Arid
DOI10.1016/j.atmosenv.2017.03.048
Observations of trace gases, photolysis rate coefficients and model simulations over semi-arid region, India
Lingaswamy, A. P.1,2,3; Arafath, S. Md1; Balakrishnaiah, G.1; Gopal, K. Rama1; Reddy, N. Siva Kumar1; Reddy, K. Raja Obul1; Reddy, R. R.1; Rao, T. Chakradhar1
通讯作者Gopal, K. Rama
来源期刊ATMOSPHERIC ENVIRONMENT
ISSN1352-2310
EISSN1873-2844
出版年2017
卷号158页码:246-258
英文摘要

Continuous groutid-based measurements of CO, SO2 and NO2 were carried out in a semi-arid rural area, Anantapur [14.62 N-0, 77.65 E-0], Southern India, for the period January 2012 December 2012. The maximum CO concentration was observed in winter (310 +/- 17 ppbv) followed by summer (180 +/- 21 ppbv) and post monsoon (174 +/- 20 ppbv), while the minimum in monsoon (72 +/- 9 ppbv). Seasonal mean NO2/NOx ratios for monsoon, post monsoon, winter and summer were about 0.88, 0.91, 0.76 and 0.80 respectively, indicating a higher conversion of NO to NO2 over the measurement site. Monthly mean low SO2 mixing ratio was found (0.46 +/- 0.02 ppbv) in monsoon and high (2.42 +/- 0.21 ppbv) in winter. Keeping the emissions aside, the levels of CO, SO2 and NO2 were influenced by meteorology, urban effects and trans-boundary transport in the lower troposphere. Atmospheric boundary layer (ABL) had the good correlation coefficient (R = 0.76) with solar radiation during daytime, while it was mainly correlated with wind speed during night time (R = 0.42). Diurnal trend of atmospheric visibility was found to be maximum during noon times at around (14:00-16:00 h) about 76 k.m. and minimum during morning periods (06:00-08:00 h) about 45 k.m. A strong positive correlation was observed between BC and CO (R = 0.71) with an average slope, suggesting common or proximate sources likely to be traffic emissions contribution for the production of BC and CO. The SO2/NOx and CO/NOx study were strongly suggested that mobile sources were larger contributors over the site and the evidence of transport of emissions from other surrounding regions. Tropospheric Ultraviolet Visible (TUV) radiative transfer model was used to calculate the Photolysis rate coefficients (J(O-3), J(NO2)). Chemical box model (NCAR-MM) was used to simulate diurnal variation of CO and the results were reported. (C) 2017 Elsevier Ltd. All rights reserved.


英文关键词Trace gases Source approximation Visibility Photolysis rate coefficients Radiative transfer model
类型Article
语种英语
国家India ; Peoples R China
收录类别SCI-E
WOS记录号WOS:000401207900023
WOS关键词AEROSOL OPTICAL-PROPERTIES ; IN-SITU MEASUREMENTS ; SURFACE OZONE ; BLACK CARBON ; AIR-QUALITY ; URBAN SITE ; SEASONAL-VARIATIONS ; ANANTAPUR ; PRECURSORS ; POLLUTANTS
WOS类目Environmental Sciences ; Meteorology & Atmospheric Sciences
WOS研究方向Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
资源类型期刊论文
条目标识符http://119.78.100.177/qdio/handle/2XILL650/197657
作者单位1.Sri Krishnadevaraya Univ, Dept Phys, Aerosol & Atmospher Res Lab, Anantapur 515003, Andhra Pradesh, India;
2.Rayalaseema Univ, Dept Phys, Kurnool 518007, Andhra Pradesh, India;
3.Shandong Univ, Environm Res Inst, Jinan 250100, Peoples R China
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Lingaswamy, A. P.,Arafath, S. Md,Balakrishnaiah, G.,et al. Observations of trace gases, photolysis rate coefficients and model simulations over semi-arid region, India[J],2017,158:246-258.
APA Lingaswamy, A. P..,Arafath, S. Md.,Balakrishnaiah, G..,Gopal, K. Rama.,Reddy, N. Siva Kumar.,...&Rao, T. Chakradhar.(2017).Observations of trace gases, photolysis rate coefficients and model simulations over semi-arid region, India.ATMOSPHERIC ENVIRONMENT,158,246-258.
MLA Lingaswamy, A. P.,et al."Observations of trace gases, photolysis rate coefficients and model simulations over semi-arid region, India".ATMOSPHERIC ENVIRONMENT 158(2017):246-258.
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