Arid
DOI10.5194/acp-15-9501-2015
Quantifying the contribution of long-range transport to particulate matter (PM) mass loadings at a suburban site in the north-western Indo-Gangetic Plain (NW-IGP)
Pawar, H.1; Garg, S.1; Kumar, V.1; Sachan, H.1; Arya, R.1,2; Sarkar, C.1; Chandra, B. P.1; Sinha, B.1
通讯作者Sinha, B.
来源期刊ATMOSPHERIC CHEMISTRY AND PHYSICS
ISSN1680-7316
EISSN1680-7324
出版年2015
卷号15期号:16页码:9501-9520
英文摘要

Many sites in the densely populated Indo-Gangetic Plain (IGP) frequently exceed the national ambient air quality standard (NAAQS) of 100 mu g m(-3) for 24 h average PM10 and 60 mu g m(-3) for 24 h average PM2.5 mass loadings, exposing residents to hazardous levels of particulate matter (PM) throughout the year.


We quantify the contribution of long-range transport to elevated PM levels and the number of exceedance events through a back-trajectory climatology analysis of air masses arriving at the IISER Mohali Atmospheric Chemistry facility (30.667 degrees N, 76.729 degrees E; 310 m a.m.s.l.) for the period August 2011-June 2013. Air masses arriving at the receptor site were classified into six clusters, which represent synoptic-scale air-mass transport patterns. Long-range transport from the west leads to significant enhancements in the average fine-and coarse-mode PM mass loadings during all seasons. The contribution of long-range transport from the west and south-west (source regions: Arabia, Thar Desert, Middle East and Afghanistan) to coarse-mode PM varied between 9 and 57% of the total PM10-2.5 mass.


Local pollution episodes (wind speed < 1 m s(-1)) contributed to enhanced PM2.5 mass loadings during both the winter and summer seasons and to enhanced coarse-mode PM only during the winter season.


South-easterly air masses (source region: eastern IGP) were associated with significantly lower fine-and coarse-mode PM mass loadings during all seasons.


The fraction of days in each season during which the PM mass loadings exceeded the national ambient air quality standard was controlled by long-range transport to a much lesser degree.


For the local cluster, which represents regional air masses (source region: NW-IGP), the fraction of days during which the national ambient air quality standard (NAAQS) of 60 mu g m(-3) for 24 h average PM2.5 was exceeded varied between 36% of the days associated with this synopticscale transport during the monsoon, and 95% during post-monsoon and winter seasons; the fraction of days during which the NAAQS of 100 mu g m(-3) for the 24 h average PM10 was exceeded, varied between 48% during the monsoon and 98% during the post-monsoon season.


Long-range transport was responsible for both, bringing air masses with a significantly lower fraction of exceedance days from the eastern IGP and air masses with a moderate increase in the fraction of exceedance days from the west (source regions: Arabia, Thar Desert, Middle East and Afghanistan).


In order to bring PM mass loadings into compliance with the NAAQS and to reduce the number of exceedance days, mitigation of regional combustion sources in the NW-IGP needs to be given highest priority.


类型Article
语种英语
国家India ; USA
收录类别SCI-E
WOS记录号WOS:000360646500024
WOS关键词ASIAN SUMMER MONSOON ; AIR-POLLUTION ; AMBIENT AIR ; INTRASEASONAL VARIABILITY ; CHEMICAL-COMPOSITION ; CLUSTER-ANALYSIS ; FINE PARTICLES ; HEALTH-RISKS ; JET-STREAM ; AEROSOLS
WOS类目Environmental Sciences ; Meteorology & Atmospheric Sciences
WOS研究方向Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
资源类型期刊论文
条目标识符http://119.78.100.177/qdio/handle/2XILL650/186060
作者单位1.Indian Inst Sci Educ & Res Mohali, Dept Earth & Environm Sci, Sas Nagar 140306, Punjab, India;
2.Cornell Univ, Sch Chem & Biomol Engn, Ithaca, NY USA
推荐引用方式
GB/T 7714
Pawar, H.,Garg, S.,Kumar, V.,et al. Quantifying the contribution of long-range transport to particulate matter (PM) mass loadings at a suburban site in the north-western Indo-Gangetic Plain (NW-IGP)[J],2015,15(16):9501-9520.
APA Pawar, H..,Garg, S..,Kumar, V..,Sachan, H..,Arya, R..,...&Sinha, B..(2015).Quantifying the contribution of long-range transport to particulate matter (PM) mass loadings at a suburban site in the north-western Indo-Gangetic Plain (NW-IGP).ATMOSPHERIC CHEMISTRY AND PHYSICS,15(16),9501-9520.
MLA Pawar, H.,et al."Quantifying the contribution of long-range transport to particulate matter (PM) mass loadings at a suburban site in the north-western Indo-Gangetic Plain (NW-IGP)".ATMOSPHERIC CHEMISTRY AND PHYSICS 15.16(2015):9501-9520.
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