Arid
DOI10.5194/acp-18-5371-2018
Vertical distribution of aerosol optical properties in the Po Valley during the 2012 summer campaigns
Bucci, Silvia1,2; Cristofanelli, Paolo3; Decesari, Stefano3; Marinoni, Angela3; Sandrini, Silvia3; Groess, Johannes4; Wiedensohler, Alfred4; Di Marco, Chiara F.5; Nemitz, Eiko5; Cairo, Francesco1; Di Liberto, Luca1; Fierli, Federico1
通讯作者Bucci, Silvia ; Fierli, Federico
来源期刊ATMOSPHERIC CHEMISTRY AND PHYSICS
ISSN1680-7316
EISSN1680-7324
出版年2018
卷号18期号:8页码:5371-5389
英文摘要

Studying the vertical distribution of aerosol particle physical and chemical properties in the troposphere is essential to understand the relative importance of local emission processes vs. long-range transport for column-integrated aerosol properties (e.g. the aerosol optical depth, AOD, affecting regional climate) as well as for the aerosol burden and its impacts on air quality at the ground. The main objective of this paper is to investigate the transport of desert dust in the middle troposphere and its intrusion into the planetary boundary layer (PBL) over the Po Valley (Italy), a region considered one of the greatest European pollution hotspots for the frequency that particulate matter (PM) limit values are exceeded. Events of mineral aerosol uplift from local (soil) sources and phenomena of hygroscopic growth at the ground are also investigated, possibly affecting the PM concentration in the region as well. During the PEGASOS 2012 field campaign, an integrated observing-modelling system was set up based on near-surface measurements (particle concentration and chemistry), vertical profiling (backscatter coefficient profiles from lidar and radiosoundings) and Lagrangian air mass transport simulations by FLEXPART model. Measurements were taken at the San Pietro Capofiume supersite (44 degrees 39’ N, 11 degrees 37’ E; 11 m a.s.l.), located in a rural area relatively close to some major urban and industrial emissive areas in the Po Valley. Mt. Cimone (44 degrees 12’ N, 10 degrees 42’ E; 2165 m a.s.l.) WMO/GAW station observations are also included in the study to characterize regional-scale variability. Results show that, in the Po Valley, aerosol is detected mainly below 2000 m a.s.l. with a prevalent occurrence of non-depolarizing particles (> 50 % throughout the campaign) and a vertical distribution modulated by the PBL daily evolution. Two intense events of mineral dust transport from northern Africa (19-21 and 29 June to 2 July) are observed, with layers advected mainly above 2000 m, but subsequently sinking and mixing in the PBL. As a consequence, a non-negligible occurrence of mineral dust is observed close to the ground (similar to 7 % of occurrence during a 1-month campaign). The observations unambiguously show Saharan dust layers intruding the Po Valley mixing layer and directly affecting the aerosol concentrations near the surface. Finally, lidar observations also indicate strong variability in aerosol on shorter timescales (hourly). Firstly, these highlight events of hygroscopic growth of anthropogenic aerosol, visible as shallow layers of low depolarization near the ground. Such events are identified during early morning hours at high relative humidity (RH) conditions (RH > 80 %). The process is observed concurrently with high PM1 nitrate concentration (up to 15 mu g cm(-3)) and hence mainly explicable by deliquescence of fine anthropogenic particles, and during mineral dust intrusion episodes, when water condensation on dust particles could instead represent the dominant contribution. Secondly, lidar images show frequent events (mean daily occurrence of similar to 22 % during the whole campaign) of rapid uplift of mineral depolarizing particles in afternoon- evening hours up to 2000 m a.s.l. height. The origin of such particles cannot be directly related to long-range transport events, being instead likely linked to processes of soil particle resuspension from agricultural lands.


类型Article
语种英语
国家Italy ; Germany ; Scotland
收录类别SCI-E
WOS记录号WOS:000430492800002
WOS关键词2165 M A.S.L. ; SAHARAN DUST ; MT.-CIMONE ; CHEMICAL-COMPOSITION ; MEDITERRANEAN BASIN ; LIDAR OBSERVATIONS ; SATELLITE-OBSERVATIONS ; DEPOLARIZATION RATIO ; FREE TROPOSPHERE ; RAMAN LIDAR
WOS类目Environmental Sciences ; Meteorology & Atmospheric Sciences
WOS研究方向Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
资源类型期刊论文
条目标识符http://119.78.100.177/qdio/handle/2XILL650/207885
作者单位1.CNR, ISAC, Natl Res Council, Inst Atmospher Sci & Climate, Rome, Italy;
2.Ferrara Univ, Sc Dept Phys, Ferrara, Italy;
3.CNR, ISAC, Natl Res Council, Inst Atmospher Sci & Climate, Bologna, Italy;
4.Leibniz Inst Tropospher Res, Leipzig, Germany;
5.NERC, Ctr Ecol & Hydrol, Penicuik, Midlothian, Scotland
推荐引用方式
GB/T 7714
Bucci, Silvia,Cristofanelli, Paolo,Decesari, Stefano,et al. Vertical distribution of aerosol optical properties in the Po Valley during the 2012 summer campaigns[J],2018,18(8):5371-5389.
APA Bucci, Silvia.,Cristofanelli, Paolo.,Decesari, Stefano.,Marinoni, Angela.,Sandrini, Silvia.,...&Fierli, Federico.(2018).Vertical distribution of aerosol optical properties in the Po Valley during the 2012 summer campaigns.ATMOSPHERIC CHEMISTRY AND PHYSICS,18(8),5371-5389.
MLA Bucci, Silvia,et al."Vertical distribution of aerosol optical properties in the Po Valley during the 2012 summer campaigns".ATMOSPHERIC CHEMISTRY AND PHYSICS 18.8(2018):5371-5389.
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