Arid
DOI10.5194/acp-16-8227-2016
Inventory of African desert dust events in the north-central Iberian Peninsula in 2003-2014 based on sun-photometer-AERONET and particulate-mass-EMEP data
Cachorro, Victoria E.1; Burgos, Maria A.1; Mateos, David1; Toledano, Carlos1; Bennouna, Yasmine1; Torres, Benjamin1; de Frutos, Angel M.1; Herguedas, Alvaro2
通讯作者Cachorro, Victoria E.
来源期刊ATMOSPHERIC CHEMISTRY AND PHYSICS
ISSN1680-7316
EISSN1680-7324
出版年2016
卷号16期号:13页码:8227-8248
英文摘要

A reliable identification of desert dust (DD) episodes over north-central Spain is carried out based on the AErosol RObotic NETwork (AERONET) columnar aerosol sun photometer (aerosol optical depth, AOD, and Angstrom exponent, alpha) and European Monitoring and Evaluation Programme (EMEP) surface particulate-mass concentration (PMx, x = 10, 2.5, and 2.5-10 mu m) as the main core data. The impact of DD on background aerosol conditions is detectable by means of aerosol load thresholds and complementary information provided by HYSPLIT (Hybrid Single Particle Lagrangian Integrated Trajectory Model) air mass back trajectories, MODIS (Moderate Resolution Imaging Spectro-radiometer) images, forecast aerosol models, and synoptic maps, which have been carefully reviewed by a human observer for each day included in the DD inventory. This identification method allows the detection of low and moderate DD intrusions and also of mixtures of mineral dust with other aerosol types by means of the analysis of alpha. During the period studied (2003-2014), a total of 152 DD episodes composed of 418 days are identified. Overall, this means similar to 13 episodes and similar to 35 days per year with DD intrusion, representing 9.5% days year(-1). During the identified DD intrusions, 19 daily exceedances over 50 mu g m(-3) are reported at the surface. The occurrence of DD event days during the year peaks in March and June, with a marked minimum in April and lowest occurrence in winter. A large interannual variability is observed showing a statistically significant temporal decreasing trend of similar to 3 days year(-1). The DD impact on the aerosol climatology is addressed by evaluating the DD contribution in magnitude and percent (in brackets) for AOD, PM10, PM2.5, and PM2.5-10, obtaining mean values of 0.015 (11.5 %), 1.3 mu g m(-3) (11.8 %), 0.55 mu g m(-3) (8.5 %) and 0.79 mu g m(-3) (16.1 %), respectively. Annual cycles of the DD contribution for AOD and PM10 present two maxima one in summer (0.03 and 2.4 mu g m(-3) for AOD in June and PM10 in August) and another in March (0.02 for AOD and 2.2 mu g m(-3) for PM10) - both displaying a similar evolution with exceptions in July and September. The seasonal cycle of the DD contribution to AOD does not follow the pattern of the total AOD (close to a bell shape), whereas both PM10 cycles (total and DD contribution) are more similar to each other in shape, with an exception in September. The interannual evolution of the DD contribution to AOD and PM10 has evidenced a progressive decrease. This decline in the levels of mineral dust aerosols can explain up to 30% of the total aerosol load decrease observed in the study area during the period 2003-2014. The relationship between columnar and surface DD contribution shows a correlation coefficient of 0.81 for the interannual averages. Finally, synoptic conditions during DD events are also analysed, observing that the north African thermal low causes most of the events (similar to 53 %). The results presented in this study highlight the relevance of the area studied since it can be considered representative of the clean background in the western Mediterranean Basin where DD events have a high impact on aerosol load levels.


类型Article
语种英语
国家Spain
收录类别SCI-E
WOS记录号WOS:000381091400011
WOS关键词AEROSOL OPTICAL DEPTH ; SAHARAN DUST ; AIR-QUALITY ; MEDITERRANEAN BASIN ; ATMOSPHERIC AEROSOLS ; SOUTHEASTERN SPAIN ; TRENDS ; TRANSPORT ; VARIABILITY ; EUROPE
WOS类目Environmental Sciences ; Meteorology & Atmospheric Sciences
WOS研究方向Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
资源类型期刊论文
条目标识符http://119.78.100.177/qdio/handle/2XILL650/191568
作者单位1.Univ Valladolid, Fac Ciencias, Grp Opt Atmosfer, Paseo Belen 7, E-47011 Valladolid, Spain;
2.Consejeria Fomento & Medio Ambiente Junta Castill, Dept Control Calidad & Cambio Climat, Valladolid, Spain
推荐引用方式
GB/T 7714
Cachorro, Victoria E.,Burgos, Maria A.,Mateos, David,et al. Inventory of African desert dust events in the north-central Iberian Peninsula in 2003-2014 based on sun-photometer-AERONET and particulate-mass-EMEP data[J],2016,16(13):8227-8248.
APA Cachorro, Victoria E..,Burgos, Maria A..,Mateos, David.,Toledano, Carlos.,Bennouna, Yasmine.,...&Herguedas, Alvaro.(2016).Inventory of African desert dust events in the north-central Iberian Peninsula in 2003-2014 based on sun-photometer-AERONET and particulate-mass-EMEP data.ATMOSPHERIC CHEMISTRY AND PHYSICS,16(13),8227-8248.
MLA Cachorro, Victoria E.,et al."Inventory of African desert dust events in the north-central Iberian Peninsula in 2003-2014 based on sun-photometer-AERONET and particulate-mass-EMEP data".ATMOSPHERIC CHEMISTRY AND PHYSICS 16.13(2016):8227-8248.
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