Knowledge Resource Center for Ecological Environment in Arid Area
DOI | 10.1039/c7cp04898j |
The role of phase separation and related topography in the exceptional ice-nucleating ability of alkali feldspars | |
Whale, Thomas F.1; Holden, Mark A.1,2; Kulak, Alexander N.2; Kim, Yi-Yeoun2; Meldrum, Fiona C.2; Christenson, Hugo K.3; Murray, Benjamin J.1 | |
通讯作者 | Whale, Thomas F. |
来源期刊 | PHYSICAL CHEMISTRY CHEMICAL PHYSICS
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ISSN | 1463-9076 |
EISSN | 1463-9084 |
出版年 | 2017 |
卷号 | 19期号:46页码:31186-31193 |
英文摘要 | Our understanding of crystal nucleation is a limiting factor in many fields, not least in the atmospheric sciences. It was recently found that feldspar, a component of airborne desert dust, plays a dominant role in triggering ice formation in clouds, but the origin of this effect was unclear. By investigating the structure/property relationships of a wide range of feldspars, we demonstrate that alkali feldspars with certain microtextures, related to phase separation into Na and K-rich regions, show exceptional icenucleating abilities in supercooled water. We found no correlation between ice-nucleating efficiency and the crystal structures or the chemical compositions of these active feldspars, which suggests that specific topographical features associated with these microtextures are key in the activity of these feldspars. That topography likely acts to promote ice nucleation, improves our understanding of ice formation in clouds, and may also enable the design and manufacture of bespoke nucleating materials for uses such as cloud seeding and cryopreservation. |
类型 | Article |
语种 | 英语 |
国家 | England |
收录类别 | SCI-E |
WOS记录号 | WOS:000416425400020 |
WOS关键词 | CRYSTAL NUCLEATION ; IMMERSION MODE ; ACTIVE-SITES ; HETEROGENEOUS NUCLEATION ; ATMOSPHERIC PARTICLES ; SURFACE-ROUGHNESS ; ORGANIC-CRYSTALS ; K-RICH ; CRYSTALLIZATION ; AEROSOLS |
WOS类目 | Chemistry, Physical ; Physics, Atomic, Molecular & Chemical |
WOS研究方向 | Chemistry ; Physics |
资源类型 | 期刊论文 |
条目标识符 | http://119.78.100.177/qdio/handle/2XILL650/201448 |
作者单位 | 1.Univ Leeds, Sch Earth & Environm, Leeds LS2 9JT, W Yorkshire, England; 2.Univ Leeds, Sch Chem, Leeds LS2 9JT, W Yorkshire, England; 3.Univ Leeds, Sch Phys & Astron, Leeds LS2 9JT, W Yorkshire, England |
推荐引用方式 GB/T 7714 | Whale, Thomas F.,Holden, Mark A.,Kulak, Alexander N.,et al. The role of phase separation and related topography in the exceptional ice-nucleating ability of alkali feldspars[J],2017,19(46):31186-31193. |
APA | Whale, Thomas F..,Holden, Mark A..,Kulak, Alexander N..,Kim, Yi-Yeoun.,Meldrum, Fiona C..,...&Murray, Benjamin J..(2017).The role of phase separation and related topography in the exceptional ice-nucleating ability of alkali feldspars.PHYSICAL CHEMISTRY CHEMICAL PHYSICS,19(46),31186-31193. |
MLA | Whale, Thomas F.,et al."The role of phase separation and related topography in the exceptional ice-nucleating ability of alkali feldspars".PHYSICAL CHEMISTRY CHEMICAL PHYSICS 19.46(2017):31186-31193. |
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