Arid
DOI10.1016/j.atmosenv.2014.04.038
WRF-Chem simulations of aerosols and anthropogenic aerosol radiative forcing in East Asia
Gao, Yi1; Zhao, Chun2; Liu, Xiaohong1,3; Zhang, Meigen1; Leung, L. Ruby2
通讯作者Liu, Xiaohong
来源期刊ATMOSPHERIC ENVIRONMENT
ISSN1352-2310
EISSN1873-2844
出版年2014
卷号92页码:250-266
英文摘要

This study aims to provide a first comprehensive evaluation of WRF-Chem for modeling aerosols and anthropogenic aerosol radiative forcing (RF, including direct, semi-direct and indirect forcing) over East Asia. Several numerical experiments were conducted from November 2007 to December 2008. Comparison between model results and observations shows that the model can generally reproduce the observed spatial distributions of aerosol concentration, aerosol optical depth (AOD) and single scattering albedo (SSA) from measurements at many sites, including the relatively higher aerosol concentration and AOD over East China and the relatively lower AOD over Southeast Asia, Korea, and Japan. The model also depicts the seasonal variation and transport of pollutions over East Asia. Particulate matter of 10 gm or less in the aerodynamic diameter (PM10), black carbon (BC), sulfate (SO42-), nitrate (NO3-) and ammonium (NH4+) concentrations are higher in spring than other seasons in Japan, which indicates the possible influence of pollutant transport from polluted area of East Asia. The model underestimates SO42- and organic carbon (OC) concentrations over mainland China by about a factor of 2, while overestimates NO3- concentration in autumn along the Yangtze River. The model captures the dust events at the Zhangye site in the semi-arid region of China. ADD is high over Southwest and Central China in winter and spring and over North China in winter, spring and summer while is low over South China in summer due to monsoon precipitation. SSA is lowest in winter and highest in summer. Anthropogenic aerosol RF is estimated to range from -5 to -20 W m(-2) over land and -20 to -40 W m(-2) over adjacent oceans at the top of atmosphere (TOA), 5-30 W m(-2) in the atmosphere (ATM) and -15 to -40 W m(-2) at the bottom (BOT). The warming effect of anthropogenic aerosol in ATM results from BC aerosol while the negative aerosol RF at TOA is caused by scattering aerosols such as SO42-, NO3- and NH4+. Positive BC RF at TOA compensates 40-50% of the TOA cooling associated with anthropogenic aerosol. (C) 2014 Elsevier Ltd. All rights reserved.


英文关键词WRF-Chem Anthropogenic aerosol East Asia Radiative forcing
类型Article
语种英语
国家Peoples R China ; USA
收录类别SCI-E
WOS记录号WOS:000338810800028
WOS关键词CLIMATE-CHEMISTRY/AEROSOL MODEL ; BLACK CARBON AEROSOLS ; SEA-SALT AEROSOLS ; REGIONAL CLIMATE ; HYDROLOGICAL CYCLE ; OZONE PRODUCTION ; SULFATE AEROSOL ; SULFUR-DIOXIDE ; MINERAL DUST ; CHINA
WOS类目Environmental Sciences ; Meteorology & Atmospheric Sciences
WOS研究方向Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
来源机构中国科学院大气物理研究所
资源类型期刊论文
条目标识符http://119.78.100.177/qdio/handle/2XILL650/180935
作者单位1.Chinese Acad Sci, Inst Atmospher Phys, State Key Lab Atmospher Boundary Layer Phys & Atm, Beijing, Peoples R China;
2.Pacific NW Natl Lab, Atmospher Sci & Global Change Div, Richland, WA 99352 USA;
3.Univ Wyoming, Dept Atmospher Sci, Laramie, WY 82071 USA
推荐引用方式
GB/T 7714
Gao, Yi,Zhao, Chun,Liu, Xiaohong,et al. WRF-Chem simulations of aerosols and anthropogenic aerosol radiative forcing in East Asia[J]. 中国科学院大气物理研究所,2014,92:250-266.
APA Gao, Yi,Zhao, Chun,Liu, Xiaohong,Zhang, Meigen,&Leung, L. Ruby.(2014).WRF-Chem simulations of aerosols and anthropogenic aerosol radiative forcing in East Asia.ATMOSPHERIC ENVIRONMENT,92,250-266.
MLA Gao, Yi,et al."WRF-Chem simulations of aerosols and anthropogenic aerosol radiative forcing in East Asia".ATMOSPHERIC ENVIRONMENT 92(2014):250-266.
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