Arid
DOI10.1016/j.wasman.2014.06.018
Field investigation of the quality of fresh and aged leachates from selected landfills receiving e-waste in an arid climate
Kiddee, Peeranart1,2; Naidu, Ravi1,2; Wong, Ming H.3; Hearn, Laurence4; Muller, Jochen F.4
通讯作者Naidu, Ravi
来源期刊WASTE MANAGEMENT
ISSN0956-053X
出版年2014
卷号34期号:11页码:2292-2304
英文摘要

The management of electronic waste (e-waste) is a serious problem worldwide and much of it is landfilled. A survey of four selected landfills in an arid region of South Australia was conducted to determine the proportion of e-waste in municipal waste and the properties of each landfill site. Leachate and groundwater samples were collected upgradient and downgradient of the landfills for analysis of polybrominated diphenyl ethers (PBDEs) and 14 metals and metalloids, including Al, As, Ba, Be, Cd, Co, Cr, Cu, Fe, Ni, Pb, Sb, V and Zn. Our data demonstrate that the selected landfills in South Australia continue to receive municipal waste containing in excess of 6%, or 25,000 tonnes per year, of e-waste. The leachates and groundwater collected from the landfills contained significantly elevated concentrations of Pb with the highest concentration in groundwater of 38 mu g/l, almost four times higher than the Australian drinking water guideline of 10 mu g/l. The presence of PBDEs was detected in both leachate and groundwater samples. Total PBDEs values of 2.13-59.75 ng/l in leachate samples were 10 times higher than in groundwater samples, which recorded a range of 0.41-6.53 ng/l at all sites. Moreover, the concentrations of metals and metalloids in sampled groundwater contained elevated levels of Al, As, Fe, Ni and Pb that exceeded Australian drinking water guideline values. For these reasons potential leaching of these contaminants is of concern and while difficult to attribute elevated contaminant levels to e-waste, we do not recommend continued disposal of e-waste in old landfills that were not originally designed to contain leachates. The survey also revealed temporal variation in the electrical conductivity and concentrations of As, Cd and Pb present in leachates of landfills in arid Mediterranean climates. These results are consistent with the marked variations in rainfall patterns observed for such climates. The solute concentration (EC and other ions including As, Cd and Pb) declines in the leachates during wet winter months (June to September), in contrast to tropical countries where such changes are observed during wet summer months. (C) 2014 Elsevier Ltd. All rights reserved.


英文关键词E-waste Landfill Heavy metals and metalloids PBDEs Leachate Groundwater
类型Article
语种英语
国家Australia ; Peoples R China
收录类别SCI-E
WOS记录号WOS:000343840800045
WOS关键词POLYBROMINATED DIPHENYL ETHERS ; MUNICIPAL SOLID-WASTE ; BROMINATED FLAME RETARDANTS ; ELECTRONIC-WASTE ; POLLUTED GROUNDWATER ; RECYCLING SITE ; WATER ; METALS ; PBDES ; IDENTIFICATION
WOS类目Engineering, Environmental ; Environmental Sciences
WOS研究方向Engineering ; Environmental Sciences & Ecology
资源类型期刊论文
条目标识符http://119.78.100.177/qdio/handle/2XILL650/185218
作者单位1.Univ S Australia, Ctr Environm Risk Assessment & Remediat, Adelaide, SA 5095, Australia;
2.Cooperat Res Ctr Contaminat Assessment & Remediat, Adelaide, SA 5095, Australia;
3.Hong Kong Baptist Univ, Dept Biol, Croucher Inst Environm Sci, Kowloon Tong, Hong Kong, Peoples R China;
4.Univ Queensland, Natl Res Ctr Environm Toxicol, Brisbane, Qld 4072, Australia
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Kiddee, Peeranart,Naidu, Ravi,Wong, Ming H.,et al. Field investigation of the quality of fresh and aged leachates from selected landfills receiving e-waste in an arid climate[J],2014,34(11):2292-2304.
APA Kiddee, Peeranart,Naidu, Ravi,Wong, Ming H.,Hearn, Laurence,&Muller, Jochen F..(2014).Field investigation of the quality of fresh and aged leachates from selected landfills receiving e-waste in an arid climate.WASTE MANAGEMENT,34(11),2292-2304.
MLA Kiddee, Peeranart,et al."Field investigation of the quality of fresh and aged leachates from selected landfills receiving e-waste in an arid climate".WASTE MANAGEMENT 34.11(2014):2292-2304.
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