formation of ice in clouds can initiate precipitation and influence a cloud’s reflectivity and lifetime, affecting climate to a highly uncertain degree. Nucleation of ice at elevated temperatures requires an ice nucleating particle (INP), which results in so-called heterogeneous freezing. Previously reported measurements for the ability of a particle to nucleate ice have been made in the absence of other aerosol which will act as cloud condensation nuclei (CCN) and are ubiquitous in the atmosphere. Here we show that CCN can "outcompete" INPs for available water vapour thus suppressing ice formation, which has the potential to significantly affect the Earth’s radiation budget. The magnitude of this suppression is shown to be dependent on the mass of condensed water required for freezing. Here we show that ice formation in a state-of-the-art cloud parcel model is strongly dependent on the criteria for heterogeneous freezing selected from those previously hypothesised. We have developed an alternative criteria which agrees well with observations from cloud chamber experiments. This study demonstrates the dominant role that competition for water vapour can play in ice formation, highlighting both a need for clarity in the requirements for heterogeneous freezing and for measurements under atmospherically appropriate conditions. |
类型 | Article |
语种 | 英语 |
国家 | England |
收录类别 | SCI-E |
WOS记录号 | WOS:000433159600002 |
WOS关键词 | ADSORPTION ACTIVATION ; INSOLUBLE PARTICLES ; STRATIFORM CLOUDS ; DROPLET FORMATION ; DUST SAMPLES ; DESERT DUST ; PART 1 ; NUCLEATION ; PARAMETERIZATION ; IMMERSION |
WOS类目 | Environmental Sciences ; Meteorology & Atmospheric Sciences |
WOS研究方向 | Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences |
资源类型 | 期刊论文 |
条目标识符 | http://119.78.100.177/qdio/handle/2XILL650/207889 |
作者单位 | Univ Manchester, Ctr Atmospher Sci, Sch Earth & Environm Sci, Manchester M13 9PL, Lancs, England |
推荐引用方式 GB/T 7714 | Simpson, Emma L.,Connolly, Paul J.,McFiggans, Gordon. Competition for water vapour results in suppression of ice formation in mixed-phase clouds[J],2018,18(10):7237-7250. |
APA | Simpson, Emma L.,Connolly, Paul J.,&McFiggans, Gordon.(2018).Competition for water vapour results in suppression of ice formation in mixed-phase clouds.ATMOSPHERIC CHEMISTRY AND PHYSICS,18(10),7237-7250. |
MLA | Simpson, Emma L.,et al."Competition for water vapour results in suppression of ice formation in mixed-phase clouds".ATMOSPHERIC CHEMISTRY AND PHYSICS 18.10(2018):7237-7250. |
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