Arid
DOI10.1016/j.scitotenv.2013.03.010
Occurrence and fate of eleven classes of antibiotics in two typical wastewater treatment plants in South China
Zhou, Li-Jun; Ying, Guang-Guo; Liu, Shan; Zhao, Jian-Liang; Yang, Bin; Chen, Zhi-Feng; Lai, Hua-Jie
通讯作者Ying, Guang-Guo
来源期刊SCIENCE OF THE TOTAL ENVIRONMENT
ISSN0048-9697
EISSN1879-1026
出版年2013
卷号452页码:365-376
英文摘要

Wastewater treatment plants (WWTPs) are regarded as one of the most important sources of antibiotics in the environment. Two sampling campaigns over a period of one year in two wastewater treatment plants (plant A: activated sludge with chlorination, and plant B: oxidation ditch with UV) of Guangdong Province, China were carried out to assess the occurrence and fate of 11 classes of 50 antibiotics. The wastewater samples were extracted by Oasis HLB cartridges (6 mL, 500 mg), while the solid samples (sludge and suspended solid matter) were extracted by ultrasonic-assisted extraction with solvents (acetonitrile and citric acid buffer), followed by an enrichment and clean-up step with solid-phase extraction using SAX-HLB cartridges in tandem. The results showed the presence of 20 and 17 target compounds in the influents and effluents, respectively, at the concentrations ranging from low ng/L to a few mu g/L. Sulfamethoxazole, norfloxacin, ofloxacin, anhydro erythromycin and trimethoprim were most frequently detected in the WWTPs wastewaters. Twenty-one antibiotics were found in the sewage sludge from the two WWTPs at the concentrations up to 5800 ng/g, with tetracycline, oxytetracycline, norfloxacin and ofloxacin being the predominant antibiotics. The total mass loads of antibiotics per capita in the two plants ranged from 494 to 901 mu g/d/inhabitant (672 +/- 182 mu g/d/inhabitant) in the influents, from 130 to 238 mu g/d/inhabitant (175 +/- 45 mu g/d/inhabitant) in the effluents and from 107 to 307 mu g/d/inhabitant (191 +/- 87.9 mu g/d/inhabitant) in the dewatered sludge, respectively. The aqueous removals for sulfonamides, macrolides, trimethoprim, lincomycin and chloramphenicol in the WWTPs were mainly attributed to the degradation processes, while those for tetracyclines and fluoroquinolones were mainly due to the adsorption onto sludge. (C) 2013 Elsevier B.V. All rights reserved.


英文关键词Antibiotics Wastewater treatment plant Wastewater Sludge Removal Mass balance
类型Article
语种英语
国家Peoples R China
收录类别SCI-E
WOS记录号WOS:000318530600039
WOS关键词SEWAGE-TREATMENT PLANTS ; FLUOROQUINOLONE ANTIBACTERIAL AGENTS ; TANDEM MASS-SPECTROMETRY ; VETERINARY ANTIBIOTICS ; RESISTANCE GENES ; AQUATIC ENVIRONMENT ; SULFONAMIDE ANTIBIOTICS ; NATIONAL RECONNAISSANCE ; RISK-ASSESSMENT ; NORTHERN CHINA
WOS类目Environmental Sciences
WOS研究方向Environmental Sciences & Ecology
资源类型期刊论文
条目标识符http://119.78.100.177/qdio/handle/2XILL650/179889
作者单位Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangzhou 510640, Guangdong, Peoples R China
推荐引用方式
GB/T 7714
Zhou, Li-Jun,Ying, Guang-Guo,Liu, Shan,et al. Occurrence and fate of eleven classes of antibiotics in two typical wastewater treatment plants in South China[J],2013,452:365-376.
APA Zhou, Li-Jun.,Ying, Guang-Guo.,Liu, Shan.,Zhao, Jian-Liang.,Yang, Bin.,...&Lai, Hua-Jie.(2013).Occurrence and fate of eleven classes of antibiotics in two typical wastewater treatment plants in South China.SCIENCE OF THE TOTAL ENVIRONMENT,452,365-376.
MLA Zhou, Li-Jun,et al."Occurrence and fate of eleven classes of antibiotics in two typical wastewater treatment plants in South China".SCIENCE OF THE TOTAL ENVIRONMENT 452(2013):365-376.
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