Arid
DOI10.5194/acp-13-7097-2013
Dust vertical profile impact on global radiative forcing estimation using a coupled chemical-transport-radiative-transfer model
Zhang, L.1,2,3; Li, Q. B.1,2; Gu, Y.1,2; Liou, K. N.1,2; Meland, B.3
通讯作者Zhang, L.
来源期刊ATMOSPHERIC CHEMISTRY AND PHYSICS
ISSN1680-7316
EISSN1680-7324
出版年2013
卷号13期号:14页码:7097-7114
英文摘要

Atmospheric mineral dust particles exert significant direct radiative forcings and are important drivers of climate and climate change. We used the GEOS-Chem global three-dimensional chemical transport model (CTM) coupled with the Fu-Liou-Gu (FLG) radiative transfer model (RTM) to investigate the dust radiative forcing and heating rate based on different vertical profiles for April 2006. We attempt to actually quantify the sensitivities of radiative forcing to dust vertical profiles, especially the discrepancies between using realistic and climatological vertical profiles. In these calculations, dust emissions were constrained by observations of aerosol optical depth (AOD). The coupled calculations utilizing a more realistic dust vertical profile simulated by GEOS-Chem minimize the physical inconsistencies between 3-D CTM aerosol fields and the RTM. The use of GEOS-Chem simulated vertical profile of dust extinction, as opposed to the FLG prescribed vertical profile, leads to greater and more spatially heterogeneous changes in the estimated radiative forcing and heating rate produced by dust. Both changes can be attributed to a different vertical structure between dust and non-dust source regions. Values of the dust vertically resolved AOD per grid level (VRAOD) are much larger in the middle troposphere, though smaller at the surface when the GEOS-Chem simulated vertical profile is used, which leads to a much stronger heating rate in the middle troposphere. Compared to the FLG vertical profile, the use of GEOS-Chem vertical profile reduces the solar radiative forcing at the top of atmosphere (TOA) by approximately 0.2-0.25 W m(-2) over the African and Asian dust source regions. While the Infrared (IR) radiative forcing decreases 0.2 W m(-2) over African dust belt, it increases 0.06 W m(-2) over the Asian dust belt when the GEOS-Chem vertical profile is used. Differences in the solar radiative forcing at the surface between the use of the GEOS-Chem and FLG vertical profiles are most significant over the Gobi desert with a value of about 1.1 W m(-2). The radiative forcing effect of dust particles is more pronounced at the surface over the Sahara and Gobi deserts by using FLG vertical profile, while it is less significant over the downwind area of Eastern Asia.


类型Article
语种英语
国家USA
收录类别SCI-E
WOS记录号WOS:000322448300023
WOS关键词GENERAL-CIRCULATION MODEL ; PARTICLE-SIZE DISTRIBUTION ; SEA-SALT AEROSOLS ; SAHARAN DUST ; MINERAL DUST ; UNITED-STATES ; SATELLITE-OBSERVATIONS ; GOCART MODEL ; ASIAN DUST ; PARAMETERIZATION
WOS类目Environmental Sciences ; Meteorology & Atmospheric Sciences
WOS研究方向Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
来源机构University of California, Los Angeles
资源类型期刊论文
条目标识符http://119.78.100.177/qdio/handle/2XILL650/175987
作者单位1.Univ Calif Los Angeles, Dept Atmospher & Ocean Sci, Los Angeles, CA 90095 USA;
2.Univ Calif Los Angeles, Joint Inst Reg Earth Syst Sci & Engn, Los Angeles, CA 90095 USA;
3.Univ Colorado, Dept Mech Engn, Boulder, CO 80309 USA
推荐引用方式
GB/T 7714
Zhang, L.,Li, Q. B.,Gu, Y.,et al. Dust vertical profile impact on global radiative forcing estimation using a coupled chemical-transport-radiative-transfer model[J]. University of California, Los Angeles,2013,13(14):7097-7114.
APA Zhang, L.,Li, Q. B.,Gu, Y.,Liou, K. N.,&Meland, B..(2013).Dust vertical profile impact on global radiative forcing estimation using a coupled chemical-transport-radiative-transfer model.ATMOSPHERIC CHEMISTRY AND PHYSICS,13(14),7097-7114.
MLA Zhang, L.,et al."Dust vertical profile impact on global radiative forcing estimation using a coupled chemical-transport-radiative-transfer model".ATMOSPHERIC CHEMISTRY AND PHYSICS 13.14(2013):7097-7114.
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