Arid
DOI10.1016/j.chemosphere.2016.04.110
Influence of long-range atmospheric transportation (LRAT) on mono- to octa-chlorinated PCDD/Fs levels and distributions in soil around Qinghai Lake, China
Han, Ying1,2; Liu, Wenbin1,2; Hansen, Hans Chr. Bruun3; Chen, Xuebin1,2; Liao, Xiao1,2; Li, Haifeng1,2; Wang, Mengjing1,2; Yan, Nan1,2
通讯作者Liu, Wenbin
来源期刊CHEMOSPHERE
ISSN0045-6535
EISSN1879-1298
出版年2016
卷号156页码:143-149
英文摘要

Long-range atmospheric transportation (LRAT) of persistent organic pollutants followed by their deposition in cold, arid regions is of wide concern. This problem occurs at Qinghai Lake in the northeastern Tibetan Plateau, a sparsely populated area with extreme weather conditions and little current or historical anthropogenic pollution. The concentrations and distribution patterns of the mono-to octachlorinated dibenzo-p-dioxin and dibenzofuran (PCDD/F) congeners in surface soil samples collected from around Qinghai Lake were quantified. Concentration differences between low-(mono-to tri-) chlorinated PCDD/Fs and high-(tetra-to octa-) chlorinated PCDD/Fs were measured. High PCDD/F levels were detected, with total concentrations of 15,108 +/- 6323 pg/g for the 27 PCDD/F congeners and 15,104 +/- 6324 pg/g for the low-chlorinated PCDD/Fs. The concentrations of 17 2,3,7,8-substituted PCDD/Fs were only 3.1 +/- 4.4 pg/g and the corresponding international toxicity equivalency (I-TEQ) was 0.11 +/- 0.22 pg I-TEQ/g. Given their higher vapor pressures and lower boiling points, low-chlorinated PCDD/Fs, were predominantly gaseous, whereas high-chlorinated PCDD/Fs were predominantly solid, indicating that there is a higher potential for long-range transport of low-chlorinated PCDD/Fs. Overall, because of their high LRAT potential, low-chlorinated PCDD/Fs may pose a greater risk to local ecosystems in cold, remote areas than high-chlorinated PCDD/Fs. (C) 2016 Elsevier Ltd. All rights reserved.


英文关键词Qinghai Lake Chlorinated PCDD/F Distribution characteristic Remote area Cold region
类型Article
语种英语
国家Peoples R China ; Denmark
收录类别SCI-E
WOS记录号WOS:000377732700018
WOS关键词DIBENZO-P-DIOXINS ; TIBETAN PLATEAU ; WASTE INCINERATOR ; LOW-TEMPERATURE ; FLY-ASH ; PCBS ; GAS ; POLYCHLOROPHENOLS ; CONTAMINATION ; BIPHENYLS
WOS类目Environmental Sciences
WOS研究方向Environmental Sciences & Ecology
资源类型期刊论文
条目标识符http://119.78.100.177/qdio/handle/2XILL650/192045
作者单位1.Res Ctr Ecoenvironm Sci, State Key Lab Environm Chem & Ecotoxicol, Beijing 100085, Peoples R China;
2.Univ Chinese Acad Sci, 19A Yuquan Rd, Beijing 100049, Peoples R China;
3.Univ Copenhagen, Fac Sci, Dept Plant & Environm Sci, Environm Chem & Phys, Thorvaldsensvej 40, DK-1871 Frederiksberg C, Denmark
推荐引用方式
GB/T 7714
Han, Ying,Liu, Wenbin,Hansen, Hans Chr. Bruun,et al. Influence of long-range atmospheric transportation (LRAT) on mono- to octa-chlorinated PCDD/Fs levels and distributions in soil around Qinghai Lake, China[J],2016,156:143-149.
APA Han, Ying.,Liu, Wenbin.,Hansen, Hans Chr. Bruun.,Chen, Xuebin.,Liao, Xiao.,...&Yan, Nan.(2016).Influence of long-range atmospheric transportation (LRAT) on mono- to octa-chlorinated PCDD/Fs levels and distributions in soil around Qinghai Lake, China.CHEMOSPHERE,156,143-149.
MLA Han, Ying,et al."Influence of long-range atmospheric transportation (LRAT) on mono- to octa-chlorinated PCDD/Fs levels and distributions in soil around Qinghai Lake, China".CHEMOSPHERE 156(2016):143-149.
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