Arid
DOI10.5194/acp-15-6707-2015
9 Vertical variation of optical properties of mixed Asian dust/pollution plumes according to pathway of air mass transport over East Asia
Shin, S-K1; Mueller, D.2; Lee, C.3; Lee, K. H.4; Shin, D.5; Kim, Y. J.1; Noh, Y. M.6
通讯作者Noh, Y. M.
来源期刊ATMOSPHERIC CHEMISTRY AND PHYSICS
ISSN1680-7316
EISSN1680-7324
出版年2015
卷号15期号:12页码:6707-6720
英文摘要

We use five years (2009-2013) of multiwavelength Raman lidar measurements at Gwangju, South Korea (35.10A degrees N, 126.53A degrees E) for the identification of changes of optical properties of East Asian dust depending on its transport path over China. Profiles of backscatter and extinction coefficients, lidar ratios, and backscatter-related angstrom ngstrom exponents (wavelength pair 355/532 nm) were measured at Gwangju. Linear particle depolarization ratios were used to identify East Asian dust layers. We used backward trajectory modeling to identify the pathway and the vertical position of dust-laden air masses over China during long-range transport. Most cases of Asian dust events can be described by the emission of dust in desert areas and subsequent transport over highly polluted regions of China. The Asian dust plumes could be categorized into two classes according to the height above ground at which these plumes were transported: (case I) the dust layers passed over China at high altitude levels (> 3 km) until arrival over Gwangju, and (case II) the Asian dust layers were transported near the surface and within the lower troposphere (< 3 km) over industrialized areas before they arrived over Gwangju. We find that the optical characteristics of these mixed Asian dust layers over Gwangju differ depending on their vertical position above ground over China and the change of height above ground during transport. The mean linear particle depolarization ratio was 0.21 +/- 0.06 (at 532 nm), the mean lidar ratios were 52 +/- 7 sr at 355 nm and 53 +/- 8 sr at 532 nm, and the mean angstrom ngstrom exponent was 0.74 +/- 0.31 for case I. In contrast, plumes transported at lower altitudes (case II) showed low depolarization ratios (0.13 +/- 0.04 at 532 nm), and higher lidar ratio (63 +/- 9 sr at 355 nm and 62 +/- 8 sr at 532 nm) and angstrom ngstrom exponents (0.98 +/- 0.51). These numbers show that the optical characteristics of mixed Asian plumes are more similar to optical characteristics of urban pollution. We find a decrease of the linear depolarization ratio of the mixed dust/pollution plume depending on transport time if the pollution layer traveled over China at low heights, i.e., below approximately 3 km above ground. In contrast, we do not find such a trend if the dust plumes traveled at heights above 3 km over China. We need a longer time series of lidar measurements in order to determine in a quantitative way the change of optical properties of dust with transport time.


类型Article
语种英语
国家South Korea ; England
收录类别SCI-E
WOS记录号WOS:000357117500010
WOS关键词MULTIWAVELENGTH RAMAN LIDAR ; DEPOLARIZATION RATIO ; AEROSOL CLASSIFICATION ; MACC REANALYSIS ; DUST AEROSOLS ; AIRBORNE HSRL ; MINERAL DUST ; SAHARAN DUST ; ACE-ASIA ; EXTINCTION
WOS类目Environmental Sciences ; Meteorology & Atmospheric Sciences
WOS研究方向Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
资源类型期刊论文
条目标识符http://119.78.100.177/qdio/handle/2XILL650/186052
作者单位1.Gwangju Inst Sci & Technol, Sch Environm Sci & Engn, Gwangju, South Korea;
2.Univ Hertfordshire, Sch Phys Astron & Math, Hatfield AL10 9AB, Herts, England;
3.Korea Meteorol Adm, Seoul, South Korea;
4.Gangneung Wonju Natl Univ, Dept Atmospher & Environm Sci, Kangnung, South Korea;
5.Natl Inst Environm Res, Climate & Air Qual Res Dept, Air Qual Forecasting Ctr, Inchon, South Korea;
6.Gwangju Inst Sci & Technol, IERC, Gwangju, South Korea
推荐引用方式
GB/T 7714
Shin, S-K,Mueller, D.,Lee, C.,et al. 9 Vertical variation of optical properties of mixed Asian dust/pollution plumes according to pathway of air mass transport over East Asia[J],2015,15(12):6707-6720.
APA Shin, S-K.,Mueller, D..,Lee, C..,Lee, K. H..,Shin, D..,...&Noh, Y. M..(2015).9 Vertical variation of optical properties of mixed Asian dust/pollution plumes according to pathway of air mass transport over East Asia.ATMOSPHERIC CHEMISTRY AND PHYSICS,15(12),6707-6720.
MLA Shin, S-K,et al."9 Vertical variation of optical properties of mixed Asian dust/pollution plumes according to pathway of air mass transport over East Asia".ATMOSPHERIC CHEMISTRY AND PHYSICS 15.12(2015):6707-6720.
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