Arid
DOI10.1002/2013JD021213
Hygroscopic growth of submicron and supermicron aerosols in the marine boundary layer
Zhang, Xiaolu1; Massoli, Paola2; Quinn, Patricia K.3; Bates, Timothy S.3; Cappa, Christopher D.1
通讯作者Cappa, Christopher D.
来源期刊JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES
ISSN2169-897X
EISSN2169-8996
出版年2014
卷号119期号:13
英文摘要

We investigate hygroscopic growth of marine aerosols from three research cruises: Texas Air Quality Study-Gulf of Mexico Atmospheric Composition and Climate Study (TexAQS-GoMACCS) 2006, International Chemistry Experiment in the Arctic Lower Troposphere (ICEALOT) 2008, and California Research at the Nexus of Air Quality and Climate Change (CalNex) 2010. Particle hygroscopic growth was characterized by measuring the effect of water uptake under subsaturated conditions on the aerosol light extinction at 532 nm. Mie theory calculations were utilized to convert the observed optical growth factors (f(ext)(RH)) into physical growth factors (GF) at 85% RH. GF is found to be a more robust measure of aerosol hygroscopic growth than f(ext)(RH), which can be biased by changes in aerosol dry size. Consistent with previous observations, the overall GF(85%) for submicron aerosol depended on the fraction of organics. The submicron GF(OM)(85%) specifically was found to range from 1.0 to 1.3 for all three campaigns. A robust positive linear dependence of the overall supermicron GF(85%) on the mass fraction of sea salt was observed. During TexAQS, two types of dust particles with distinct hygroscopic properties were identified in the supermicron mode; one that originated from the Sahara desert was moderately hygroscopic (GF(dust)(85%) = similar to 1.4) and the other from continental sources was nearly hydrophobic. The GF(85%) of supermicron organics was estimated through hygroscopicity closure calculations. Supermicron organics that originated from marine sources were found to be substantially more hygroscopic than those from continental sources, with the latter having a GF(85%) similar to that of the submicron organics. This study demonstrates the potential of using aerosol optical measurements to retrieve hygroscopic growth factor and underlines the importance and need for future investigations on the hygroscopic properties of marine supermicron aerosols.


类型Article
语种英语
国家USA
收录类别SCI-E
WOS记录号WOS:000340408000036
WOS关键词OPTICAL-PROPERTIES ; RELATIVE-HUMIDITY ; CHEMICAL-COMPOSITION ; ORGANIC AEROSOL ; SCATTERING COEFFICIENT ; SPECIES CONTRIBUTIONS ; MASS-SPECTROMETER ; SEA-SALT ; DASH-SP ; SIZE
WOS类目Meteorology & Atmospheric Sciences
WOS研究方向Meteorology & Atmospheric Sciences
来源机构University of California, Davis
资源类型期刊论文
条目标识符http://119.78.100.177/qdio/handle/2XILL650/183355
作者单位1.Univ Calif Davis, Dept Civil & Environm Engn, Davis, CA 95616 USA;
2.Aerodyne Res Inc, Billerica, MA USA;
3.Natl Ocean & Atmospher Adm, Pacific Marine Environm Lab, Seattle, WA USA
推荐引用方式
GB/T 7714
Zhang, Xiaolu,Massoli, Paola,Quinn, Patricia K.,et al. Hygroscopic growth of submicron and supermicron aerosols in the marine boundary layer[J]. University of California, Davis,2014,119(13).
APA Zhang, Xiaolu,Massoli, Paola,Quinn, Patricia K.,Bates, Timothy S.,&Cappa, Christopher D..(2014).Hygroscopic growth of submicron and supermicron aerosols in the marine boundary layer.JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES,119(13).
MLA Zhang, Xiaolu,et al."Hygroscopic growth of submicron and supermicron aerosols in the marine boundary layer".JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES 119.13(2014).
条目包含的文件
条目无相关文件。
个性服务
推荐该条目
保存到收藏夹
导出为Endnote文件
谷歌学术
谷歌学术中相似的文章
[Zhang, Xiaolu]的文章
[Massoli, Paola]的文章
[Quinn, Patricia K.]的文章
百度学术
百度学术中相似的文章
[Zhang, Xiaolu]的文章
[Massoli, Paola]的文章
[Quinn, Patricia K.]的文章
必应学术
必应学术中相似的文章
[Zhang, Xiaolu]的文章
[Massoli, Paola]的文章
[Quinn, Patricia K.]的文章
相关权益政策
暂无数据
收藏/分享

除非特别说明,本系统中所有内容都受版权保护,并保留所有权利。