干旱区生态环境知识资源中心

North China (Huabei in Chinese) is a geographical region located between 32 degrees N and 42 degrees N latitude in eastern China, including several provinces and large municipalities (e. g., Beijing and Tianjin). In the past decades the region has experienced dramatic changes in air quality and climate. Among the multiple causes aerosol pollution is expected to play a particularly important role. To investigate this, a field measurement campaign was performed in April-May 2006 as part of the project Influence of Pollution on Aerosols and Cloud Microphysics in North China. Here we report the first aircraft measurements of atmospheric trace gases, aerosols, and clouds over this part of China, a region strongly affected by both natural desert dust and pollution smog. We observed very high concentrations of gaseous air pollutants and haze particles, partly together with nonprecipitating stratiform clouds. The clouds were characterized by numerous droplets, much smaller than in a less-polluted atmosphere. Our data reveal that the highly efficient coating of dust particles by pollution acids provides the predominant source of cloud condensation nuclei. The pollution-enhanced activation of dust particles into droplets is shown to be remarkably efficient so that clouds even form below 100% relative humidity. Contrary to previous analyses, we find that the haze particles influence the spectral shape of the cloud droplet size distribution such that the indirect climate cooling effect of aerosols on clouds is increased. The widespread haze, combined with low clouds, diminishes air quality and exerts an unusually strong cooling forcing on climate.