Arid
DOI10.1016/j.jenvrad.2016.03.005
Investigation of uranium geochemistry along groundwater flow path in the Continental Intercalaire aquifer (Southern Tunisia)
Dhaoui, Z.1; Chkir, N.2; Zouari, K.1; Ammar, F. Hadj1; Agoune, A.3
通讯作者Dhaoui, Z.
来源期刊JOURNAL OF ENVIRONMENTAL RADIOACTIVITY
ISSN0265-931X
EISSN1879-1700
出版年2016
卷号157页码:67-76
英文摘要

Environmental tracers (H-2, O-18, isotopes of Uranium) and geochemical processes occurring within groundwaters from the Continental Intercalaire (CI) in Southern Tunisia were used to understand the hydrodynamics and the recharge conditions of this aquifer. This study investigates the chemical and isotopic compositions of the CI groundwater. The water types are dominated by Na+, SO42-, Cl- throughout most of the basin with a general increase in total dissolved solids from the Saharan Platform margins towards the Chotts region. Large scale groundwater flow paths are toward the Chotts region. The stable isotopes composition of the analyzed groundwater ranges from -8.8 to -6 parts per thousand vs V-SMOW for delta O-18 and from -67 to -40 parts per thousand vs V-SMOW for delta H-2. The relatively enriched stable isotopes contents suggest the contribution of the Dahar sandstones outcrops in the current recharge of the CI aquifer in an arid context. However, the most depleted values in heavy isotopes indicate a paleorecharge of the aquifer under wetter conditions revealing a long residence time of groundwaters. The results from water samples using alpha spectrometry method indicate a range in U-238 concentrations and U-234/U-238 activity ratios (AR) of 0.044-1.285 mu g kg(-1) and 1.2 to 8.84 respectively. The geochemistry of uranium isotopes in groundwater is controlled by many factors, essentially, the influence of water rock interactions, the preferential dissolution of U-234 relative to U-238 due to alpha recoil and the mixing processes between different waters with distinct AR as well as U-238 concentrations. (C) 2016 Elsevier Ltd. All rights reserved.


英文关键词Continental Intercalaire Geochemistry Uranium Activity ratios
类型Article
语种英语
国家Tunisia
收录类别SCI-E
WOS记录号WOS:000375811700008
WOS关键词ELECTRODEPOSITION ; EVOLUTION
WOS类目Environmental Sciences
WOS研究方向Environmental Sciences & Ecology
资源类型期刊论文
条目标识符http://119.78.100.177/qdio/handle/2XILL650/194370
作者单位1.Natl Sch Engn Sfax, Dept Geol, Lab Radioanal & Environm, Route Soukra,BP 1173, Sfax 3038, Tunisia;
2.Fac Letters & Humanities, Dept Geog, Lab Radioanal & Environm, Route El Matar,BP 1168, Sfax 3029, Tunisia;
3.CRDA, De Kebili, Tunisia
推荐引用方式
GB/T 7714
Dhaoui, Z.,Chkir, N.,Zouari, K.,et al. Investigation of uranium geochemistry along groundwater flow path in the Continental Intercalaire aquifer (Southern Tunisia)[J],2016,157:67-76.
APA Dhaoui, Z.,Chkir, N.,Zouari, K.,Ammar, F. Hadj,&Agoune, A..(2016).Investigation of uranium geochemistry along groundwater flow path in the Continental Intercalaire aquifer (Southern Tunisia).JOURNAL OF ENVIRONMENTAL RADIOACTIVITY,157,67-76.
MLA Dhaoui, Z.,et al."Investigation of uranium geochemistry along groundwater flow path in the Continental Intercalaire aquifer (Southern Tunisia)".JOURNAL OF ENVIRONMENTAL RADIOACTIVITY 157(2016):67-76.
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