Arid
DOI10.1016/j.atmosenv.2010.04.015
Using Si depletion in aerosol to identify the sources of crustal dust in two Chinese megacities
Zhao, Qing1; He, Kebin1; Rahn, Kenneth A.1,2; Ma, Yongliang1; Yang, Fumo3; Duan, Fengkui1
通讯作者He, Kebin
来源期刊ATMOSPHERIC ENVIRONMENT
ISSN1352-2310
EISSN1873-2844
出版年2010
卷号44期号:21-22页码:2615-2624
英文摘要

Depletion of Si in transported dust has been recognized for many years. It can be used to distinguish between transported and local dust in cities, although it rarely has been. Here we use the variations of the Si/Al ratio in 15 months of continuous PM2.5 samples at Beijing (northern China) and Chongqing (southwestern China) to reveal the seasonal patterns of their dust sources. For both cities, peaks of concentration for Si and Al in PM2.5 corresponded with minima of Si/Al, and could often be linked to pulsed air flow from deserts to the northwest. With significant depletion (up to 80%) and homogeneous distribution at urban and rural sites, Si/Al showed a clear seasonal evolution, which decreased from spring to slimmer, increased from fall to winter, and collapsed during Chinese Spring Festival, indicating the dominance of transported dust, local fugitive dust and firework influence, respectively. The low ratios implied that desert dust is a common source during spring at Chongqing, whereas its presence during cold season at Beijing was also more frequent than expected. Failing to recognize the depletion of Si may lead to an overestimate of desert dust by 15%-65% when using the average abundance of Al in crust (6%-8%), as in previous studies. The difference in Si/Al ratio between local and transported dust implies that >60% of the dust at Beijing came from outside the city during the springs of 2004-2006. This result can help resolve the contradictory findings on this topic that have been presented earlier. (C) 2010 Elsevier Ltd. All rights reserved.


英文关键词Elemental indicator Desert dust Local fugitive dust Long-range transport
类型Article
语种英语
国家Peoples R China ; USA
收录类别SCI-E
WOS记录号WOS:000279648400013
WOS关键词POSITIVE MATRIX FACTORIZATION ; LONG-RANGE TRANSPORT ; SOURCE APPORTIONMENT ; MINERAL DUST ; AFRICAN DUST ; ATMOSPHERIC AEROSOLS ; POLLUTION AEROSOLS ; SOURCE PROFILES ; AIR-POLLUTION ; FUGITIVE DUST
WOS类目Environmental Sciences ; Meteorology & Atmospheric Sciences
WOS研究方向Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
来源机构清华大学
资源类型期刊论文
条目标识符http://119.78.100.177/qdio/handle/2XILL650/163366
作者单位1.Tsinghua Univ, State Key Joint Lab Environm Simulat & Pollut Con, Dept Environm Sci & Engn, Beijing 100084, Peoples R China;
2.Univ Rhode Isl, Grad Sch Oceanog, Narragansett, RI 02882 USA;
3.Chinese Acad Sci, Grad Univ, Sch Earth Sci, Beijing 100049, Peoples R China
推荐引用方式
GB/T 7714
Zhao, Qing,He, Kebin,Rahn, Kenneth A.,et al. Using Si depletion in aerosol to identify the sources of crustal dust in two Chinese megacities[J]. 清华大学,2010,44(21-22):2615-2624.
APA Zhao, Qing,He, Kebin,Rahn, Kenneth A.,Ma, Yongliang,Yang, Fumo,&Duan, Fengkui.(2010).Using Si depletion in aerosol to identify the sources of crustal dust in two Chinese megacities.ATMOSPHERIC ENVIRONMENT,44(21-22),2615-2624.
MLA Zhao, Qing,et al."Using Si depletion in aerosol to identify the sources of crustal dust in two Chinese megacities".ATMOSPHERIC ENVIRONMENT 44.21-22(2010):2615-2624.
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