Arid
DOI10.1007/s11869-018-0549-5
Ambient PM10 impacts brought by the extreme flooding event of March 24-26, 2015, in Copiapo, Chile
Jorquera, Hector1; Maria Villalobos, Ana1; Barraza, Francisco2
通讯作者Jorquera, Hector
来源期刊AIR QUALITY ATMOSPHERE AND HEALTH
ISSN1873-9318
EISSN1873-9326
出版年2018
卷号11期号:3页码:341-351
英文摘要

On March 24-26, 2015, the Chilean city of Copiapo (27 degrees 22’ S, 70 degrees 20’ W), located in the hyperarid Atacama Desert, suffered an intense flooding brought by an extreme, unique rainfall event with a 35-year record of daily precipitation. A receptor model (positive matrix factorization, version 5) analysis, applied to ambient PM10 chemical speciation from three short-term sampling campaigns, resolved four sources: crustal/road dust, sea salt, secondary sulfates, and emissions from Paipote copper smelter located 8 km east of Copiapo. Wind trajectories computed with US NOAA’s Hybrid Single-Particle Lagrangian Integrated Trajectory model (HYSPLIT) supported the above source identification and explained variability in source contributions. It was found that crustal/road dust increased 50 mu g/m(3), in April 8-10, 2015, as compared with values in November 2014 and October-November 2015, respectively. This was the dominant PM10 source after the flooding and before debris were cleaned up, being on order of magnitude higher that the other source contributions. The Paipote copper smelter contributed with primary PM10 emissions and secondary sulfates; this combined contribution averaged 11.8 mu g/m(3). Sea salt contributions contributed an average of 3.3 mu g/m(3). In normal conditions, crustal/road dust averaged 2.9 mu g/m(3), but the other resolved sources also contributed with crustal elements as their emissions are transported by winds to Copiapo. The positive matrix factorization solution included an unresolved concentration of 7.4 mu g/m(3). The small number of samples and the lack of measurements of nitrate, ammonia, and organic and elemental carbon may explain this result. Hence, sources such as secondary nitrates and combustion sources plus fugitive dust from sources surrounding Copiapo might be included in that unresolved concentration.


英文关键词Source apportionment Copper smelter Atacama Desert Flooding event Sustainable urban development Suspended soil dust
类型Article
语种英语
国家Chile
收录类别SCI-E
WOS记录号WOS:000430849900009
WOS关键词POSITIVE MATRIX FACTORIZATION ; SOURCE APPORTIONMENT ; RECEPTOR MODELS ; NORTHERN CHILE ; PM2.5 ; REGION ; SITES
WOS类目Environmental Sciences
WOS研究方向Environmental Sciences & Ecology
资源类型期刊论文
条目标识符http://119.78.100.177/qdio/handle/2XILL650/207466
作者单位1.Pontificia Univ Catolica Chile, Dept Ingn Quim & Bioproc, Vicuna Mackenna 4860, Santiago 7820436, Chile;
2.Pontificia Univ Catolica Chile, Inst Geog, Vicuna Mackenna 4860, Santiago 7820436, Chile
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Jorquera, Hector,Maria Villalobos, Ana,Barraza, Francisco. Ambient PM10 impacts brought by the extreme flooding event of March 24-26, 2015, in Copiapo, Chile[J],2018,11(3):341-351.
APA Jorquera, Hector,Maria Villalobos, Ana,&Barraza, Francisco.(2018).Ambient PM10 impacts brought by the extreme flooding event of March 24-26, 2015, in Copiapo, Chile.AIR QUALITY ATMOSPHERE AND HEALTH,11(3),341-351.
MLA Jorquera, Hector,et al."Ambient PM10 impacts brought by the extreme flooding event of March 24-26, 2015, in Copiapo, Chile".AIR QUALITY ATMOSPHERE AND HEALTH 11.3(2018):341-351.
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