Knowledge Resource Center for Ecological Environment in Arid Area
DOI | 10.1016/j.jenvrad.2015.06.009 |
Mechanical environmental transport of actinides and Cs-137 from an arid radioactive waste disposal site | |
Snow, Mathew S.1,2; Clark, Sue B.1; Morrison, Samuel S.1; Watrous, Matthew G.2; Olson, John E.2; Snyder, Darin C.2 | |
通讯作者 | Snow, Mathew S. |
来源期刊 | JOURNAL OF ENVIRONMENTAL RADIOACTIVITY
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ISSN | 0265-931X |
EISSN | 1879-1700 |
出版年 | 2015 |
卷号 | 148页码:42-49 |
英文摘要 | Aeolian and pluvial processes represent important mechanisms for the movement of actinides and fission products at the Earth’s surface. Soil samples taken in the early 1970’s near a Department of Energy radioactive waste disposal site (the Subsurface Disposal Area, SDA, located in southeastern Idaho) provide a case study for studying the mechanisms and characteristics of environmental actinide and Cs-137 transport in an arid environment. Multi-component mixing models suggest actinide contamination within 2.5 km of the SDA can be described by mixing between 2 distinct SDA end members and regional nuclear weapons fallout. The absence of chemical fractionation between Am-241 and Pu239+240 with depth for samples beyond the northeastern corner and lack of 241Am in-growth over time (due to Pu-241 decay) suggest mechanical transport and mixing of discrete contaminated particles under arid conditions. Occasional samples northeast of the SDA (the direction of the prevailing winds) contain anomalously high concentrations of Pu with Pu-240/Pu-239 isotopic ratios statistically identical to those in the northeastern corner. Taken together, these data suggest flooding resulted in mechanical transport of contaminated particles into the area between the SDA and a flood containment dike in the northeastern corner, following which subsequent contamination spreading in the northeastern direction resulted from wind transport of discrete particles. (C) 2015 Elsevier Ltd. All rights reserved. |
英文关键词 | Plutonium Americium Pu Am-241 Cs-137 Wind Flood Particulate |
类型 | Article |
语种 | 英语 |
国家 | USA |
收录类别 | SCI-E |
WOS记录号 | WOS:000361162100006 |
WOS关键词 | SNAKE RIVER PLAIN ; VERTICAL MIGRATION ; SOIL-EROSION ; IDAHO SOIL ; PU-239,PU-240 ; CONTAMINATION ; PLUTONIUM ; PU-238 ; AM-241 ; RATES |
WOS类目 | Environmental Sciences |
WOS研究方向 | Environmental Sciences & Ecology |
资源类型 | 期刊论文 |
条目标识符 | http://119.78.100.177/qdio/handle/2XILL650/188565 |
作者单位 | 1.Washington State Univ, Dept Chem, Pullman, WA 99164 USA; 2.Idaho Natl Lab, Idaho Falls, ID 83415 USA |
推荐引用方式 GB/T 7714 | Snow, Mathew S.,Clark, Sue B.,Morrison, Samuel S.,et al. Mechanical environmental transport of actinides and Cs-137 from an arid radioactive waste disposal site[J],2015,148:42-49. |
APA | Snow, Mathew S.,Clark, Sue B.,Morrison, Samuel S.,Watrous, Matthew G.,Olson, John E.,&Snyder, Darin C..(2015).Mechanical environmental transport of actinides and Cs-137 from an arid radioactive waste disposal site.JOURNAL OF ENVIRONMENTAL RADIOACTIVITY,148,42-49. |
MLA | Snow, Mathew S.,et al."Mechanical environmental transport of actinides and Cs-137 from an arid radioactive waste disposal site".JOURNAL OF ENVIRONMENTAL RADIOACTIVITY 148(2015):42-49. |
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