Arid
DOI10.1016/j.jenvrad.2015.06.009
Mechanical environmental transport of actinides and Cs-137 from an arid radioactive waste disposal site
Snow, Mathew S.1,2; Clark, Sue B.1; Morrison, Samuel S.1; Watrous, Matthew G.2; Olson, John E.2; Snyder, Darin C.2
通讯作者Snow, Mathew S.
来源期刊JOURNAL OF ENVIRONMENTAL RADIOACTIVITY
ISSN0265-931X
EISSN1879-1700
出版年2015
卷号148页码:42-49
英文摘要

Aeolian and pluvial processes represent important mechanisms for the movement of actinides and fission products at the Earth’s surface. Soil samples taken in the early 1970’s near a Department of Energy radioactive waste disposal site (the Subsurface Disposal Area, SDA, located in southeastern Idaho) provide a case study for studying the mechanisms and characteristics of environmental actinide and Cs-137 transport in an arid environment. Multi-component mixing models suggest actinide contamination within 2.5 km of the SDA can be described by mixing between 2 distinct SDA end members and regional nuclear weapons fallout. The absence of chemical fractionation between Am-241 and Pu239+240 with depth for samples beyond the northeastern corner and lack of 241Am in-growth over time (due to Pu-241 decay) suggest mechanical transport and mixing of discrete contaminated particles under arid conditions. Occasional samples northeast of the SDA (the direction of the prevailing winds) contain anomalously high concentrations of Pu with Pu-240/Pu-239 isotopic ratios statistically identical to those in the northeastern corner. Taken together, these data suggest flooding resulted in mechanical transport of contaminated particles into the area between the SDA and a flood containment dike in the northeastern corner, following which subsequent contamination spreading in the northeastern direction resulted from wind transport of discrete particles. (C) 2015 Elsevier Ltd. All rights reserved.


英文关键词Plutonium Americium Pu Am-241 Cs-137 Wind Flood Particulate
类型Article
语种英语
国家USA
收录类别SCI-E
WOS记录号WOS:000361162100006
WOS关键词SNAKE RIVER PLAIN ; VERTICAL MIGRATION ; SOIL-EROSION ; IDAHO SOIL ; PU-239,PU-240 ; CONTAMINATION ; PLUTONIUM ; PU-238 ; AM-241 ; RATES
WOS类目Environmental Sciences
WOS研究方向Environmental Sciences & Ecology
资源类型期刊论文
条目标识符http://119.78.100.177/qdio/handle/2XILL650/188565
作者单位1.Washington State Univ, Dept Chem, Pullman, WA 99164 USA;
2.Idaho Natl Lab, Idaho Falls, ID 83415 USA
推荐引用方式
GB/T 7714
Snow, Mathew S.,Clark, Sue B.,Morrison, Samuel S.,et al. Mechanical environmental transport of actinides and Cs-137 from an arid radioactive waste disposal site[J],2015,148:42-49.
APA Snow, Mathew S.,Clark, Sue B.,Morrison, Samuel S.,Watrous, Matthew G.,Olson, John E.,&Snyder, Darin C..(2015).Mechanical environmental transport of actinides and Cs-137 from an arid radioactive waste disposal site.JOURNAL OF ENVIRONMENTAL RADIOACTIVITY,148,42-49.
MLA Snow, Mathew S.,et al."Mechanical environmental transport of actinides and Cs-137 from an arid radioactive waste disposal site".JOURNAL OF ENVIRONMENTAL RADIOACTIVITY 148(2015):42-49.
条目包含的文件
条目无相关文件。
个性服务
推荐该条目
保存到收藏夹
导出为Endnote文件
谷歌学术
谷歌学术中相似的文章
[Snow, Mathew S.]的文章
[Clark, Sue B.]的文章
[Morrison, Samuel S.]的文章
百度学术
百度学术中相似的文章
[Snow, Mathew S.]的文章
[Clark, Sue B.]的文章
[Morrison, Samuel S.]的文章
必应学术
必应学术中相似的文章
[Snow, Mathew S.]的文章
[Clark, Sue B.]的文章
[Morrison, Samuel S.]的文章
相关权益政策
暂无数据
收藏/分享

除非特别说明,本系统中所有内容都受版权保护,并保留所有权利。