Arid
DOI10.1016/j.jclepro.2015.04.054
Comparative analysis of chemical composition and sources of aerosol particles in urban Beijing during clear, hazy, and dusty days using single particle aerosol mass spectrometry
Ma, Li1; Li, Mei1; Zhang, Hefeng2; Li, Lei1; Huang, Zhengxu1; Gao, Wei1; Chen, Duohong3; Fu, Zhong4; Nian, Huiqing5; Zou, Lilin5; Gao, Jian2; Chai, Fahe2; Zhou, Zhen1
通讯作者Zhou, Zhen
来源期刊JOURNAL OF CLEANER PRODUCTION
ISSN0959-6526
EISSN1879-1786
出版年2016
卷号112页码:1319-1329
英文摘要

A single particle aerosol mass spectrometer (SPAMS) was employed to characterize the particles in urban Beijing in the spring of 2011. The whole sampling time was divided into clear, hazy, and dusty day periods. Based on SPAMS results, the chemical composition of size-resolved particles in five major classes, including K-rich, carbonaceous, industry metal, dust, and Na-rich particles, and their corresponding sources were compared during clear, hazy, and dusty days. Air mass back trajectories are used to identify likely source regions for each period. Under stagnant meteorological conditions, local and regional emissions are a key factor in haze formation. K-rich and carbonaceous particles dominated under all conditions (25-54%), with higher contributions (23% and 29%) from industrial metal particles during hazy days, which could be attributed to the emission of biomass burning, coal combustion, and vehicle exhaust during all periods, whereas industrial metal processes are also a likely source for K-rich particles during hazy days. The aging of particles was observed over the whole sampling period, as evidenced by the presence of secondary species in all particle classes. Industrial metal particles possibly originate from industrial metal processes, vehicle exhaust, and coal combustion etc, while road and soil dust is also a possible source during dusty days. Dust particles increased greatly (17%) in a dust storm event with a coarse mode distribution, which are mainly associated with the mineral dust from deserted regions, whereas they could originate from local dust and coal combustion during non-dusty days. Last, Na-rich particles are mainly associated with industrial metal particles, coal, and fuel combustion during hazy days, and mineral dust during dusty days, respectively. Sea salt is a possible source of Na-rich particles under all conditions. Our analysis could shed a light on the understanding of the different source apportionment of aerosol particles under different meteorology/pollution conditions. (C) 2015 Elsevier Ltd. All rights reserved.


英文关键词Dust Haze Single particle Chemical composition Source Mass spectrometry
类型Article
语种英语
国家Peoples R China
收录类别SCI-E
WOS记录号WOS:000368206800007
WOS关键词PARTICULATE AIR-POLLUTION ; MIXING STATE ; SOURCE APPORTIONMENT ; ORGANIC AEROSOL ; BLOOD-PRESSURE ; BLACK CARBON ; MEXICO-CITY ; SOIL DUST ; SIZE ; LEAD
WOS类目Green & Sustainable Science & Technology ; Engineering, Environmental ; Environmental Sciences
WOS研究方向Science & Technology - Other Topics ; Engineering ; Environmental Sciences & Ecology
资源类型期刊论文
条目标识符http://119.78.100.177/qdio/handle/2XILL650/194289
作者单位1.Jinan Univ, Inst Atmospher Environm Safety & Pollut Control, Jinan 510632, Guangdong, Peoples R China;
2.Chinese Res Inst Environm Sci, State Key Lab Environm Criteria & Risk Assessment, Beijing 100012, Peoples R China;
3.Guangdong Environm Monitoring Ctr, State Environm Protect Key Lab Reg Air Qual Monit, Guangzhou 510308, Guangdong, Peoples R China;
4.Shanghai Univ, Sch Environm & Chem Engn, Shanghai 200444, Peoples R China;
5.Guangzhou Hexin Analyt Instrument Co Ltd, Guangzhou 510530, Guangdong, Peoples R China
推荐引用方式
GB/T 7714
Ma, Li,Li, Mei,Zhang, Hefeng,et al. Comparative analysis of chemical composition and sources of aerosol particles in urban Beijing during clear, hazy, and dusty days using single particle aerosol mass spectrometry[J],2016,112:1319-1329.
APA Ma, Li.,Li, Mei.,Zhang, Hefeng.,Li, Lei.,Huang, Zhengxu.,...&Zhou, Zhen.(2016).Comparative analysis of chemical composition and sources of aerosol particles in urban Beijing during clear, hazy, and dusty days using single particle aerosol mass spectrometry.JOURNAL OF CLEANER PRODUCTION,112,1319-1329.
MLA Ma, Li,et al."Comparative analysis of chemical composition and sources of aerosol particles in urban Beijing during clear, hazy, and dusty days using single particle aerosol mass spectrometry".JOURNAL OF CLEANER PRODUCTION 112(2016):1319-1329.
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