Knowledge Resource Center for Ecological Environment in Arid Area
DOI | 10.5194/acp-16-8157-2016 |
Model development of dust emission and heterogeneous chemistry within the Community Multiscale Air Quality modeling system and its application over East Asia | |
Dong, Xinyi1; Fu, Joshua S.1,2; Huang, Kan1; Tong, Daniel3,4,5; Zhuang, Guoshun6 | |
通讯作者 | Fu, Joshua S. |
来源期刊 | ATMOSPHERIC CHEMISTRY AND PHYSICS
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ISSN | 1680-7316 |
EISSN | 1680-7324 |
出版年 | 2016 |
卷号 | 16期号:13页码:8157-8180 |
英文摘要 | The Community Multiscale Air Quality (CMAQ) model has been further developed in terms of simulating natural wind-blown dust in this study, with a series of modifications aimed at improving the model’s capability to predict the emission, transport, and chemical reactions of dust. The default parameterization of initial threshold friction velocity constants are revised to correct the double counting of the impact of soil moisture in CMAQ by the reanalysis of field experiment data; source-dependent speciation profiles for dust emission are derived based on local measurements for the Gobi and Taklamakan deserts in East Asia; and dust heterogeneous chemistry is also implemented. The improved dust module in the CMAQ is applied over East Asia for March and April from 2006 to 2010. The model evaluation result shows that the simulation bias of PM10 and aerosol optical depth (AOD) is reduced, respectively, from -55.42 and -31.97% by the original CMAQ to -16.05 and -22.1% by the revised CMAQ. Comparison with observations at the nearby Gobi stations of Duolun and Yulin indicates that applying a source-dependent profile helps reduce simulation bias for trace metals. Implementing heterogeneous chemistry also results in better agreement with observations for sulfur dioxide (SO2), sulfate (SO42-), nitric acid (HNO3), nitrous oxides (NOx), and nitrate (NO3-). The investigation of a severe dust storm episode from 19 to 21 March 2010 suggests that the revised CMAQ is capable of capturing the spatial distribution and temporal variation of dust. The model evaluation also indicates potential uncertainty within the excessive soil moisture used by meteorological simulation. The mass contribution of fine-mode particles in dust emission may be underestimated by 50 %. The revised CMAQ model provides a useful tool for future studies to investigate the emission, transport, and impact of wind-blown dust over East Asia and elsewhere. |
类型 | Article |
语种 | 英语 |
国家 | USA ; Peoples R China |
收录类别 | SCI-E |
WOS记录号 | WOS:000381091400007 |
WOS关键词 | UNDERSTANDING INTERANNUAL VARIATIONS ; PENINSULAR SOUTHEAST-ASIA ; YANGTZE-RIVER DELTA ; MINERAL-DUST ; TROPOSPHERIC CHEMISTRY ; CHEMICAL-COMPOSITION ; SOIL PARTICLES ; UNITED-STATES ; STORM PERIOD ; AFRICAN DUST |
WOS类目 | Environmental Sciences ; Meteorology & Atmospheric Sciences |
WOS研究方向 | Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences |
资源类型 | 期刊论文 |
条目标识符 | http://119.78.100.177/qdio/handle/2XILL650/191569 |
作者单位 | 1.Univ Tennessee, Dept Civil & Environm Engn, Knoxville, TN 37996 USA; 2.Oak Ridge Natl Lab, Climate Change Sci Inst, Oak Ridge, TN 37831 USA; 3.NOAA, OAR, ARL, Ctr Weather & Climate Predict, College Pk, MD 20740 USA; 4.George Mason Univ, Ctr Spatial Informat Sci & Syst, Fairfax, VA 22030 USA; 5.Univ Maryland, Cooperat Inst Climate & Satellites, College Pk, MD 20740 USA; 6.Fudan Univ, Dept Environm Sci & Engn, Ctr Atmospher Chem Study, Shanghai 200433, Peoples R China |
推荐引用方式 GB/T 7714 | Dong, Xinyi,Fu, Joshua S.,Huang, Kan,et al. Model development of dust emission and heterogeneous chemistry within the Community Multiscale Air Quality modeling system and its application over East Asia[J],2016,16(13):8157-8180. |
APA | Dong, Xinyi,Fu, Joshua S.,Huang, Kan,Tong, Daniel,&Zhuang, Guoshun.(2016).Model development of dust emission and heterogeneous chemistry within the Community Multiscale Air Quality modeling system and its application over East Asia.ATMOSPHERIC CHEMISTRY AND PHYSICS,16(13),8157-8180. |
MLA | Dong, Xinyi,et al."Model development of dust emission and heterogeneous chemistry within the Community Multiscale Air Quality modeling system and its application over East Asia".ATMOSPHERIC CHEMISTRY AND PHYSICS 16.13(2016):8157-8180. |
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