Arid
DOI10.5194/acp-13-9195-2013
Absorption properties of Mediterranean aerosols obtained from multi-year ground-based remote sensing observations
Mallet, M.1; Dubovik, O.2; Nabat, P.3; Dulac, F.4; Kahn, R.5; Sciare, J.4; Paronis, D.6; Leon, J. F.1
通讯作者Mallet, M.
来源期刊ATMOSPHERIC CHEMISTRY AND PHYSICS
ISSN1680-7316
EISSN1680-7324
出版年2013
卷号13期号:18页码:9195-9210
英文摘要

Aerosol absorption properties are of high importance to assess aerosol impact on regional climate. This study presents an analysis of aerosol absorption products obtained over the Mediterranean basin or land stations in the region from multi-year ground-based AERONET observations with a focus on the Absorbing Aerosol Optical Depth (AAOD), Single Scattering Albedo (SSA) and their spectral dependence. The AAOD and Absorption Angstrom Exponent (AAE) dataset is composed of daily averaged AERONET level 2 data from a total of 22 Mediterranean stations having long time series, mainly under the influence of urban-industrial aerosols and/or soil dust. This dataset covers the 17-yr period 1996-2012 with most data being from 2003-2011 (similar to 89% of level-2 AAOD data). Since AERONET level-2 absorption products require a high aerosol load (AOD at 440 nm >0.4), which is most often related to the presence of desert dust, we also consider level-1.5 SSA data, despite their higher uncertainty, and filter out data with an Angstrom exponent <1.0 in order to study absorption by carbonaceous aerosols. The SSA dataset includes AERONET level-2 products. Sun-photometer observations show that values of AAOD at 440 nm vary between 0.024 +/- 0.01 (resp. 0.040 +/- 0.01) and 0.050 +/- 0.01 (0.055 +/- 0.01) for urban (dusty) sites. Analysis shows that the Mediterranean urban-industrial aerosols appear "moderately" absorbing with values of SSA close to similar to 0.94-0.95 +/- 0.04 (at 440 nm) in most cases except over the large cities of Rome and Athens, where aerosol appears more absorbing (SSA similar to 0.89-0.90 +/- 0.04). The aerosol Absorption Angstrom Exponent (AAE, estimated using 440 and 870 nm) is found to be larger than 1 for most sites over the Mediterranean, a manifestation of mineral dust (iron) and/or brown carbon producing the observed absorption. AERONET level-2 sun-photometer data indicate a possible East-West gradient, with higher values over the eastern basin (AAE(East) = 1.39/AAE(West) = 1.33). The North-South AAE gradient is more pronounced, especially over the western basin. Our additional analysis of AERONET level-1.5 data also shows that organic absorbing aerosols significantly affect some Mediterranean These results indicate that current climate models treating organics as nonabsorbing over the Mediterranean certainly underestimate the warming effect due to carbonaceous aerosols.


类型Article
语种英语
国家France ; USA ; Greece
收录类别SCI-E
WOS记录号WOS:000325283800005
WOS关键词SUMMER AIRBORNE MEASUREMENTS ; OPTICAL-PROPERTIES ; LIGHT-ABSORPTION ; SAHARAN DUST ; URBAN ZONE ; CARBONACEOUS AEROSOLS ; INVERSION ALGORITHM ; BLACK CARBON ; WEST-AFRICA ; AEGEAN SEA
WOS类目Environmental Sciences ; Meteorology & Atmospheric Sciences
WOS研究方向Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
资源类型期刊论文
条目标识符http://119.78.100.177/qdio/handle/2XILL650/175992
作者单位1.UMR5560, Lab Aerol, Toulouse, France;
2.Opt Atmospher Lab, Lille, France;
3.Meteo France, CNRM GAME, Toulouse, France;
4.CEA CNRS USVQ, Lab Sci Climat & Environm IPSL LSCE, Gif Sur Yvette, France;
5.NASA, Goddard Space Flight Ctr, Greenbelt, MD USA;
6.Natl Observ Athens, Inst Astron Astrophys Space Applicat & Remote Sen, Athens, Greece
推荐引用方式
GB/T 7714
Mallet, M.,Dubovik, O.,Nabat, P.,et al. Absorption properties of Mediterranean aerosols obtained from multi-year ground-based remote sensing observations[J],2013,13(18):9195-9210.
APA Mallet, M..,Dubovik, O..,Nabat, P..,Dulac, F..,Kahn, R..,...&Leon, J. F..(2013).Absorption properties of Mediterranean aerosols obtained from multi-year ground-based remote sensing observations.ATMOSPHERIC CHEMISTRY AND PHYSICS,13(18),9195-9210.
MLA Mallet, M.,et al."Absorption properties of Mediterranean aerosols obtained from multi-year ground-based remote sensing observations".ATMOSPHERIC CHEMISTRY AND PHYSICS 13.18(2013):9195-9210.
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