Arid
DOI10.1021/es4028698
Optical and Chemical Characterization of Aerosols Emitted from Coal, Heavy and Light Fuel Oil, and Small-Scale Wood Combustion
Frey, Anna K.1; Saarnio, Karri1; Lamberg, Heikki2; Myllari, Fanni3; Karjalainen, Panu3; Teinila, Kimmo1; Carbone, Samara1; Tissari, Jarkko; Niemela, Ville4; Hayrinen, Anna5; Rautiainen, Jani5; Kytomaki, Jorma5; Artaxo, Paulo6; Virkkula, Aki1; Pirjola, Liisa7; Ronkko, Topi3; Keskinen, Jorma3; Jokiniemi, Jorma2,8; Hillamo, Risto1
通讯作者Frey, Anna K.
来源期刊ENVIRONMENTAL SCIENCE & TECHNOLOGY
ISSN0013-936X
EISSN1520-5851
出版年2014
卷号48期号:1页码:827-836
英文摘要

Particle emissions affect radiative forcing in the atmosphere. Therefore, it is essential to know the physical and chemical characteristics of them. This work studied the chemical, physical, and optical characteristics of particle emissions from small-scale wood combustion, coal combustion of a heating and power plant, as well as heavy and light fuel oil combustion at a district heating station. Fine particle (PM1) emissions were the highest in wood combustion with a high fraction of absorbing material. The emissions were lowest from coal combustion mostly because of efficient cleaning techniques used at the power plant. The chemical composition of aerosols from coal and oil combustion included mostly ions and trace elements with a rather low fraction of absorbing material. The single scattering albedo and aerosol forcing efficiency showed that primary particles emitted from wood combustion and some cases of oil combustion would have a clear climate warming effect even over dark earth surfaces. Instead, coal combustion particle emissions had a cooling effect. Secondary processes in the atmosphere will further change the radiative properties of these emissions but are not considered in this study.


类型Article
语种英语
国家Finland ; Brazil
收录类别SCI-E
WOS记录号WOS:000329548800105
WOS关键词SIZE DISTRIBUTIONS ; PARTICULATE MATTER ; PARTICLE EMISSIONS ; ORGANIC AEROSOLS ; MIXING STATE ; DESERT DUST ; ABSORPTION ; URBAN ; CALIBRATION ; SCATTERING
WOS类目Engineering, Environmental ; Environmental Sciences
WOS研究方向Engineering ; Environmental Sciences & Ecology
资源类型期刊论文
条目标识符http://119.78.100.177/qdio/handle/2XILL650/181955
作者单位1.Finnish Meteorol Inst, FI-00101 Helsinki, Finland;
2.Univ Eastern Finland, Dept Environm Sci, Fine Particle & Aerosol Technol Lab, FI-70211 Kuopio, Finland;
3.Tampere Univ Technol, Dept Phys, FI-33101 Tampere, Finland;
4.Dekati Ltd, FI-36240 Kangasala, Finland;
5.Helsingin Energia Plc, FI-00090 Helen, Finland;
6.Univ Sao Paulo, BR-05508900 Sao Paulo, Brazil;
7.Metropolia Univ Appl Sci, Dept Technol, FI-00180 Helsinki, Finland;
8.VTT Tech Res Ctr Finland, FI-02044 Espoo, Finland
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GB/T 7714
Frey, Anna K.,Saarnio, Karri,Lamberg, Heikki,et al. Optical and Chemical Characterization of Aerosols Emitted from Coal, Heavy and Light Fuel Oil, and Small-Scale Wood Combustion[J],2014,48(1):827-836.
APA Frey, Anna K..,Saarnio, Karri.,Lamberg, Heikki.,Myllari, Fanni.,Karjalainen, Panu.,...&Hillamo, Risto.(2014).Optical and Chemical Characterization of Aerosols Emitted from Coal, Heavy and Light Fuel Oil, and Small-Scale Wood Combustion.ENVIRONMENTAL SCIENCE & TECHNOLOGY,48(1),827-836.
MLA Frey, Anna K.,et al."Optical and Chemical Characterization of Aerosols Emitted from Coal, Heavy and Light Fuel Oil, and Small-Scale Wood Combustion".ENVIRONMENTAL SCIENCE & TECHNOLOGY 48.1(2014):827-836.
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