Arid
DOI10.1016/j.jenvrad.2013.01.005
Recent measurements of U-234/U-238 isotope ratio in spring waters from the Hadzici area
Vidic, Alfred1; Ilic, Zorana1; Benedik, Ljudmila2
通讯作者Vidic, Alfred
来源期刊JOURNAL OF ENVIRONMENTAL RADIOACTIVITY
ISSN0265-931X
出版年2013
卷号120页码:6-13
英文摘要

The Hadzici area has become interesting for investigation since depleted uranium ammunition had been employed in 1995 during the NATO air strike campaign in Bosnia and Herzegovina. The purpose of this study is to determine uranium concentration and U-234/U-238 activity ratio in the spring waters of this area and to investigate their relationship, as well as spatial variations. The spring water samples were taken at 18 sites in total. For the determination of uranium radioisotopes, radiochemical separation procedure followed by alpha-particle spectrometry was applied. Uranium concentration in analyzed waters range from 0.15 to 1.12 mu g/L. Spring waters from carbonate based sediments have a lower uranium concentration of between 0.15 and 0.43 mu g/L, in comparison to waters sampled within sandstone-based sediments ranging from 0.53 to 1.12 mu g/L. Dissolved uranium shows significant spatial variability and correlation with bedrock type confirmed by Principal Component Analysis and Hierarchical Cluster Analysis. The majority of the analyzed waters have a U-234/U-238 activity ratio ranging from 1.02 to 1.90, of which half of the results range between 1.02 and 1.16. No apparent depleted uranium (DU) contamination was observed, as U-234/U-238 activity ratio is dependent on geochemical conditions in the environment. Even though the tested spring waters demonstrate significant variability in uranium concentration, U-234/U-238 activity ratio and U-234 excess, waters with similar uranium isotopic signatures are observable within the region. The guidelines on the spatial redistribution of dissolved uranium (corresponding to U-238 mass concentration), along with U-234/U-238 activity ratios were provided by the Inverse Distance Weighting (IDW) method. Waters having similar isotopic signature have been delineated. (c) 2013 Elsevier Ltd. All rights reserved.


英文关键词Spring water U-234/U-238 activity ratio Alpha spectrometry
类型Article
语种英语
国家Bosnia & Herceg ; Slovenia
收录类别SCI-E
WOS记录号WOS:000317445200002
WOS关键词URANIUM ISOTOPES ; DEPLETED URANIUM ; SURFACE WATERS ; WESTERN DESERT ; GROUNDWATER ; AQUIFER ; DISEQUILIBRIUM ; EGYPT ; GEOCHEMISTRY ; TRACERS
WOS类目Environmental Sciences
WOS研究方向Environmental Sciences & Ecology
资源类型期刊论文
条目标识符http://119.78.100.177/qdio/handle/2XILL650/178293
作者单位1.Inst Publ Hlth FB&H, Sarajevo 71000, Bosnia & Herceg;
2.Jozef Stefan Inst, Ljubljana 1000, Slovenia
推荐引用方式
GB/T 7714
Vidic, Alfred,Ilic, Zorana,Benedik, Ljudmila. Recent measurements of U-234/U-238 isotope ratio in spring waters from the Hadzici area[J],2013,120:6-13.
APA Vidic, Alfred,Ilic, Zorana,&Benedik, Ljudmila.(2013).Recent measurements of U-234/U-238 isotope ratio in spring waters from the Hadzici area.JOURNAL OF ENVIRONMENTAL RADIOACTIVITY,120,6-13.
MLA Vidic, Alfred,et al."Recent measurements of U-234/U-238 isotope ratio in spring waters from the Hadzici area".JOURNAL OF ENVIRONMENTAL RADIOACTIVITY 120(2013):6-13.
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